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CN102574886A - 有机金属骨架和其制造方法 - Google Patents

有机金属骨架和其制造方法 Download PDF

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Publication number
CN102574886A
CN102574886A CN2010800369497A CN201080036949A CN102574886A CN 102574886 A CN102574886 A CN 102574886A CN 2010800369497 A CN2010800369497 A CN 2010800369497A CN 201080036949 A CN201080036949 A CN 201080036949A CN 102574886 A CN102574886 A CN 102574886A
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CN
China
Prior art keywords
metal
skeleton
organometallic skeletal
irmof
organometallic
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Chinese (zh)
Inventor
克里斯蒂安·J·杜南
威廉·莫里斯
奥玛尔·M·亚纪
王博
邓鹤翔
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University of California San Diego UCSD
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University of California San Diego UCSD
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    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07F—ACYCLIC, CARBOCYCLIC OR HETEROCYCLIC COMPOUNDS CONTAINING ELEMENTS OTHER THAN CARBON, HYDROGEN, HALOGEN, OXYGEN, NITROGEN, SULFUR, SELENIUM OR TELLURIUM
    • C07F19/00—Metal compounds according to more than one of main groups C07F1/00 - C07F17/00
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07F—ACYCLIC, CARBOCYCLIC OR HETEROCYCLIC COMPOUNDS CONTAINING ELEMENTS OTHER THAN CARBON, HYDROGEN, HALOGEN, OXYGEN, NITROGEN, SULFUR, SELENIUM OR TELLURIUM
    • C07F3/00—Compounds containing elements of Groups 2 or 12 of the Periodic Table
    • C07F3/003—Compounds containing elements of Groups 2 or 12 of the Periodic Table without C-Metal linkages
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J20/00—Solid sorbent compositions or filter aid compositions; Sorbents for chromatography; Processes for preparing, regenerating or reactivating thereof
    • B01J20/22—Solid sorbent compositions or filter aid compositions; Sorbents for chromatography; Processes for preparing, regenerating or reactivating thereof comprising organic material
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J20/00—Solid sorbent compositions or filter aid compositions; Sorbents for chromatography; Processes for preparing, regenerating or reactivating thereof
    • B01J20/22—Solid sorbent compositions or filter aid compositions; Sorbents for chromatography; Processes for preparing, regenerating or reactivating thereof comprising organic material
    • B01J20/223—Solid sorbent compositions or filter aid compositions; Sorbents for chromatography; Processes for preparing, regenerating or reactivating thereof comprising organic material containing metals, e.g. organo-metallic compounds, coordination complexes
    • B01J20/226—Coordination polymers, e.g. metal-organic frameworks [MOF], zeolitic imidazolate frameworks [ZIF]
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J31/00—Catalysts comprising hydrides, coordination complexes or organic compounds
    • B01J31/16—Catalysts comprising hydrides, coordination complexes or organic compounds containing coordination complexes
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J31/00—Catalysts comprising hydrides, coordination complexes or organic compounds
    • B01J31/16—Catalysts comprising hydrides, coordination complexes or organic compounds containing coordination complexes
    • B01J31/1691—Coordination polymers, e.g. metal-organic frameworks [MOF]
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J31/00—Catalysts comprising hydrides, coordination complexes or organic compounds
    • B01J31/16—Catalysts comprising hydrides, coordination complexes or organic compounds containing coordination complexes
    • B01J31/22—Organic complexes
    • B01J31/2265—Carbenes or carbynes, i.e.(image)
    • B01J31/2269—Heterocyclic carbenes
    • B01J31/2273—Heterocyclic carbenes with only nitrogen as heteroatomic ring members, e.g. 1,3-diarylimidazoline-2-ylidenes
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07D—HETEROCYCLIC COMPOUNDS
    • C07D235/00—Heterocyclic compounds containing 1,3-diazole or hydrogenated 1,3-diazole rings, condensed with other rings
    • C07D235/02—Heterocyclic compounds containing 1,3-diazole or hydrogenated 1,3-diazole rings, condensed with other rings condensed with carbocyclic rings or ring systems
    • C07D235/04—Benzimidazoles; Hydrogenated benzimidazoles
    • C—CHEMISTRY; METALLURGY
    • C07—ORGANIC CHEMISTRY
    • C07F—ACYCLIC, CARBOCYCLIC OR HETEROCYCLIC COMPOUNDS CONTAINING ELEMENTS OTHER THAN CARBON, HYDROGEN, HALOGEN, OXYGEN, NITROGEN, SULFUR, SELENIUM OR TELLURIUM
    • C07F15/00—Compounds containing elements of Groups 8, 9, 10 or 18 of the Periodic Table
    • C07F15/0006—Compounds containing elements of Groups 8, 9, 10 or 18 of the Periodic Table compounds of the platinum group
    • C07F15/006—Palladium compounds
    • F—MECHANICAL ENGINEERING; LIGHTING; HEATING; WEAPONS; BLASTING
    • F17—STORING OR DISTRIBUTING GASES OR LIQUIDS
    • F17C—VESSELS FOR CONTAINING OR STORING COMPRESSED, LIQUEFIED OR SOLIDIFIED GASES; FIXED-CAPACITY GAS-HOLDERS; FILLING VESSELS WITH, OR DISCHARGING FROM VESSELS, COMPRESSED, LIQUEFIED, OR SOLIDIFIED GASES
    • F17C11/00—Use of gas-solvents or gas-sorbents in vessels
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01D—SEPARATION
    • B01D2253/00—Adsorbents used in seperation treatment of gases and vapours
    • B01D2253/20—Organic adsorbents
    • B01D2253/204—Metal organic frameworks (MOF's)
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01D—SEPARATION
    • B01D2257/00—Components to be removed
    • B01D2257/50—Carbon oxides
    • B01D2257/504—Carbon dioxide
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01D—SEPARATION
    • B01D53/00—Separation of gases or vapours; Recovering vapours of volatile solvents from gases; Chemical or biological purification of waste gases, e.g. engine exhaust gases, smoke, fumes, flue gases, aerosols
    • B01D53/02—Separation of gases or vapours; Recovering vapours of volatile solvents from gases; Chemical or biological purification of waste gases, e.g. engine exhaust gases, smoke, fumes, flue gases, aerosols by adsorption, e.g. preparative gas chromatography
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2531/00—Additional information regarding catalytic systems classified in B01J31/00
    • B01J2531/80—Complexes comprising metals of Group VIII as the central metal
    • B01J2531/82—Metals of the platinum group
    • B01J2531/824—Palladium
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02C—CAPTURE, STORAGE, SEQUESTRATION OR DISPOSAL OF GREENHOUSE GASES [GHG]
    • Y02C20/00—Capture or disposal of greenhouse gases
    • Y02C20/40—Capture or disposal of greenhouse gases of CO2
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P20/00—Technologies relating to chemical industry
    • Y02P20/151—Reduction of greenhouse gas [GHG] emissions, e.g. CO2

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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Engineering & Computer Science (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Inorganic Chemistry (AREA)
  • Materials Engineering (AREA)
  • Analytical Chemistry (AREA)
  • Mechanical Engineering (AREA)
  • General Engineering & Computer Science (AREA)
CN2010800369497A 2009-06-19 2010-06-19 有机金属骨架和其制造方法 Pending CN102574886A (zh)

Applications Claiming Priority (7)

Application Number Priority Date Filing Date Title
US21889109P 2009-06-19 2009-06-19
US61/218,891 2009-06-19
US24735109P 2009-09-30 2009-09-30
US61/247,351 2009-09-30
US30430010P 2010-02-12 2010-02-12
US61/304,300 2010-02-12
PCT/US2010/039284 WO2010148374A2 (en) 2009-06-19 2010-06-19 Organo-metallic frameworks and methods of making same

Publications (1)

Publication Number Publication Date
CN102574886A true CN102574886A (zh) 2012-07-11

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Country Status (5)

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EP (1) EP2443133A4 (ja)
JP (1) JP2012530722A (ja)
KR (1) KR20120096454A (ja)
CN (1) CN102574886A (ja)
WO (1) WO2010148374A2 (ja)

Cited By (14)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN104056598A (zh) * 2014-06-20 2014-09-24 浙江大学 一种MOFs基二氧化碳吸附剂及其制备方法和应用
CN104710559A (zh) * 2015-02-15 2015-06-17 北京理工大学 一种制备金属有机骨架材料薄膜的方法
CN105051269A (zh) * 2013-03-11 2015-11-11 乌第有限合伙公司 金属有机框架及其制备和用途
CN105813711A (zh) * 2013-08-05 2016-07-27 纽麦特科技公司 用于电子气体储存的金属有机骨架材料
CN105860958A (zh) * 2016-04-01 2016-08-17 山西大学 一种Cu2+化学传感器及其制备方法和应用
CN106892945A (zh) * 2015-12-18 2017-06-27 温州大学 一种氮杂环卡宾-钯络合物、其制备方法及应用
CN107855109A (zh) * 2017-11-03 2018-03-30 商丘师范学院 一种提高含锌沸石类唑基骨架材料co2吸附性能的方法
CN108152260A (zh) * 2017-12-23 2018-06-12 福州大学 一种检测尿酸的荧光传感器及其制备方法
CN108290135A (zh) * 2015-11-27 2018-07-17 加利福尼亚大学董事会 具有编织结构的共价有机框架
CN108503853A (zh) * 2018-05-04 2018-09-07 武汉大学 一种基于仲胺基键合的共价有机框架材料及其制备方法和应用
CN109174189A (zh) * 2018-09-07 2019-01-11 辽宁大学 基于PCN-222-Co@TpPa-1的多孔结晶核壳杂化材料及其制备方法和应用
CN111196876A (zh) * 2020-02-14 2020-05-26 武汉大学 具有核酸筛分功能的孔径可调的Co基MOF材料的合成方法及其应用
US11230562B2 (en) 2018-04-25 2022-01-25 Uti Limited Partnership Synthesis of zinc MOF materials
CN114450327A (zh) * 2019-08-29 2022-05-06 乔治亚技术研究公司 金属有机骨架材料及其用途

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EP2155608A4 (en) 2007-05-11 2011-01-12 Univ California ADSORPTIVE GAS SEPARATION OF MULTICOMPOSE GASES
WO2009020745A2 (en) 2007-07-17 2009-02-12 The Regents Of The University Of California Preparation of functionalized zeolitic frameworks
JP5730574B2 (ja) 2007-09-25 2015-06-10 ザ リージェンツ オブ ザ ユニバーシティ オブ カリフォルニア 食用に適した生体適合性金属有機構造体
US8946454B2 (en) 2008-06-05 2015-02-03 The Regents Of The University Of California Chemical framework compositions and methods of use
EP2356072A1 (en) 2008-12-29 2011-08-17 The Regents of the University of California A gas sensor incorporating a porous framework
US8674128B2 (en) 2009-01-15 2014-03-18 The Regents Of The University Of California Conductive organometallic framework
WO2010088629A1 (en) 2009-02-02 2010-08-05 The Regents Of The University Of California Reversible ethylene oxide capture in porous frameworks
EP2438073A4 (en) 2009-06-19 2013-01-02 Univ California MATERIALS FOR AN OPEN FRAME FROM COMPLEX MIXING LIGANDS
US8876953B2 (en) 2009-06-19 2014-11-04 The Regents Of The University Of California Carbon dioxide capture and storage using open frameworks
US9045387B2 (en) 2009-07-27 2015-06-02 The Regents Of The University Of California Oxidative homo-coupling reactions of aryl boronic acids using a porous copper metal-organic framework as a highly efficient heterogeneous catalyst
US8841471B2 (en) 2009-09-25 2014-09-23 The Regents Of The University Of California Open metal organic frameworks with exceptional surface area and high gas storage capacity
CA2804313A1 (en) 2010-07-20 2012-01-26 The Regents Of The University Of California Functionalization of organic molecules using metal-organic frameworks (mofs) as catalysts
US9269473B2 (en) 2010-09-27 2016-02-23 The Regents Of The University Of California Conductive open frameworks
US8852320B2 (en) 2011-01-21 2014-10-07 The Regents Of The University Of California Preparation of metal-triazolate frameworks
JP2014507431A (ja) 2011-02-04 2014-03-27 ザ リージェンツ オブ ザ ユニバーシティー オブ カリフォルニア 金属カテコレート骨格体の製造
EP2766046B1 (en) 2011-10-13 2017-08-02 The Regents of The University of California Metal-organic frameworks with exceptionally large pore aperatures
JP2013111563A (ja) * 2011-11-30 2013-06-10 Sumitomo Chemical Co Ltd 組成物及び該組成物を用いたアンモニア製造方法
JP5829924B2 (ja) * 2012-01-16 2015-12-09 東洋紡株式会社 多孔性複合材料とその製造方法、及び硫化水素ガス除去材
CN102936239B (zh) * 2012-11-16 2014-05-14 山东师范大学 有机配体和基于Cu(I)离子的金属有机框架、其合成方法和应用
EP3074404B1 (en) 2014-02-19 2020-01-01 The Regents of The University of California Acid, solvent, and thermal resistant metal-organic frameworks
EP3074405A2 (en) 2014-03-18 2016-10-05 The Regents of the University of California Mesoscopic materials comprised of ordered superlattices of microporous metal-organic frameworks
WO2015195179A2 (en) 2014-03-28 2015-12-23 The Regents Of The University Of California Metal organic frameworks comprising a plurality of sbus with different metal ions and/or a plurality of organic linking ligands with different functional groups.
DE102014210464B4 (de) * 2014-06-03 2018-02-22 Hydrogenious Technologies Gmbh Verwendung eines Substrates zur Wasserstoffspeicherung
CN108473325A (zh) 2015-11-27 2018-08-31 加利福尼亚大学董事会 沸石咪唑酯框架
US12227526B2 (en) * 2019-04-01 2025-02-18 ExxonMobil Technology and Engineering Company Metal-organic framework materials comprising a diimine scaffold and methods for production thereof

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Cited By (23)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN105051269A (zh) * 2013-03-11 2015-11-11 乌第有限合伙公司 金属有机框架及其制备和用途
CN105051269B (zh) * 2013-03-11 2019-03-19 乌第有限合伙公司 金属有机框架及其制备和用途
CN105813711A (zh) * 2013-08-05 2016-07-27 纽麦特科技公司 用于电子气体储存的金属有机骨架材料
CN105813711B (zh) * 2013-08-05 2019-09-24 纽麦特科技公司 用于电子气体储存的金属有机骨架材料
US9751074B2 (en) 2013-08-05 2017-09-05 Numat Technologies, Inc. Metal organic frameworks for electronic gas storage
CN104056598A (zh) * 2014-06-20 2014-09-24 浙江大学 一种MOFs基二氧化碳吸附剂及其制备方法和应用
CN104710559A (zh) * 2015-02-15 2015-06-17 北京理工大学 一种制备金属有机骨架材料薄膜的方法
CN108290135A (zh) * 2015-11-27 2018-07-17 加利福尼亚大学董事会 具有编织结构的共价有机框架
CN106892945A (zh) * 2015-12-18 2017-06-27 温州大学 一种氮杂环卡宾-钯络合物、其制备方法及应用
CN105860958A (zh) * 2016-04-01 2016-08-17 山西大学 一种Cu2+化学传感器及其制备方法和应用
CN105860958B (zh) * 2016-04-01 2018-07-06 山西大学 一种Cu2+化学传感器及其制备方法和应用
CN107855109A (zh) * 2017-11-03 2018-03-30 商丘师范学院 一种提高含锌沸石类唑基骨架材料co2吸附性能的方法
CN108152260A (zh) * 2017-12-23 2018-06-12 福州大学 一种检测尿酸的荧光传感器及其制备方法
CN108152260B (zh) * 2017-12-23 2019-06-07 福州大学 一种检测尿酸的荧光传感器及其制备方法
US11230562B2 (en) 2018-04-25 2022-01-25 Uti Limited Partnership Synthesis of zinc MOF materials
CN108503853A (zh) * 2018-05-04 2018-09-07 武汉大学 一种基于仲胺基键合的共价有机框架材料及其制备方法和应用
CN108503853B (zh) * 2018-05-04 2020-09-08 武汉大学 一种基于仲胺基键合的共价有机框架材料及其制备方法和应用
CN109174189B (zh) * 2018-09-07 2021-03-05 辽宁大学 基于PCN-222(Co)@TpPa-1的多孔结晶核壳杂化材料及其制备方法和应用
CN109174189A (zh) * 2018-09-07 2019-01-11 辽宁大学 基于PCN-222-Co@TpPa-1的多孔结晶核壳杂化材料及其制备方法和应用
CN114450327A (zh) * 2019-08-29 2022-05-06 乔治亚技术研究公司 金属有机骨架材料及其用途
CN114450327B (zh) * 2019-08-29 2024-04-05 乔治亚技术研究公司 金属有机骨架材料及其用途
CN111196876A (zh) * 2020-02-14 2020-05-26 武汉大学 具有核酸筛分功能的孔径可调的Co基MOF材料的合成方法及其应用
CN111196876B (zh) * 2020-02-14 2021-08-03 武汉大学 具有核酸筛分功能的孔径可调的Co基MOF材料的合成方法及其应用

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Publication number Publication date
EP2443133A4 (en) 2013-02-27
WO2010148374A3 (en) 2011-04-28
EP2443133A2 (en) 2012-04-25
JP2012530722A (ja) 2012-12-06
WO2010148374A2 (en) 2010-12-23
KR20120096454A (ko) 2012-08-30

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Application publication date: 20120711