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DE10351234A1 - Herbizid wirksames Mittel - Google Patents

Herbizid wirksames Mittel Download PDF

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Publication number
DE10351234A1
DE10351234A1 DE10351234A DE10351234A DE10351234A1 DE 10351234 A1 DE10351234 A1 DE 10351234A1 DE 10351234 A DE10351234 A DE 10351234A DE 10351234 A DE10351234 A DE 10351234A DE 10351234 A1 DE10351234 A1 DE 10351234A1
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oder
esters
salts
crops
methyl
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DE10351234A
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Inventor
Gerhard Dr. Schnabel
Detlev Dr. Haase
Roland Dr. Deckwer
Frank Dr. Ziemer
Christopher Dr. Rosinger
David Anthony Dr. Feist
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Bayer CropScience AG
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Bayer CropScience AG
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Priority to DE10351234A priority Critical patent/DE10351234A1/de
Priority to EA200600856A priority patent/EA012521B1/ru
Priority to PCT/EP2004/011893 priority patent/WO2005041654A2/de
Priority to CA002544415A priority patent/CA2544415A1/en
Priority to UAA200606174A priority patent/UA83698C2/ru
Priority to DK04790700T priority patent/DK1681932T3/da
Priority to CNA2004800354706A priority patent/CN1886051A/zh
Priority to BRPI0416159-9A priority patent/BRPI0416159A/pt
Priority to EP04790700A priority patent/EP1681932B1/de
Priority to AU2004285269A priority patent/AU2004285269B2/en
Priority to DE502004006612T priority patent/DE502004006612D1/de
Priority to PL04790700T priority patent/PL1681932T3/pl
Priority to AT04790700T priority patent/ATE389327T1/de
Priority to ES04790700T priority patent/ES2302038T3/es
Priority to US10/976,217 priority patent/US7432226B2/en
Priority to TW093133238A priority patent/TW200517058A/zh
Priority to ARP040104023A priority patent/AR046224A1/es
Publication of DE10351234A1 publication Critical patent/DE10351234A1/de
Priority to ZA200603267A priority patent/ZA200603267B/xx
Priority to IL175359A priority patent/IL175359A0/en
Priority to US12/201,115 priority patent/US20090054236A1/en
Ceased legal-status Critical Current

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    • A—HUMAN NECESSITIES
    • A01—AGRICULTURE; FORESTRY; ANIMAL HUSBANDRY; HUNTING; TRAPPING; FISHING
    • A01N—PRESERVATION OF BODIES OF HUMANS OR ANIMALS OR PLANTS OR PARTS THEREOF; BIOCIDES, e.g. AS DISINFECTANTS, AS PESTICIDES OR AS HERBICIDES; PEST REPELLANTS OR ATTRACTANTS; PLANT GROWTH REGULATORS
    • A01N43/00—Biocides, pest repellants or attractants, or plant growth regulators containing heterocyclic compounds
    • A01N43/34—Biocides, pest repellants or attractants, or plant growth regulators containing heterocyclic compounds having rings with one nitrogen atom as the only ring hetero atom
    • A01N43/40—Biocides, pest repellants or attractants, or plant growth regulators containing heterocyclic compounds having rings with one nitrogen atom as the only ring hetero atom six-membered rings
    • A—HUMAN NECESSITIES
    • A01—AGRICULTURE; FORESTRY; ANIMAL HUSBANDRY; HUNTING; TRAPPING; FISHING
    • A01N—PRESERVATION OF BODIES OF HUMANS OR ANIMALS OR PLANTS OR PARTS THEREOF; BIOCIDES, e.g. AS DISINFECTANTS, AS PESTICIDES OR AS HERBICIDES; PEST REPELLANTS OR ATTRACTANTS; PLANT GROWTH REGULATORS
    • A01N25/00—Biocides, pest repellants or attractants, or plant growth regulators, characterised by their forms, or by their non-active ingredients or by their methods of application, e.g. seed treatment or sequential application; Substances for reducing the noxious effect of the active ingredients to organisms other than pests
    • A01N25/32—Ingredients for reducing the noxious effect of the active substances to organisms other than pests, e.g. toxicity reducing compositions, self-destructing compositions
    • A—HUMAN NECESSITIES
    • A01—AGRICULTURE; FORESTRY; ANIMAL HUSBANDRY; HUNTING; TRAPPING; FISHING
    • A01N—PRESERVATION OF BODIES OF HUMANS OR ANIMALS OR PLANTS OR PARTS THEREOF; BIOCIDES, e.g. AS DISINFECTANTS, AS PESTICIDES OR AS HERBICIDES; PEST REPELLANTS OR ATTRACTANTS; PLANT GROWTH REGULATORS
    • A01N47/00—Biocides, pest repellants or attractants, or plant growth regulators containing organic compounds containing a carbon atom not being member of a ring and having no bond to a carbon or hydrogen atom, e.g. derivatives of carbonic acid
    • A01N47/08—Biocides, pest repellants or attractants, or plant growth regulators containing organic compounds containing a carbon atom not being member of a ring and having no bond to a carbon or hydrogen atom, e.g. derivatives of carbonic acid the carbon atom having one or more single bonds to nitrogen atoms
    • A01N47/28—Ureas or thioureas containing the groups >N—CO—N< or >N—CS—N<
    • A01N47/36—Ureas or thioureas containing the groups >N—CO—N< or >N—CS—N< containing the group >N—CO—N< directly attached to at least one heterocyclic ring; Thio analogues thereof
    • A—HUMAN NECESSITIES
    • A01—AGRICULTURE; FORESTRY; ANIMAL HUSBANDRY; HUNTING; TRAPPING; FISHING
    • A01N—PRESERVATION OF BODIES OF HUMANS OR ANIMALS OR PLANTS OR PARTS THEREOF; BIOCIDES, e.g. AS DISINFECTANTS, AS PESTICIDES OR AS HERBICIDES; PEST REPELLANTS OR ATTRACTANTS; PLANT GROWTH REGULATORS
    • A01N2300/00—Combinations or mixtures of active ingredients covered by classes A01N27/00 - A01N65/48 with other active or formulation relevant ingredients, e.g. specific carrier materials or surfactants, covered by classes A01N25/00 - A01N65/48

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  • Life Sciences & Earth Sciences (AREA)
  • Health & Medical Sciences (AREA)
  • General Health & Medical Sciences (AREA)
  • Dentistry (AREA)
  • Plant Pathology (AREA)
  • Engineering & Computer Science (AREA)
  • Pest Control & Pesticides (AREA)
  • Agronomy & Crop Science (AREA)
  • Wood Science & Technology (AREA)
  • Zoology (AREA)
  • Environmental Sciences (AREA)
  • Toxicology (AREA)
  • Agricultural Chemicals And Associated Chemicals (AREA)

Abstract

Herbizid wirksames Mittel, enthaltend DOLLAR A (A) eine herbizid wirksame Menge an einem oder mehreren Sulfonylharnstoffe aus der Gruppe Metsulfuron, Thifensulfuron, Tribenuron, Chlorsulfuron und deren Salze und Ester und DOLLAR A (B) einer antidotisch wirksamen Menge an einem oder mehreren Safenern aus der Gruppe Mefenpyr, Isoxadifen, Cloquintocet und deren Salze und Ester.

Description

  • Die Erfindung betrifft das technische Gebiet der Pflanzenschutzmittel, insbesondere herbizid wirksame Mittel, enthaltend Sulfonylharnstoff-Safener-Kombinationen (Wirkstoff-Antidot-Kombinationen), die hervorragend für den Einsatz gegen konkurrierende Schadpflanzen in Nutzpflanzenkulturen geeignet sind.
  • Kombinationen von Herbiziden, welche das Enzym Acetolactatsynthase (ALS) hemmen, und Safenern sind bekannt. So sind in EP 0 492 367 A2 Kombinationen verschiedenster ALS-Inhibitoren mit verschiedensten Safenern beschrieben. Allerdings sind die dort spezifisch offenbarten Kombinationen im Hinblick auf Selektivität und Wirkungsspektrum nicht immer ausreichend.
    •
  • Aufgabe der vorliegenden Erfindung war es daher, herbizid wirksame Mittel zu finden, in welchen die Selektivität gegenüber wichtigen Kulturpflanzen erhöht ist bei gleichzeitig hoher Wirksamkeit gegenüber Schadpflanzen. Diese Aufgabe wird überraschend gelöst durch das herbizid wirksame Mittel der vorliegenden Erfindung.
  • Gegenstand der Erfindung ist daher ein herbizid wirksames Mittel, enthaltend
    • (A) eine herbizid wirksame Menge an einem oder mehreren Sulfonylharnstoffen aus der Gruppe Metsulfuron, Thifensulfuron, Tribenuron, Chlorsulfuron und deren Salze und Ester, und
    • (B) einer antidotisch wirksamen Menge an einem oder mehreren Safenern aus der Gruppe Mefenpyr, Isoxadifen, Cloquintocet und deren Salze und Ester.
  • Die Sulfonylharnstoffe A) und die Safener B) können auch in Form ihrer Salze vorliegen, z.B. als Salze mit anorganischen und organischen Gegenionen. Diese Salze sind beispielsweise Metallsalze, insbesondere Alkalimetallsalze oder Erdalkalimetallsalze, insbesondere Natrium- und Kaliumsalze, oder auch Ammoniumsalze oder Salze mit organischen Aminen. Ebenso kann Salzbildung durch Anlagerung einer Säure an basischen Gruppen, wie z.B. Amino und Alkylamino, erfolgen. Geeignete Säuren hierfür sind starke anorganische und organische Säuren, beispielsweise HCl, HBr, H2SO4 oder HNO3. Bevorzugte Salze sind die Alkalimetallsalze wie die Natriumsalze und Kaliumsalze. Die Sulfonylharnstoffe A) können z.B. Salze bilden, bei denen der Wasserstoff der -SO2-NH-Gruppe durch ein für die Landwirtschaft geeignetes Kation ersetzt ist, z.B. eine Metallion wie ein Alkalimetallion, vorzugsweise ein Natrium- oder Kaliumion.
  • Die Sulfonylharnstoffe A) und die Safener B) können auch in Form ihrer Ester vorliegen, insbesondere in Form ihrer Alkylester wie C1-C10-Alkylester. Bei den Sulfonylharnstoffen A) sind besonders bevorzugt Methylester und Ethylester. Bei den Safenern B) sind besonders bevorzugt die Methylester, Ethylester und Methylhexylester.
  • Die Sulfonylharnstoffe (A) sind vorzugsweise ausgewählt aus der Gruppe bestehend aus Metsulfuron-methyl (A1.1), Thifensulfuron-methyl (A2.1), Tribenuron-methyl (A3.1) und (Chlorsulfuron (A4.1) einschließlich der in der Landwirtschaft gebräuchlichen Salze wie der Natriumsalze Metsulfuron-methyl-natrium (A1.2), Thifensulfuron-methyl-natrium (A2.2), Tribenuron-methyl-natrium (A3.2) und Chlorsulfuron-natrium (A4.2). Weiterhin bevorzugt sind Metsulfuron (A1.3), Metsulfuron-natrium (A1.4), Thifensulfuron (A2.3), Thifensulfuron-natrium (A2.4), Tribenuron (A3.3) und Tribenuron-natrium (A3.4). Besonders bevorzugte Sulfonylharnstoffe (A) sind Metsulfuron-methyl (A1.1), Thifensulfuron-methyl (A2.1), Tribenuron-methyl (A3.1) und (Chlorsulfuron (A4.1).
  • Die Safener (B) sind vorzugsweise ausgewählt aus der Gruppe bestehend aus 1-(2,4-Dichlorphenyl)-5-(ethoxycarbonyl)-5-methyl-2-pyrazolin-3-carbonsäureethylester (B1, Mefenpyr-diethyl), 5,5-Diphenyl-2-isoxazolin-carbonsäureethylester (B2, Isoxadifen-ethyl), (5-Chlor-8-chinolinoxy)essigsäure-(1-methylhexyl)-ester (B3, Cloquintocet-mexyl), Mefenpyr-dimethyl (B4), Mefenpyr (B5), Isoxadifen (B6) und Cloquintocet (B7) einschließlich der in der Landwirtschaft gebräuchlichen Salze wie der Natriumsalze. Ein besonders bevorzugter Safener ist Mefenpyr-diethyl (B1).
  • Herbizid wirksame Menge bedeutet im Sinne der Erfindung eine Menge an einem oder mehreren Herbiziden, die geeignet ist, den Pflanzenwuchs negativ zu beeinflussen.
  • Antidotisch wirksame Menge bedeutet im Sinne der Erfindung eine Menge an einem oder mehreren Safenern, die geeignet ist, der phytotoxischen Wirkung eines Herbizids oder Herbizidgemisches an einer Nutzpflanze zumindest teilweise entgegenzuwirken.
  • Von den Verbindungen (A) und (B) umfaßt sind auch alle Stereoisomeren, welche die gleiche topologische Verknüpfung der Atome aufweisen, und deren Gemische. Solche Verbindungen enthalten ein oder mehrere asymmetrische C-Atome oder auch Doppelbindungen, die in den allgemeinen Formeln nicht gesondert angegeben sind. Die durch ihre spezifische Raumform definierten möglichen Stereoisomeren, wie Enantiomere, Diastereomere, Z- und E-Isomere, können nach üblichen Methoden aus Gemischen der Stereoisomeren erhalten oder auch durch stereoselektive Reaktionen in Kombination mit dem Einsatz von stereochemisch reinen Ausgangsstoffen hergestellt werden.
  • Sulfonylharnstoffe (A) sind kommerziell erhältlich und z.B. aus US 4,370,480 , EP 30138 , US 4,701,535 , EP 30142 , EP 202830 und US 4,127,405 bekannt, die ausführliche Angaben zu Herstellungsverfahren und Ausgangsmaterialien enthalten. Auf diese Schriften wird ausdrücklich Bezug genommen, sie gelten durch Zitat als Bestandteil dieser Beschreibung.
  • Safener (B) sind sind kommerziell erhältlich und z.B. aus WO 91/7874, WO 95/7897 und EP 94349 bekannt, die ausführliche Angaben zu Herstellungsverfahren und Ausgangsmaterialien enthalten. Auf diese Schriften wird ausdrücklich Bezug genommen, sie gelten durch Zitat als Bestandteil dieser Beschreibung.
  • Beispiele bevorzugter erfindungsgemäßer Kombinationen von Sulfonylharnstoffen (A) und Safenern (B) sind:
    (A1.1) + (B1), (A1.1) + (B2), (A1.1) + (B3), (A2.1) + (B1), (A2.1) + (B2), (A2.1) + (B3), (A3.1) + (B1), (A3.1) + (B2), (A3.1) + (B3), (A4.1) + (B1), (A4.1) + (B2), (A4.1) + (B3), (A1.2) + (B1), (A1.2) + (B2), (A1.2) + (B3), (A2.2) + (B1), (A2.2) + (B2), (A2.2) + (B3), (A3.2) + (B1), (A3.2) + (B2), (A3.2) + (B3), (A4.2) + (B1), (A4.2) + (B2), (A4.2) + (B3), (A1.3) + (B1), (A1.3) + (B2), (A1.3) + (B3), (A2.3) + (B1), (A2.3) + (B2), (A2.3) + (B3), (A3.3) + (B1), (A3.3) + (B2), (A3.3) + (B3), (A1.4) + (B1), (A1.4) + (B2), (A1.4) + (B3), (A2.4) + (B1), (A2.4) + (B2), (A2.4) + (B3), (A3.4) + (B1), (A3.4) + (B2), (A3.4) + (B3);
    (A1.1) + (A1.2) + (B1), (A1.1) + (A2.1) + (B1), (A1.1) + (A2.2) + (B1), (A1.1) + (A3.1) + (B1), (A1.1) + (A3.2) + (B1), (A1.1) + (A4.1) + (B1), (A1.1) + (A4.2) + (B1);
    (A1.2) + (A2.1) + (B1), (A1.2) + (A2.2) + (B1), (A1.2) + (A3.1) + (B1), (A1.2) + (A3.2) + (B1), (A1.2) + (A4.1) + (B1), (A1.2) + (A4.2) + (B1);
    (A2.1) + (A2.2) + (B1), (A2.1) + (A3.1) + (B1), (A2.1) + (A3.2) + (B1), (A2.1) + (A4.1) + (B1), (A2.1) + (A4.2) + (B1);
    (A2.2) + (A3.1) + (B1), (A2.2) + (A3.2) + (B1), (A2.2) + (A4.1) + (B1), (A2.2) + (A4.2) + (B1);
    (A3.1) + (A3.2) + (B1), (A3.1) + (A4.1) + (B1), (A3.1) + (A4.2) + (B1); (A3.2) + (A4.1) + (B1), (A3.2) + (A4.2) + (B1), (A4.1) + (A4.2) + (B1);
    (A1.1) + (A1.2) + (B2), (A1.1) + (A2.1) + (B2), (A1.1) + (A2.2) + (B2), (A1.1) + (A3.1) + (B2), (A1.1) + (A3.2) + (B2), (A1.1) + (A4.1) + (B2), (A1.1) + (A4.2) + (B2);
    (A1.2) + (A2.1) + (B2), (A1.2) + (A2.2) + (B2), (A1.2) + (A3.1) + (B2), (A1.2) + (A3.2) + (B2), (A1.2) + (A4.1) + (B2), (A1.2) + (A4.2) + (B2);
    (A2.1) + (A2.2) + (B2), (A2.1) + (A3.1) + (B2), (A2.1) + (A3.2) + (B2), (A2.1) + (A4.1) + (B2), (A2.1) + (A4.2) + (B2);
    (A2.2) + (A3.1) + (B2), (A2.2) + (A3.2) + (B2), (A2.2) + (A4.1) + (B2), (A2.2) + (A4.2) + (B2);
    (A3.1) + (A3.2) + (B2), (A3.1) + (A4.1) + (B2), (A3.1) + (A4.2) + (B2); (A3.2) + (A4.1) + (B2), (A3.2) + (A4.2) + (B2), (A4.1) + (A4.2) + (B2);
    (A1.1) + (A1.2) + (B3), (A1.1) + (A2.1) + (B3), (A1.1) + (A2.2) + (B3), (A1.1) + (A3.1) + (B3), (A1.1) + (A3.2) + (B3), (A1.1) + (A4.1) + (B3), (A1.1) + (A4.2) + (B3);
    (A1.2) + (A2.1) + (B3), (A1.2) + (A2.2) + (B3), (A1.2) + (A3.1) + (B3), (A1.2) + (A3.2) + (B3), (A1.2) + (A4.1) + (B3), (A1.2) + (A4.2) + (B3);
    (A2.1) + (A2.2) + (B3), (A2.1) + (A3.1) + (B3), (A2.1) + (A3.2) + (B3), (A2.1) + (A4.1) + (B3), (A2.1) + (A4.2) + (B3);
    (A2.2) + (A3.1) + (B3), (A2.2) + (A3.2) + (B3), (A2.2) + (A4.1) + (B3), (A2.2) + (A4.2) + (B3);
    (A3.1) + (A3.2) + (B3), (A3.1) + (A4.1) + (B3), (A3.1) + (A4.2) + (B3); (A3.2) + (A4.1) + (B3), (A3.2) + (A4.2) + (B3), (A4.1) + (A4.2) + (B3).
  • Die Safener (Antidote) der Gruppe (B) reduzieren oder unterbinden phytotoxische Effekte, die beim Einsatz der herbiziden Wirkstoffe (A) in Nutzpflanzenkulturen auftreten können, ohne die Wirksamkeit dieser herbiziden Wirkstoffe gegen Schadpflanzen wesentlich zu beeinträchtigen. Hierdurch kann das Einsatzgebiet herkömmlicher Pflanzenschutzmittel ganz erheblich erweitert und z.B. auf Kulturen wie Weizen, Gerste, Mais, Reis und andere Kulturen ausgedehnt werden, in denen bisher ein Einsatz der Herbizide nicht möglich oder nur beschränkt, das heißt, in niedrigen Dosierungen mit wenig Breitenwirkung möglich war.
  • Die Sulfonylharnstoffe (A) und die Safener (B) der erfindungsgemäßen Sulfonylharnstoff-Safener-Kombinationen können zusammen (z.B. als fertige Formulierung oder als Tank-Mischung) oder in beliebiger Reihenfolge nacheinander ausgebracht werden. Das Gewichtsverhältnis Safener: Sulfonylharnstoff kann innerhalb weiter Grenzen variieren und liegt vorzugsweise im Bereich von 1:100 bis 100:1, insbesondere von 1:10 bis 10:1. Die jeweils optimalen Mengen an Sulfonylharnstoff und Safener sind vom Typ des verwendeten Sulfonylharnstoffs oder vom verwendeten Safener sowie von der Art des zu behandelnden Pflanzenbestandes abhängig und lassen sich von Fall zu Fall durch einfache, routinemäßige Vorversuche ermitteln.
  • Haupteinsatzgebiete für die Anwendung der erfindungsgemäßen herbizid wirksamen Mittel sind vor allem Getreidekulturen (z.B. Weizen, Roggen, Gerste, Hafer), Reis, Mais, Sorghum, Baumwolle und Sojabohne, vorzugsweise Getreide, Reis und Mais.
  • Die in dem erfindungsgemäßen herbizid wirksamen Mittel enthaltenen Safener können je nach ihren Eigenschaften zur Vorbehandlung des Saatgutes der Kulturpflanze (Beizung der Samen) verwendet werden oder vor der Saat in die Saatfurchen eingebracht oder zusammen mit einem Herbizid, insbesondere einem Sulfonylharnstoff (A), vor oder nach dem Auflaufen der Pflanzen angewendet werden. Vorauflaufbehandlung schließt sowohl die Behandlung der Anbaufläche vor der Aussaat als auch die Behandlung der angesäten, aber noch nicht bewachsenen Anbauflächen ein. Bevorzugt ist die gemeinsame Anwendung mit einem Herbizid. Hierzu können z.B. Tankmischungen oder Fertigformulierungen eingesetzt werden.
  • Die benötigten Aufwandmengen der Safener können je nach Indikation und verwendetem herbiziden Wirkstoff innerhalb weiter Grenzen schwanken und sind in der Regel im Bereich von 0,001 bis 5 kg, vorzugsweise 0,005 bis 0,5 kg Wirkstoff je Hektar.
  • Die erfindungsgemäßen herbiziden Mittel bzw. Sulfonylharnstoff-Safener-Kombination können gegebenenfalls als zusätzliche Komponenten noch enthalten:
    • (C) ein oder mehrere Lösungsmittel, bevorzugt organische Lösungsmittel,
    • (D) ein oder mehrere Sulfosuccinate,
    • (E) einen oder mehrere von (A) und (B) verschiedene agrochemische Wirkstoffe, und/oder
    • (F) üblichen Hilfs- und Zusatzstoff.
  • Als optional enthaltene organische Lösungsmittel (Komponente C) kommen z.B. in Frage:
    • 1, ( Kohlenwasserstoffe, die unsubstituiert oder substituiert sein können, z.B. 1a) aromatische Kohlenwasserstoffe, z.B. • ein- oder mehrfach alkyl-substituierte Benzole wie Toluol, Xylole, Mesitylen, Ethylbenzol, oder • ein- oder mehrfach alkyl-substituierte Naphthaline wie 1-Methylnaphthalin, 2-Methylnaphthalin oder Dimethylnaphtalin, oder • andere vom Benzol abgeleitete aromatische Kohlenwasserstoffe, wie Indan oder Tetralin® , oder • Gemische hieraus, 1b) aliphatische Kohlenwasserstoffe, z.B. • lineare oder verzweigte Aliphaten, z.B. der allgemeinen Formel CnH2n+z, wie Pentan, Hexan, Octan, 2-Methylbutan oder 2,2,4-Trimethylpentan, oder • cyclische, gegebenenfalls alkyl-substituierte Aliphaten, wie Cyclohexan oder Methylcyclopentan, oder • Gemische hieraus, wie Lösungsmittel der Exxsol®D-Reihe, Isopar®-Reihe oder Bayol®-Reihe z.B. Bayol®82 (ExxonMobil Chemicals) oder der Isane®IP-Reihe oder Hydroseal®G-Reihe (TotalFinaElf), 1c) Gemische von aromatischen und aliphatischen Kohlenwasserstoffen, wie Lösungsmittel der Solvesso®-Reihe z.B. Solvesso®100, Solvesso®150 oder Solvesso®200 (ExxonMobil Chemicals), der Solvarex®/Solvaro®-Reihe (TotalFinaElf) oder der Caromax®-Reihe z.B. Caromax®28 (Petrochem Carless), oder 1d) halogenierte Kohlenwasserstoffe wie halogenierte aromatische und aliphatische Kohlenwasserstoffe, wie Chlorbenzol oder Methylenchlorid, oder
    • 2) aprotische, polare Lösungsmittel, wie Ether, Ester von C1-C9-Alkansäuren, die mono-, di- oder polyfunktional sein können, wie deren Mono-, Di- oder Triester, z.B. mit C1-C18-Alkylalkoholen, Ketone mit geringer Tautomerietendenz, Phophorsäureester, Amide, Nitrile oder Sulfone, z.B. Diisobutyladipat, Rhodiasolv® RPDE (Rhodia), Cyclohexanon, Jeftsol®PC (Huntsman), γ- Butyrolacton, N-Methylpyrrolidon, Dimethylsulfoxid, Acetonitril, Tributylphosphatam oder Hostarex®PO-Reihe (Clariant), oder
    • 3) Fettsäureester, z.B. natürlichen Ursprungs, z.B. natürliche Öle wie tierische Öle oder Pflanzenöle, oder synthetischen Ursprungs, z.B. Edenor®-Reihe z.B. Edenor®MEPa oder Edenor®MESU oder Agnique®ME-Reihe oder Agnique®AE-Reihe (Cognis), Salim®ME-Reihe (Salim), Radia®-Reihe z.B. Radia®30167 (ICI), Prilube®-Reihe z.B. Prilube®1530 (Petrofina), Stepan®C-Reihe (Stepan) oder Witconol®23-Reihe (Witco). Die Fettsäureester sind bevorzugt Ester von C10-C22-, vorzugsweise C12-C20-Fettsäuren. Die C10-C22-Fettsäureester sind beispielsweise Ester ungesättigter oder gesättigter C10-C22-Fettsäuren, insbesondere mit gerader Kohlenstoffatomzahl, z.B. Erucasäure, Laurinsäure, Palmitinsäure und insbesondere C18-Fettsäuren wie Stearinsäure, Ölsäure, Linolsäure oder Linolensäure.
  • Beispiele für Fettsäureester wie C10-C22-Fettsäure-Ester sind Glycerin- und Glykolester von Fettsäuren wie C10-C22-Fettsäuren oder deren Umesterungsprodukte, z.B. Alkyl-Fettsäureester wie C1-C20-Alkyl-C10-C22-Fettsäure-Ester, wie sie z.B. durch Umesterung der vorgenannten Glycerin- oder Glykol-Fettsäureester wie C10-C22-Fettsäure-Ester mit C1-C20-Alkoholen (z.B. Methanol, Ethanol, Propanol oder Butanol) erhalten werden können. Die Umesterung kann nach bekannten Methoden erfolgen, wie sie z.B. beschrieben sind im Römpp Chemie Lexikon, 9. Auflage, Band 2, Seite 1343, Thieme Verlag Stuttgart.
  • Als Alkyl-Fettsäureester wie C1-C20-Alkyl-C10-C22-Fettsäure-Ester bevorzugt sind Methylester, Ethylester, Propylester, Butylester, 2-ethyl-hexylester und Dodecylester. Als Glykol- und Glycerin-Fettsäureester wie C10-C22-Fettsäure-Ester bevorzugt sind die einheitlichen oder gemischten Glykolester und Glycerinester von C10-C22-Fettsäuren, insbesondere solcher Fettsäuren mit gerader Anzahl an Kohlenstoffatomen, z.B. Erucasäure, Laurinsäure, Palmitinsäure und insbesondere C18-Fettsäuren wie Stearinsäure, Ölsäure, Linolsäure oder Linolensäure.
  • Tierische Öle sind allgemein bekannt und kommerziell erhältlich. Unter dem Begriff tierische Öle im Sinne der vorliegenden Erfindung werden z.B. Öle tierischen Ursprungs verstanden wie Waltranöl, Lebertranöl, Moschusöl oder Nerzöl.
  • Pflanzenöle sind allgemein bekannt und kommerziell erhältlich. Unter dem Begriff Pflanzenöle im Sinne der vorliegenden Erfindung werden z.B. Öle aus ölliefernden Pflanzenarten wie Sojaöl, Rapsöl, Maiskeimöl, Sonnenblumenöl, Baumwollsaatöl, Leinöl, Kokosöl, Palmöl, Distelöl, Walnussöl, Erdnussöl, Olivenöl oder Rhizinusöl, insbesondere Rapsöl verstanden, wobei unter den Pflanzenölen auch deren Umesterungsprodukte verstanden werden, z.B. Alkylester wie Rapsölmethylester oder Rapsölethylester.
  • Die Pflanzenöle sind bevorzugt Ester von C10-C22-, vorzugsweise C10-C20-Fettsäuren. Die C10-C22-Fettsäureester sind beispielsweise Ester ungesättigter oder gesättigter C10-C22-Fettsäuren, insbesondere mit gerader Kohlenstoffatomzahl, z.B. Erucasäure, Laurinsäure, Palmitinsäure und insbesondere C18-Fettsäuren wie Stearinsäure, Ölsäure, Linolsäure oder Linolensäure.
  • Beispiele für Pflanzenöle sind C10-C22-Fettsäure-Ester von Glycerin oder Glykol mit den C10-C22-Fettsäuren, oder C10-C20-Alkyl-C10-C22-Fettsäure-Ester, wie sie z.B. durch Umesterung der vorgenannten Glycerin- oder Glykol-C10-C22-Fettsäure-Ester mit C10-C20-Alkoholen (z.B. Methanol, Ethanol, Propanol oder Butanol) erhalten werden können. Die Umesterung kann nach bekannten Methoden erfolgen, wie sie z.B. beschrieben sind im Römpp Chemie Lexikon, 9. Auflage, Band 2, Seite 1343, Thieme Verlag Stuttgart.
  • Die Pflanzenöle können z.B. in Form kommerziell erhältlicher Pflanzenöle, insbesondere Rapsöle wie Rapsölmethylester, z.B. Phytorob®B (Novance, Frankreich), Edenor® MESU und Agnique®ME-Reihe (Cognis, Deutschland) Radia®-Reihe (ICI), Prilube®-Reihe (Petrofina) oder Biodiesel oder in Form kommerziell erhältlicher pflanzenölhaltiger Formulierungszusatzstoffe, insbesondere solcher auf Basis von Rapsölen wie Rapsölmethylester, z.B. Hasten® (Victorian Chemical Company, Australien, nachfolgend Hasten genannt, Hauptbestandteil: Rapsölethylester), Actirob®B (Novance, Frankreich, nachfolgend ActirobB genannt, Hauptbestandteil: Rapsölmethylester), Rako-Binol® (Bayer AG, Deutschland, nachfolgend Rako-Binol genannt, Hauptbestandteil: Rapsöl), Renol® (Stefes, Deutschland, nachfolgend Renol genannt, Pflanzenölbestandteil: Rapsölmethylester) oder Stefes Mero® (Stefes, Deutschland, nachfolgend Mero genannt, Hauptbestandteil: Rapsölmethylester) enthalten sein.
  • Beispiele für synthetische Fettsäureester sind z.B. solche die sich von Fettsäuren mit ungerader Kohlenstoffatomanzahl ableiten, wie C11-C21-Fettsäureester.
  • Bevorzugte organische Lösungsmittel sind aromatische Kohlenwasserstoffe, aliphatische Kohlenwasserstoffe und Fettsäureester wie pflanzliche Öle wie Triglyceride von Fettsäuren mit 10 bis 22 C-Atomen, die sowohl gesättigt als auch ungesättigt, linear oder verzweigt sein können und gegebenenfalls weitere funktionelle Gruppen tragen, wie Maiskeimöl, Rapsöl, Sonnenblumenkernöl, Baumwollsaatöl, Leinöl, Sojaöl, Kokosöl, Palmöl, Distelöl oder Rizinusöl, und deren Umesterungsprodukte wie Fettsäurealkylester, sowie Mischungen hieraus.
  • Die Lösungsmittel können allein oder im Gemisch enthalten sein. Das verwendete Lösungsmittel bzw. Lösungsmittelgemisch weist bevorzugt ein geringes Lösevermögen für das verwendete bzw. die verwendeten Sulfonylharnstoffe (Komponente A) auf.
  • Der Gesamtlösungsmittelanteil in den erfindungsgemäßen herbiziden Mitteln liegt im allgemeinen zwischen 0 und 95 Gew.%, bevorzugt im Bereich zwischen 20 und 80 Gew.%. Der Anteil an polaren Lösungsmitteln wie aprotischen, polaren liegt im allgemeinen unter 20 Gew.-%, bevorzugt im Bereich von 0 bis 10 Gew.%.
  • Die in den erfindungsgemäßen herbiziden Mitteln optional enthaltenen Sulfosuccinate (Komponente D) können z.B. Mono- oder Diester der Sulfobernsteinsäure sein, vorzugsweise solche der allgemeinen Formel (III) R1-(X1)n-O-CO-CH2-CH(SO3M)-CO-O-(X2)m-R2 (III)worin
    R1 H oder ein unsubstituierter oder substituierter C1-C30-Kohlenwasserstoffrest wie C1-C30-Alkyl oder C7-C30-Alkylaryl bedeutet,
    R2 H oder ein unsubstituierter oder substituierter C1-C30-Kohlenwasserstoffrest wie C1-C30-Alkyl oder C7-C30-Alkylaryl bedeutet, oder ein Kation ist, z.B. ein Metallkation wie ein Alkali- oder Erdalkalimetallkation, oder ein Ammoniumkation wie NH4, Alkyl-, Alkylaryl- oder Poly(arylalkyl)phenyl-ammoniumkation,
    X1, X2 unabhängig voneinander gleich oder verschieden eine Spacereinheit wie eine Polyethereinheit oder eine Polyestereinheit bedeuten,
    n, m unabhängig voneinander gleich oder verschieden Null oder 1 sind, vorzugsweise Null sind, und
    M ein Kation ist, z.B. ein Metallkation wie ein Alkali- oder Erdalkalimetallkation, oder ein Ammoniumkation wie NH4, Alkyl-, Alkylaryl- oder Poly(arylalkyl)phenyl-ammoniumkation.
  • Bevorzugt sind Sulfosuccinate der Formel (III), worin R1 und R2 unabhängig voneinander gleich oder verschieden lineare, verzweigte oder cyclische, gesättigte oder ungesättigte C1-C20- vorzugsweise C4-C18-Alkylreste sind, wie Methyl-, Ethyl-, Butyl-, Hexyl-, Cyclohexyl-, Octyl wie 2-Ethylhexyl-, Decyl-, Tridecyl- oder Octadecyl- Reste, oder R1 und R2 sind C1-C20-Alkylarylreste, wie Nonylphenyl, 2,4,6-Tri-sec-butylphenyl, 2,4,6-Tris-(1-phenylethyl)-phenyl, Alkylbenzyl oder ein Hydrozimtrest, X1 und X2 unabhängig voneinander gleich oder verschieden Polyethereinheiten sind, wie Polyethylenglykole -(C2H4O)p- oder Polypropylenglykole -(C3H6O)p- mit p=1 bis p=20, insbesondere p=1 bis p=12, oder Polyestereinheiten sind, wie Polyhydroxybuttersäure -(CH[CH3]-CH2-COO)q- oder Polymilchsäure -(CH[CH3]-COO)q- mit q=1 bis q=15, insbesondere q=1 bis q=8, n, m unabhängig voneinander gleich oder verschieden Null oder 1 sind, vorzugsweise Null sind, und M ein Kation ist, z.B. ein Metallkation, wie Alkali- oder Erdalkalimetallkation, oder ein Ammoniumkation, welches alkyl-substituiert sein kann.
  • Beispiele bevorzugt enthaltener Sulfosuccinate sind,
    • a1) ein- oder zweifach mit linearen, cyclischen oder verzweigten aliphatischen, cycloaliphatischen und/oder aromatischen Alkoholen verestertes Sulfosuccinat, beispielsweise mit 1 bis 22 C-Atomen im Alkylrest, vorzugsweise ein- oder zweifach mit Methanol, Ethanol, (Iso)propanol, (Iso)butanol, (Iso)pentanol, (Iso)hexanol, Cyclohexanol, (Iso)heptanol, (Iso)octanol (insbesondere: Ethylhexanol), (Iso)nonanol, (Iso)decanol, (Iso)undecanol, (Iso)dodecanol oder (Iso)tridecanol verestertes Mono- oder Dialkalisulfosuccinat, insbesondere Mono- oder Dinatriumsulfosuccinat,
    • a2) ein- oder zweifach mit (Poly) Alkylenoxidaddukten von Alkoholen verestertes Sulfosuccinat, beispielsweise mit 1 bis 22 C-Atomen im Alkylrest und 1 bis 200, vorzugsweise 2 bis 200 Alkylenoxideinheiten im (Poly) Alkylenoxidanteil, vorzugsweise ein- oder zweifach mit Dodecyl/Tetradecyl-Alkohol +2-5 mol Ethylenoxid oder mit i-Tridecyl+3mol Ethylenoxid verestertes Mono- oder Dialkalisulfosuccinat, insbesondere Mono- oder Dinatriumsulfosuccinat,
    • a3) das Dialkali, vorzugsweise das Dinatriumsalz von einfach mit Aminen oder aminoterminierten (Poly) Alkylenoxidaddukten von Alkoholen, Aminen, Fettsäuren, Estern oder Amiden umgesetztem und nachfolgend sulfoniertem Maleinsäureanhydrid, beispielsweise mit 1 bis 22 C-Atomen im Alkylrest und 1 bis 200, vorzugsweise 2 bis 200 Alkylenoxy-Einheiten im (Poly) Alkylenoxidteil, vorzugsweise das Dinatriumsalz von einfach mit Kokosfettamin umgesetztem und nachfolgend sulfoniertem Maleinsäureanhydrid,
    • a4) das Dialkali, vorzugsweise das Dinatriumsalz von einfach mit Amiden oder (Poly) Alkylenoxidaddukten von Amiden umgesetztem und nachfolgend sulfoniertem Maleinsäureanhydrid, beispielsweise mit 1 bis 22 C-Atomen im Alkylrest und 1 bis 200, vorzugsweise 2 bis 200 Alykylenoxy-Einheiten im (Poly) Alkylenoxidteil, vorzugsweise das Dinatriumsalz von einfach mit Oleylamid+2 mol Ethylenoxid umgesetztem und nachfolgend sulfoniertem Maleinsäureanhydrid und/oder
    • a5) das Tetraalkali, vorzugsweise das Tetranatriumsalz von N-(1,2-dicarboxyethyl-)-N-Octadecylsulfo-succinamat.
  • Beispiele kommerziell erhältlicher und im Rahmen der vorliegenden Erfindung bevorzugter Sulfosuccinate der Gruppen a1) bis a5) sind nachfolgend aufgeführt:
    • a1) Natrium-Dialkylsulfosuccinat, z.B. Natrium-Di(C4-C18)alkylsulfosuccinat wie Natrium-Diisooctylsulfosuccinat, vorzugsweise Natrium-Di(2-ethylhexyl)sulfosuccinat, kommerziell beispielsweise in Form der Aerosol®-Marken (Cytec), der Agrilan®- oder Lankropol®-Marken (Akzo Nobel), der Empimin®-Marken (Albright&Wilson), der Cropol®-Marken (Croda), der Lutensit®-Marken (BASF) der Triton®-Marken (Union Carbide), der Geropon®-Marken (Rhodia) oder der Imbirol®-, Madeol®- oder Polirol®-Marken (Cesalpinia) erhältlich,
    • a2) Natrium- Alkoholpolyethylenglykolethersulfosuccinat, kommerziell beispielsweise in Form von Geropon® ACR-Marken (Rhodia) erhältlich,
    • a3) Dinatrium-Alkoholpolyethylenglykolethersemisulfosuccinat, kommerziell beispielsweise in Form der Aerosol®-Marken (Cytec), der Marlinat®- oder Sermul®-Marken (Condea), der Empicol®-Marken (Albright&Wilson), der Secosol®-Marken (Stepan), der Geropon®-Marken (Rhodia), der Disponil®- oder Texapon®-Marken (Cognis) oder der Rolpon®-Marken (Cesalpinia) erhältlich,
    • a4) Dinatrium-N-Alkylsulfosuccinamat, kommerziell beispielsweise in Form der Aerosol®-Marken (Cytec), der Rewopol®- oder Rewoderm®-Marken (Rewo), der Empimin®-Marken (Albright&Wilson), der Geropon®-Marken (Rhodia) oder der Polirol®-Marken (Cesalpinia) erhältlich,
    • a5) Dinatrium-Fettsäureamidpolyethylenglykolethersemisulfosuccinat, kommerziell beispielsweise in Form der Elfanol®- oder Lankropol®-Marken (Akzo Nobel), der Rewoderm®-, Rewocid®- oder Rewopol®-Marken (Rewo), der Emcol®-Marken (Witco), der Standapol®-Marken (Cognis) oder der Rolpon®-Marken (Cesalpinia) erhältlich, und
    • a6) Tetranatrium-N-(1,2-dicarboxyethyl)-N-Octadecyl-sulfosuccinamat, kommerziell beispielsweise in Form von Aerosol 22®- (Cytec) erhältlich.
  • Kommerziell sind Sulfosuccinate zum Beispiel als Aerosol®- (Cytec), Agrilan®- oder Lankropol®- (Akzo Nobel), Empimin®- (Huntsman), Cropol®- (Croda), Lutensit®-(BASF), Triton®GR-Reihe (UnionCarbide), Imbirol®-/Madeol®-/Polirol®- (Cesalpinia); Geropon®AR-Reihe oder Geropon®SDS (Rhodia) erhältlich.
  • Bevorzugte Sulfosuccinate sind z.B. die Natrium-, Kalium- und Ammoniumsalze von Bis(alkyl)sulfosuccinaten, wobei die Alkylreste gleich oder verschieden 4 bis 16 Kohlenstoffatome enthalten, und bevorzugt Butyl-, Hexyl-, Octyl- wie 2-Ethylhexyl- oder Decyl-Reste sind, die linear oder verzweigt sein können.
  • Der Gesamtanteil des Sulfosuccinats bzw. der Sulfosuccinate in den erfindungsgemäßen herbiziden Mitteln liegt im allgemeinen zwischen 0 und 60 Gew.%, insbesondere im Bereich zwischen 0,5 und 30 Gew.%.
  • Als optional enthaltene von (A) und (B) verschiedene agrochemische Wirkstoffe (E) kommen für die erfindungsgemäßen herbiziden Mittel beispielsweise bekannte Wirkstoffe wie Herbizide, Insektizide oder Fungizide in Frage, wie sie in z.B. Weed Research 26, 441-445 (1986), oder "The Pesticide Manual", 12th edition, The British Crop Protection Council, 2000, und dort zitierter Literatur beschrieben sind, z.B. in Mischungsformulierungen oder als Tank-Mischpartner. Als literaturbekannte Herbizide, die in den erfindungsgemäßen herbiziden Mitteln enthalten sein können, sind z.B. folgende Wirkstoffe zu nennen Die Verbindungen sind entweder mit dem "common narre" nach der International Organization for Standardization (ISO) oder mit dem chemischen Namen, ggf. zusammen mit einer üblichen Codenummer bezeichnet und umfassen stets sämtliche Anwendungsformen wie Säuren, Salze, Ester und Isomere wie Stereoisomere und optische Isomere: acetochlor; acifluorfen; aclonifen; AKH 7088, d.h. [[[1-[5-[2-Chloro-4-(trifluoromethyl)-phenoxy]-2-nitrophenyl]-2-methoxyethylidene]-amino]-oxy]-essigsäure und -essigsäure-methylester; alachlor; alloxydim; ametryn; amidosulfuron; amitrol; AMS, d.h. Ammoniumsulfamat; anilofos; asulam; atrazin; azafenidine (DPX-R6447), azimsulfurone (DPX-A8947); aziprotryn; barban; BAS 516 N, d.h. 5-Fluor-2-phenyl-4H-3,1-benzoxazin-4-on; benazolin; benfluralin; benfuresate; bensulfuron-methyl; bensulide; bentazone; benzofluor; benzoylprop-ethyl; benzthiazuron; bialaphos; bifenox; bispyribac-natrium (KIH-2023), bromacil; bromobutide; bromofenoxim; bromoxynil, insbesondere bromoxynil-octanoat und bromoxynil-heptanoat; butachlor; butamifos; butenachlor; buthidazole; butralin; butroxydim (ICI-0500), butylate; cafenstrole (CH-900); carbetamide; cafentrazone; CDAA, d.h. 2-Chlor-N,N-di-2-propenylacetamid; CDEC, d.h. Diethyldithiocarbaminsäure-2-chlorallylester; chlomethoxyfen; chloramben; cloransulam-methyl (XDE-565), chlorazifop-butyl, chlorbromuron; chlorbufam; chlorfenac; chlorflurenol-methyl; chloridazon; chlorimuron ethyl; chlornitrofen; chlorotoluron; chloroxuron; chlorpropham; chlorthal-dimethyl; chlorthiamid; cinidon-ethyl, cinmethylin; cinosulfuron; clethodim; clodinafop und dessen Esterderivate (z.B. clodinafop-propargyl); clomazone; clomeprop; cloproxydim; clopyralid; cumyluron (JC 940); cyanazine; cycloate; cyclosulfamuron (AC 014); cycloxydim; cycluron; cyhalofop und dessen Esterderivate (z.B. Butylester, DEH-112); cyperquat; cyprazine; cyprazole; 2,4-D; 2,4-DB; dalapon; desmedipham; desmetryn; di-allate; dicamba; dichlobenil; dichlorprop; diclofop und dessen Ester wie diclofop-methyl; diclosulam (XDE-564), diethatyl; difenoxuron; difenzoquat; diflufenican; diflufenzopyr-natrium (SAN-835H), dimefuron; dimethachlor; dimethametryn; dimethenamid (SAN-582H); dimidazone, 5-(4,6-Dimethylpyrimidin-2-yl-carbamoylsulfamoyl)-1-(2-pyridyl)-pyrazol-4-carbonsäuremethylester (NC-330); triaziflam (IDH-1105), cinosulfon; dimethipin; dinitramine; dinoseb; dinoterb; diphenamid; dipropetryn; diquat; dithiopyr; diuron; DNOC; eglinazine-ethyl; EL 177, d.h. 5-Cyano-1-(1,1-dimethylethyl)-N-methyl-1H-pyrazole-4-carboxamid; endothal; indanofan (MK-243), EPTC; esprocarb; ethalfluralin; ethametsulfuron-methyl; ethidimuron; ethiozin; ethofumesate; F5231, d.h. N-[2-Chlor-4-fluor-5-[4-(3-fluorpropyl)-4,5-dihydro-5-oxo-1H-tetrazol-1-yl]-phenyl]-ethansulfonamid; ethoxyfen und dessen Ester (z.B. Ethylester, HN-252); ethoxysulfuron (aus EP 342569 ); etobenzanid (HW 52); 3-(4-Ethoxy-6-ethyl-1,3,5-triazin-2-yl)-1-(2,3-dihydro-1,1-dioxo-2-methylbenzo[b]thiophen-7-sulfonyl)harnstoff (EP-A 079 683); 3-(4-Ethyl-6-methoxy-1,3,5-triazin-2-yl)-1-(2,3-dihydro-1,1-dioxo-2-methylbenzo[b]thiophen-7-sulfonyl)harnstoff (EP-A 079 683); fenoprop; clomazone, fenoxaprop und fenoxaprop-P sowie deren Ester, z.B. fenoxaprop-P-ethyl und fenoxaprop-ethyl; butroxydim; fenuron; flamprop-methyl; flazasulfuron; flufenacet (BAY-FOE-5043), fluazifop und fluazifop-P und deren Ester, z.B. fluazifop-butyl und fluazifop-P-butyl, florasulam (DE-570); fluchloralin; flumetsulam; fluometuron; flumiclorac und dessen Ester (z.B. Pentylester, S-23031); flumioxazin (S-482); flumipropyn; flupoxam (KNW-739); fluorodifen; fluoroglycofen-ethyl; flupropacil (UBIC-4243); flupyrsulfuron-methyl natrium (DPX-KE459), fluridone; flurochloridone; fluroxypyr; flurtamone; fluthiacet-methyl (KIH-9201), fomesafen; fosamine; furyloxyfen; glufosinate; glyphosate; halosafen; halosulfuron und dessen Ester (z.B. Methylester, NC-319); haloxyfop und dessen Ester; haloxyfop-P (= R-haloxyfop) und dessen Ester; hexazinone; imazamethabenzmethyl; imazamox (AC-299263), imazapyr; imazaquin und Salze wie das Ammoniumsalz; imazapic; imazethapyr; imazosulfuron; iodosulfuron-methyl-natrium (Methyl-4-iod-2-[3-(4-methoxy-6-methyl-1,3,5-triazin-2-yl)ureidosulfonyl]-benzoat, Natriumsalz, WO 92/13845); ioxynil; isocarbamid; isopropalin; isoproturon; isouron; isoxaben; isoxapyrifop; karbutilate; lactofen; lenacil; linuron; MCPA; MCPB; mecoprop; mefenacet; mefluidid; metamitron; metazachlor; methabenzthiazuron; metam; methazole; methoxyphenone; methyldymron; metobenzuron, mesosulfuronmethyl (WO 95/10507); metobromuron; metolachlor; S-metolachlor, metosulam (XRD 511); metoxuron; metribuzin; maleic hydrazide; molinate; monalide; monocarbamide dihydrogensulfate; monolinuron; monuron; MT 128, d.h. 6-Chlor-N(3-chlor-2-propenyl)-5-methyl-N-phenyl-3-pyridazinamin; MT 5950, d.h. N-[3-Chlor-4- (1-methylethyl)-phenyl]-2-methylpentanamid; foramsulfuron (WO 95/01344); naproanilide; napropamide; naptalam; NC 310, d.h. 4-(2,4-dichlorbenzoyl)-1-methyl-5-benzyloxypyrazol; neburon; nicosulfuron; nipyraclofen; nitralin; nitrofen; nitrofluorfen; norflurazon; orbencarb; oryzalin; oxadiargyl (RP-020630); oxadiazon; oxaziclomefone (MY-100), oxyfluorfen; oxasulfuron (CGA-277476), paraquat; pebulate; pendimethalin; pentoxazone (KPP-314), perfluidone; phenisopham; phenmedipham; picloram; piperophos; pyributicarb; pirifenop-butyl; pretilachlor; primisulfuron-methyl; procyazine; prodiamine; profluralin; proglinazine-ethyl; prometon; prometryn; propachlor; propanil; propaquizafop und dessen Ester; propazine; propham; propisochlor; propoxycarbazone-natrium; propyzamide; prosulfalin; prosulfocarb; prosulfuron (CGA-152005); prynachlor; pyraflufen-ethyl (ET-751), chloridazon; pyrazosulfuron-ethyl; pyrazoxyfen; pyribenzoxim, pyridate; pyriminobac-methyl (KIH-6127), pyrithiobac (KIH-2031); pyroxofop und dessen Ester (z.B. Propargylester); quinclorac; quinmerac; quizalofop, quizalofop und quizalofop-P und deren Esterderivate z.B. quizalofop-ethyl; quizalofop-P-tefuryl und -ethyl; rimsulfuron (DPX-E 9636); S 275, d.h. 2-[4-Chlor-2-fluor-5-(2-propynyloxy)-phenyl]-4,5,6,7-tetrahydro-2H-indazol; secbumeton; sethoxydim; siduron; simazine; simetryn; SN 106279, d.h. 2-[[7-[2-Chlor-4-(trifluor-methyl)-phenoxy]-2-naphthalenyl]-oxy]-propansäure und -methylester; fluzasulfuron (FMC-97285, F-6285); sulfazuron; sulfometuron-methyl; glyphosate-trimesium (ICI-A0224); sulfosulfuron (MON-37500), TCA; tebutam (GCP-5544); tebuthiuron; tepraloxydim (BAS-620H), terbacil; terbucarb; terbuchlor; terbumeton; terbuthylazine; terbutryn; TFH 450, d.h. N,N-Diethyl-3-[(2-ethyl-6-methylphenyl)-sulfonyl]-1H-1,2,4-triazol-1-carboxamid; thenylchlor (NSK-850); thiazafluron; thiazopyr (Mon-13200); thidiazimin (SN-124085); thiobencarb; tiocarbazil; tralkoxydim; tri-allate; triasulfuron; triazofenamide; triclopyr; tridiphane; trietazine; trifluralin; triflusulfuron und Ester (z.B. Methylester, DPX-66037); trimeturon; tsitodef; vernolate; WL 110547, d.h. 5-Phenoxy-1-[3-(trifluormethyl)-phenyl]-1H-tetrazol; UBH-509; D-489; LS 82-556; KPP-300; KPP-421, MT-146, NC-324; butenachlor (KH-218); DPX-N8189; haloxyfopetotyl (DOWCO-535); DK-8910; flumioxazin (V-53482); PP-600; MBH-001, amicarbazone, aminopyralid, beflubutamid, benzobicyclon, benzofenap, benzfendizone, butafenacil, chlorfenprop, cloprop, daimuron, dichlorprop-P, dimepipeate, dimethenamid-P, fentrazamide, flamprop-M, fluazolate, flucarbazone, flucetosulfuron, foramsulfuron, indanofan, isoxachlortole, isoxaflutole, MCPA-thioethyl, mecoprop-P, mesosulfuron, mesotrione, metamifop, penoxsulam, pethoxamid, picolinafen, profluazol, profoxydim, propxycarbazone, pyraclonil, pyrazolynate, pyridafol, pyriftalid, sulcotrione, thidiazuron, trifloxysulfuron, tritosulfuron.
  • Die Mischungspartner E), die Sulfonylharnstoffe A) und die Safener B) können zusammen (als fertige Formulierung oder als Tankmischung) oder in beliebiger Reihenfolge nacheinander ausgebracht werden.
  • Bevorzugte Mischungspartner E) sind Bromoxynil (E1) in sämtlichen seiner Anwendungsformen einschließlich der Salze und Ester, z.B. Bromoxynil-octanoat (E1.1), Bromoxynil-heptanoat (E1.2), Bromoxynil-butyrat (E1.3), Bromoxynil-Natrium (E1.4) und Bromoxynil-Kalium (E1.5); 2,4-D (E2) in sämtlichen seiner Anwendungsformen einschließlich der Salze und Ester, z.B. 2,4-D-Butotyl (E2.1), 2,4-D-butyl (E2.2), 2,4-D-dimethylammonium (E2.3), 2,4-D-diethanolamin (E2.4), 2,4-D-2-ethylhexyl (E2.5), 2,4-D-isooctyl (E2.6), 2,4-D-isopropyl (E2.7), 2,4-D-Natrium (E2.8) und 2,4-D-triethanolamin (E2.9); Dicamba (E3) in sämtlichen seiner Anwendungsformen einschließlich der Salze und Ester, z.B. Dicamba-Natrium (E3.1), Dicamba-Kalium (E3.2) und Dicamba-dimethylammonium (E3.3); Fenoxaprop (E4) in sämtlichen seiner Anwendungsformen einschließlich der Ester, z.B. Fenoxaprop-ethyl (E4.1) und Fenoxaprop-P-ethyl (E4.2); Fluroxypyr (E5) in sämtlichen seiner Anwendungsformen einschließlich der Salze und Ester, z.B. Fluroxypyr-meptyl (E5.1) und Fluroxypyr-2-butoxy-1-methylethyl (E5.2); MCPA (E6) in sämtlichen seiner Anwendungsformen einschließlich der Salze und Ester, z.B. MCPA-Natrium (E6.1), MCPA-Kalium (E6.2), MCPA-2-ethylhexyl (E6.3), MCPA-butotyl (E6.4) und MCPA-dimethylammonium (E6.5); Iodosulfuron (E7) in sämtlichen seiner Anwendungsformen einschließlich der Salze und Ester, z.B. Iodosulfuronmethyl (E7.1) und Iodosulfuron-methyl-Natrium (E7.2); Mesosulfuron (E8) in sämtlichen seiner Anwendungsformen einschließlich der Salze und Ester, z.B. Mesosulfuron-methyl (E8.1) und Mesosulfuron-methyl-Natrium (E8.2); Propoxycarbazone (E9) in sämtlichen seiner Anwendungsformen einschließlich der Salze und Ester, z.B. Propoxycarbazone-Natrium (E9.1).
  • Bevorzugte erfindungsgemäße Kombinationen (A), (B), (E) sind beispielsweise:
    (E1) + (A1.1) + (B1), (E1) + (A1.1) + (B2), (E1) + (A1.1) + (B3), (E1) + (A2.1) + (B1), (E1) + (A2.1) + (B2), (E1) + (A2.1) + (B3), (E1) + (A3.1) + (B1), (E1) + (A3.1) + (B2), (E1) + (A3.1) + (B3), (E1) + (A4.1) + (B1), (E1) + (A4.1) + (B2), (E1) + (A4.1) + (B3), (E1) + (A1.2) + (B1), (E1) + (A1.2) + (B2), (E1) + (A1.2) + (B3), (E1) + (A2.2) + (B1), (E1) + (A2.2) + (B2), (E1) + (A2.2) + (B3), (E1) + (A3.2) + (B1), (E1) + (A3.2) + (B2), (E1) + (A3.2) + (B3), (E1) + (A4.2) + (B1), (E1) + (A4.2) + (B2), (E1) + (A4.2) + (B3), (E1) + (A1.1) + (A1.2) + (B1), (E1) + (A1.1) + (A2.1) + (B1), (E1) + (A1.1) + (A2.2) + (B1), (E1) + (A1.1) + (A3.1) + (B1), (E1) + (A1.1) + (A3.2) + (B1),(E1) + (A1.1) + (A4.1) + (B1), (E1) + (A1.1) + (A4.2) + (B1);
    (E1) + (A1.2) + (A2.1) + (B1),(E1) + (A1.2) + (A2.2) + (B1),(E1) + (A1.2) + (A3.1) + (B1), (E1) + (A1.2) + (A3.2) + (B1), (E1) + (A1.2) + (A4.1) + (B1), (E1) + (A1.2) + (A4.2) + (B1);
    (E1) + (A2.1) + (A2.2) + (B1),(E1) + (A2.1) + (A3.1) + (B1),(E1) + (A2.1) + (A3.2) + (B1), (E1) + (A2.1) + (A4.1) + (B1), (E1) + (A2.1) + (A4.2) + (B1);
    (E1) + (A2.2) + (A3.1) + (B1),(E1) + (A2.2) + (A3.2) + (B1),(E1) + (A2.2) + (A4.1) + (B1), (E1) + (A2.2) + (A4.2) + (B1);
    (E1) + (A3.1) + (A3.2) + (B1),(E1) + (A3.1) + (A4.1) + (B1),(E1) + (A3.1) + (A4.2) + (B1); (E1) + (A3.2) + (A4.1) + (B1), (E1) + (A3.2) + (A4.2) + (B1), (E1) + (A4.1) + (A4.2) + (B1);
    (E1) + (A1.1) + (A1.2) + (B2), (E1) + (A1.1) + (A2.1) + (B2), (E1) + (A1.1) + (A2.2) + (B2), (E1) + (A1.1) + (A3.1) + (B2), (E1) + (A1.1) + (A3.2) + (B2), (E1) + (A1.1) + (A4.1) + (B2), (E1) + (A1.1) + (A4.2) + (B2);
    (E1) + (A1.2) + (A2.1) + (B2), (E1) + (A1.2) + (A2.2) + (B2), (E1) + (A1.2) + (A3.1) + (B2), (E1) + (A1.2) + (A3.2) + (B2), (E1) + (A1.2) + (A4.1) + (B2), (E1) + (A1.2) + (A4.2) + (B2);
    (E1) + (A2.1) + (A2.2) + (B2),(E1) + (A2.1) + (A3.1) + (B2),(E1) + (A2.1) + (A3.2) + (B2), (E1) + (A2.1) + (A4.1) + (B2), (E1) + (A2.1) + (A4.2) + (B2);
    (E1) + (A2.2) + (A3.1) + (B2),(E1) + (A2.2) + (A3.2) + (B2),(E1) + (A2.2) + (A4.1) + (B2), (E1) + (A2.2) + (A4.2) + (B2);
    (E1) + (A3.1) + (A3.2) + (B2), (E1) + (A3.1) + (A4.1) + (B2),(E1) + (A3.1) + (A4.2) + (B2); (E1) + (A3.2) + (A4.1) + (B2), (E1) + (A3.2) + (A4.2) + (B2), (E1) + (A4.1) + (A4.2) + (B2);
    (E1) + (A1.1) + (A1.2) + (B3), (E1) + (A1.1) + (A2.1) + (B3), (E1) + (A1.1) + (A2.2) + (B3), (E1) + (A1.1) + (A3.1) + (B3), (E1) + (A1.1) + (A3.2) + (B3), (E1) + (A1.1) + (A4.1) + (B3), (E1) + (A1.1) + (A4.2) + (B3);
    (E1) + (A1.2) + (A2.1) + (B3), (E1) + (A1.2) + (A2.2) + (B3), (E1) + (A1.2) + (A3.1) + (B3), (E1) + (A1.2) + (A3.2) + (B3), (E1) + (A1.2) + (A4.1) + (B3), (E1) + (A1.2) + (A4.2) + (B3);
    (E1) + (A2.1) + (A2.2) + (B3), (E1) + (A2.1) + (A3.1) + (B3), (E1) + (A2.1) + (A3.2) + (B3), (E1) + (A2.1) + (A4.1) + (B3), (E1) + (A2.1) + (A4.2) + (B3);
    (E1) + (A2.2) + (A3.1) + (B3), (E1) + (A2.2) + (A3.2) + (B3), (E1) + (A2.2) + (A4.1) + (B3), (E1) + (A2.2) + (A4.2) + (B3);
    (E1) + (A3.1) + (A3.2) + (B3), (E1) + (A3.1) + (A4.1) + (B3), (E1) + (A3.1) + (A4.2) + (B3); (E1) + (A3.2) + (A4.1) + (B3), (E1) + (A3.2) + (A4.2) + (B3), (E1) + (A4.1) + (A4.2) + (B3);
    (E1.1) + (A1.1) + (B1), (E1.1) + (A1.1) + (B2), (E1.1) + (A1.1) + (B3), (E1.1) + (A2.1) + (B1), (E1.1) + (A2.1) + (B2), (E1.1) + (A2.1) + (B3), (E1.1) + (A3.1) + (B1), (E1.1) + (A3.1) + (B2), (E1.1) + (A3.1) + (B3), (E1.1) + (A4.1) + (B1), (E1.1) + (A4.1) + (B2), (E1.1) + (A4.1) + (B3), (E1.1) + (A1.2) + (B1), (E1.1) + (A1.2) + (B2), (E1.1) + (A1.2) + (B3), (E1.1) + (A2.2) + (B1), (E1.1) + (A2.2) + (B2), (E1.1) + (A2.2) + (B3), (E1.1) + (A3.2) + (B1), (E1.1) + (A3.2) + (B2), (E1.1) + (A3.2) + (B3), (E1.1) + (A4.2) + (B1), (E1.1) + (A4.2) + (B2), (E1.1) + (A4.2) + (B3),
    (E1.1) + (A1.1) + (A1.2) + (B1), (E1.1) + (A1.1) + (A2.1) + (B1), (E1.1) + (A1.1) + (A2.2) + (B1), (E1.1) + (A1.1) + (A3.1) + (B1), (E1.1) + (A1.1) + (A3.2) + (B1), (E1.1) + (A1.1) + (A4.1) + (B1), (E1.1) + (A1.1) + (A4.2) + (B1);
    (E1.1) + (A1.2) + (A2.1) + (B1), (E1.1) + (A1.2) + (A2.2) + (B1), (E1.1) + (A1.2) + (A3.1) + (B1), (E1.1) + (A1.2) + (A3.2) + (B1), (E1.1) + (A1.2) + (A4.1) + (B1), (E1.1) + (A1.2) + (A4.2) + (B1);
    (E1.1) + (A2.1) + (A2.2) + (B1), (E1.1) + (A2.1) + (A3.1) + (B1), (E1.1) + (A2.1) + (A3.2) + (B1), (E1.1) + (A2.1) + (A4.1) + (B1), (E1.1) + (A2.1) + (A4.2) + (B1);
    (E1.1) + (A2.2) + (A3.1) + (B1), (E1.1) + (A2.2) + (A3.2) + (B1), (E1.1) + (A2.2) + (A4.1) + (B1), (E1.1) + (A2.2) + (A4.2) + (B1);
    (E1.1) + (A3.1) + (A3.2) + (B1), (E1.1) + (A3.1) + (A4.1) + (B1), (E1.1) + (A3.1) + (A4.2) + (B1); (E1.1) + (A3.2) + (A4.1) + (B1), (E1.1) + (A3.2) + (A4.2) + (B1), (E1.1) + (A4.1) + (A4.2) + (B1);
    (E1.1) + (A1.1) + (A1.2) + (B2), (E1.1) + (A1.1) + (A2.1) + (B2), (E1.1) + (A1.1) + (A2.2) + (B2), (E1.1) + (A1.1) + (A3.1) + (B2), (E1.1) + (A1.1) + (A3.2) + (B2), (E1.1) + (A1.1) + (A4.1) + (B2), (E1.1) + (A1.1) + (A4.2) + (B2);
    (E1.1) + (A1.2) + (A2.1) + (B2), (E1.1) + (A1.2) + (A2.2) + (B2), (E1.1) + (A1.2) + (A3.1) + (B2), (E1.1) + (A1.2) + (A3.2) + (B2), (E1.1) + (A1.2) + (A4.1) + (B2), (E1.1) + (A1.2) + (A4.2) + (B2);
    (E1.1) + (A2.1) + (A2.2) + (B2), (E1.1) + (A2.1) + (A3.1) + (B2), (E1.1) + (A2.1) + (A3.2) + (B2), (E1.1) + (A2.1) + (A4.1) + (B2), (E1.1) + (A2.1) + (A4.2) + (B2);
    (E1.1) + (A2.2) + (A3.1) + (B2), (E1.1) + (A2.2) + (A3.2) + (B2), (E1.1) + (A2.2) + (A4.1) + (B2), (E1.1) + (A2.2) + (A4.2) + (B2);
    (E1.1) + (A3.1) + (A3.2) + (B2), (E1.1) + (A3.1) + (A4.1) + (B2), (E1.1) + (A3.1) + (A4.2) + (B2); (E1.1) + (A3.2) + (A4.1) + (B2), (E1.1) + (A3.2) + (A4.2) + (B2), (E1.1) + (A4.1) + (A4.2) + (B2);
    (E1.1) + (A1.1) + (A1.2) + (B3), (E1.1) + (A1.1) + (A2.1) + (B3), (E1.1) + (A1.1) + (A2.2) + (B3), (E1.1) + (A1.1) + (A3.1) + (B3), (E1.1) + (A1.1) + (A3.2) + (B3), (E1.1) + (A1.1) + (A4.1) + (B3), (E1.1) + (A1.1) + (A4.2) + (B3);
    (E1.1) + (A1.2) + (A2.1) + (B3), (E1.1) + (A1.2) + (A2.2) + (B3), (E1.1) + (A1.2) + (A3.1) + (B3), (E1.1) + (A1.2) + (A3.2) + (B3), (E1.1) + (A1.2) + (A4.1) + (B3), (E1.1) + (A1.2) + (A4.2) + (B3);
    (E1.1) + (A2.1) + (A2.2) + (B3), (E1.1) + (A2.1) + (A3.1) + (B3), (E1.1) + (A2.1) + (A3.2) + (B3), (E1.1) + (A2.1) + (A4.1) + (B3), (E1.1) + (A2.1) + (A4.2) + (B3);
    (E1.1) + (A2.2) + (A3.1) + (B3), (E1.1) + (A2.2) + (A3.2) + (B3), (E1.1) + (A2.2) + (A4.1) + (B3), (E1.1) + (A2.2) + (A4.2) + (B3);
    (E1.1) + (A3.1) + (A3.2) + (B3), (E1.1) + (A3.1) + (A4.1) + (B3), (E1.1) + (A3.1) + (A4.2) + (B3); (E1.1) + (A3.2) + (A4.1) + (B3), (E1.1) + (A3.2) + (A4.2) + (B3), (E1.1) + (A4.1) + (A4.2) + (B3);
    (E1.2) + (A1.1) + (B1), (E1.2) + (A1.1) + (B2), (E1.2) + (A1.1) + (B3), (E1.2) + (A2.1) + (B1), (E1.2) + (A2.1) + (B2), (E1.2) + (A2.1) + (B3), (E1.2) + (A3.1) + (B1), (E1.2) + (A3.1) + (B2), (E1.2) + (A3.1) + (B3), (E1.2) + (A4.1) + (B1), (E1.2) + (A4.1) + (B2), (E1.2) + (A4.1) + (B3), (E1.2) + (A1.2) + (B1), (E1.2) + (A1.2) + (B2), (E1.2) + (A1.2) + (B3), (E1.2) + (A2.2) + (B1), (E1.2) + (A2.2) + (B2), (E1.2) + (A2.2) + (B3), (E1.2) + (A3.2) + (B1), (E1.2) + (A3.2) + (B2), (E1.2) + (A3.2) + (B3), (E1.2) + (A4.2) + (B1), (E1.2) + (A4.2) + (B2), (E1.2) + (A4.2) + (B3),
    (E1.2) + (A1.1) + (A1.2) + (B1), (E1.2) + (A1.1) + (A2.1) + (B1), (E1.2) + (A1.1) + (A2.2) + (B1), (E1.2) + (A1.1) + (A3.1) + (B1), (E1.2) + (A1.1) + (A3.2) + (B1), (E1.2) + (A1.1) + (A4.1) + (B1), (E1.2) + (A1.1) + (A4.2) + (B1);
    (E1.2) + (A1.2) + (A2.1) + (B1), (E1.2) + (A1.2) + (A2.2) + (B1), (E1.2) + (A1.2) + (A3.1) + (B1), (E1.2) + (A1.2) + (A3.2) + (B1), (E1.2) + (A1.2) + (A4.1) + (B1), (E1.2) + (A1.2) + (A4.2) + (B1);
    (E1.2) + (A2.1) + (A2.2) + (B1), (E1.2) + (A2.1) + (A3.1) + (B1), (E1.2) + (A2.1) + (A3.2) + (B1), (E1.2) + (A2.1) + (A4.1) + (B1), (E1.2) + (A2.1) + (A4.2) + (B1);
    (E1.2) + (A2.2) + (A3.1) + (B1), (E1.2) + (A2.2) + (A3.2) + (B1), (E1.2) + (A2.2) + (A4.1) + (B1), (E1.2) + (A2.2) + (A4.2) + (B1);
    (E1.2) + (A3.1) + (A3.2) + (B1), (E1.2) + (A3.1) + (A4.1) + (B1), (E1.2) + (A3.1) + (A4.2) + (B1); (E1.2) + (A3.2) + (A4.1) + (B1), (E1.2) + (A3.2) + (A4.2) + (B1), (E1.2) + (A4.1) + (A4.2) + (B1);
    (E1.2) + (A1.1) + (A1.2) + (B2), (E1.2) + (A1.1) + (A2.1) + (B2), (E1.2) + (A1.1) + (A2.2) + (B2), (E1.2) + (A1.1) + (A3.1) + (B2), (E1.2) + (A1.1) + (A3.2) + (B2), (E1.2) + (A1.1) + (A4.1) + (B2), (E1.2) + (A1.1) + (A4.2) + (B2);
    (E1.2) + (A1.2) + (A2.1) + (B2), (E1.2) + (A1.2) + (A2.2) + (B2), (E1.2) + (A1.2) + (A3.1) + (B2), (E1.2) + (A1.2) + (A3.2) + (B2), (E1.2) + (A1.2) + (A4.1) + (B2), (E1.2) + (A1.2) + (A4.2) + (B2);
    (E1.2) + (A2.1) + (A2.2) + (B2), (E1.2) + (A2.1) + (A3.1) + (B2), (E1.2) + (A2.1) + (A3.2) + (B2), (E1.2) + (A2.1) + (A4.1) + (B2), (E1.2) + (A2.1) + (A4.2) + (B2);
    (E1.2) + (A2.2) + (A3.1) + (B2), (E1.2) + (A2.2) + (A3.2) + (B2), (E1.2) + (A2.2) + (A4.1) + (B2), (E1.2) + (A2.2) + (A4.2) + (B2);
    (E1.2) + (A3.1) + (A3.2) + (B2), (E1.2) + (A3.1) + (A4.1) + (B2), (E1.2) + (A3.1) + (A4.2) + (B2); (E1.2) + (A3.2) + (A4.1) + (B2), (E1.2) + (A3.2) + (A4.2) + (B2), (E1.2) + (A4.1) + (A4.2) + (B2);
    (E1.2) + (A1.1) + (A1.2) + (B3), (E1.2) + (A1.1) + (A2.1) + (B3), (E1.2) + (A1.1) + (A2.2) + (B3), (E1.2) + (A1.1) + (A3.1) + (B3), (E1.2) + (A1.1) + (A3.2) + (B3), (E1.2) + (A1.1) + (A4.1) + (B3), (E1.2) + (A1.1) + (A4.2) + (B3);
    (E1.2) + (A1.2) + (A2.1) + (B3), (E1.2) + (A1.2) + (A2.2) + (B3), (E1.2) + (A1.2) + (A3.1) + (B3), (E1.2) + (A1.2) + (A3.2) + (B3), (E1.2) + (A1.2) + (A4.1) + (B3), (E1.2) + (A1.2) + (A4.2) + (B3);
    (E1.2) + (A2.1) + (A2.2) + (B3), (E1.2) + (A2.1) + (A3.1) + (B3), (E1.2) + (A2.1) + (A3.2) + (B3), (E1.2) + (A2.1) + (A4.1) + (B3), (E1.2) + (A2.1) + (A4.2) + (B3);
    (E1.2) + (A2.2) + (A3.1) + (B3), (E1.2) + (A2.2) + (A3.2) + (B3), (E1.2) + (A2.2) + (A4.1) + (B3), (E1.2) + (A2.2) + (A4.2) + (B3);
    (E1.2) + (A3.1) + (A3.2) + (B3), (E1.2) + (A3.1) + (A4.1) + (B3), (E1.2) + (A3.1) + (A4.2) + (B3); (E1.2) + (A3.2) + (A4.1) + (B3), (E1.2) + (A3.2) + (A4.2) + (B3), (E1.2) + (A4.1) + (A4.2) + (B3);
    (E1.3) + (A1.1) + (B1), (E1.3) + (A1.1) + (B2), (E1.3) + (A1.1) + (B3), (E1.3) + (A2.1) + (B1), (E1.3) + (A2.1) + (B2), (E1.3) + (A2.1) + (B3), (E1.3) + (A3.1) + (B1), (E1.3) + (A3.1) + (B2), (E1.3) + (A3.1) + (B3), (E1.3) + (A4.1) + (B1), (E1.3) + (A4.1) + (B2), (E1.3) + (A4.1) + (B3), (E1.3) + (A1.2) + (B1), (E1.3) + (A1.2) + (B2), (E1.3) + (A1.2) + (B3), (E1.3) + (A2.2) + (B1), (E1.3) + (A2.2) + (B2), (E1.3) + (A2.2) + (B3), (E1.3) + (A3.2) + (B1), (E1.3) + (A3.2) + (B2), (E1.3) + (A3.2) + (B3), (E1.3) + (A4.2) + (B1), (E1.3) + (A4.2) + (B2), (E1.3) + (A4.2) + (B3),
    (E1.3) + (A1.1) + (A1.2) + (B1), (E1.3) + (A1.1) + (A2.1) + (B1), (E1.3) + (A1.1) + (A2.2) + (B1), (E1.3) + (A1.1) + (A3.1) + (B1), (E1.3) + (A1.1) + (A3.2) + (B1), (E1.3) + (A1.1) + (A4.1) + (B1), (E1.3) + (A1.1) + (A4.2) + (B1);
    (E1.3) + (A1.2) + (A2.1) + (B1), (E1.3) + (A1.2) + (A2.2) + (B1), (E1.3) + (A1.2) + (A3.1) + (B1), (E1.3) + (A1.2) + (A3.2) + (B1), (E1.3) + (A1.2) + (A4.1) + (B1), (E1.3) + (A1.2) + (A4.2) + (B1);
    (E1.3) + (A2.1) + (A2.2) + (B1), (E1.3) + (A2.1) + (A3.1) + (B1), (E1.3) + (A2.1) + (A3.2) + (B1), (E1.3) + (A2.1) + (A4.1) + (B1), (E1.3) + (A2.1) + (A4.2) + (B1); (E1.3) + (A2.2) + (A3.1) + (B1), (E1.3) + (A2.2) + (A3.2) + (B1), (E1.3) + (A2.2) + (A4.1) + (B1), (E1.3) + (A2.2) + (A4.2) + (B1);
    (E1.3) + (A3.1) + (A3.2) + (B1), (E1.3) + (A3.1) + (A4.1) + (B1), (E1.3) + (A3.1) + (A4.2) + (B1); (E1.3) + (A3.2) + (A4.1) + (B1), (E1.3) + (A3.2) + (A4.2) + (B1), (E1.3) + (A4.1) + (A4.2) + (B1);
    (E1.3) + (A1.1) + (A1.2) + (B2), (E1.3) + (A1.1) + (A2.1) + (B2), (E1.3) + (A1.1) + (A2.2) + (B2), (E1.3) + (A1.1) + (A3.1) + (B2), (E1.3) + (A1.1) + (A3.2) + (B2), (E1.3) + (A1.1) + (A4.1) + (B2), (E1.3) + (A1.1) + (A4.2) + (B2);
    (E1.3) + (A1.2) + (A2.1) + (B2), (E1.3) + (A1.2) + (A2.2) + (B2), (E1.3) + (A1.2) + (A3.1) + (B2), (E1.3) + (A1.2) + (A3.2) + (B2), (E1.3) + (A1.2) + (A4.1) + (B2), (E1.3) + (A1.2) + (A4.2) + (B2);
    (E1.3) + (A2.1) + (A2.2) + (B2), (E1.3) + (A2.1) + (A3.1) + (B2), (E1.3) + (A2.1) + (A3.2) + (B2), (E1.3) + (A2.1) + (A4.1) + (B2), (E1.3) + (A2.1) + (A4.2) + (B2);
    (E1.3) + (A2.2) + (A3.1) + (B2), (E1.3) + (A2.2) + (A3.2) + (B2), (E1.3) + (A2.2) + (A4.1) + (B2), (E1.3) + (A2.2) + (A4.2) + (B2);
    (E1.3) + (A3.1) + (A3.2) + (B2), (E1.3) + (A3.1) + (A4.1) + (B2), (E1.3) + (A3.1) + (A4.2) + (B2); (E1.3) + (A3.2) + (A4.1) + (B2), (E1.3) + (A3.2) + (A4.2) + (B2), (E1.3) + (A4.1) + (A4.2) + (B2);
    (E1.3) + (A1.1) + (A1.2) + (B3), (E1.3) + (A1.1) + (A2.1) + (B3), (E1.3) + (A1.1) + (A2.2) + (B3), (E1.3) + (A1.1) + (A3.1) + (B3), (E1.3) + (A1.1) + (A3.2) + (B3), (E1.3) + (A1.1) + (A4.1) + (B3), (E1.3) + (A1.1) + (A4.2) + (B3);
    (E1.3) + (A1.2) + (A2.1) + (B3), (E1.3) + (A1.2) + (A2.2) + (B3), (E1.3) + (A1.2) + (A3.1) + (B3), (E1.3) + (A1.2) + (A3.2) + (B3), (E1.3) + (A1.2) + (A4.1) + (B3), (E1.3) + (A1.2) + (A4.2) + (B3);
    (E1.3) + (A2.1) + (A2.2) + (B3), (E1.3) + (A2.1) + (A3.1) + (B3), (E1.3) + (A2.1) + (A3.2) + (B3), (E1.3) + (A2.1) + (A4.1) + (B3), (E1.3) + (A2.1) + (A4.2) + (B3);
    (E1.3) + (A2.2) + (A3.1) + (B3), (E1.3) + (A2.2) + (A3.2) + (B3), (E1.3) + (A2.2) + (A4.1) + (B3), (E1.3) + (A2.2) + (A4.2) + (B3);
    (E1.3) + (A3.1) + (A3.2) + (B3), (E1.3) + (A3.1) + (A4.1) + (B3), (E1.3) + (A3.1) + (A4.2) + (B3); (E1.3) + (A3.2) + (A4.1) + (B3), (E1.3) + (A3.2) + (A4.2) + (B3), (E1.3) + (A4.1) + (A4.2) + (B3);
    (E1.4) + (A1.1) + (B1), (E1.4) + (A1.1) + (B2), (E1.4) + (A1.1) + (B3), (E1.4) + (A2.1) + (B1), (E1.4) + (A2.1) + (B2), (E1.4) + (A2.1) + (B3), (E1.4) + (A3.1) + (B1), (E1.4) + (A3.1) + (B2), (E1.4) + (A3.1) + (B3), (E1.4) + (A4.1) + (B1), (E1.4) + (A4.1) + (B2), (E1.4) + (A4.1) + (B3), (E1.4) + (A1.2) + (B1), (E1.4) + (A1.2) + (B2), (E1.4) + (A1.2) + (B3), (E1.4) + (A2.2) + (B1), (E1.4) + (A2.2) + (B2), (E1.4) + (A2.2) + (B3), (E1.4) + (A3.2) + (B1), (E1.4) + (A3.2) + (B2), (E1.4) + (A3.2) + (B3), (E1.4) + (A4.2) + (B1), (E1.4) + (A4.2) + (B2), (E1.4) + (A4.2) + (B3),
    (E1.4) + (A1.1) + (A1.2) + (B1), (E1.4) + (A1.1) + (A2.1) + (B1), (E1.4) + (A1.1) + (A2.2) + (B1), (E1.4) + (A1.1) + (A3.1) + (B1), (E1.4) + (A1.1) + (A3.2) + (B1), (E1.4) + (A1.1) + (A4.1) + (B1), (E1.4) + (A1.1) + (A4.2) + (B1);
    (E1.4) + (A1.2) + (A2.1) + (B1), (E1.4) + (A1.2) + (A2.2) + (B1), (E1.4) + (A1.2) + (A3.1) + (B1), (E1.4) + (A1.2) + (A3.2) + (B1), (E1.4) + (A1.2) + (A4.1) + (B1), (E1.4) + (A1.2) + (A4.2) + (B1);
    (E1.4) + (A2.1) + (A2.2) + (B1), (E1.4) + (A2.1) + (A3.1) + (B1), (E1.4) + (A2.1) + (A3.2) + (B1), (E1.4) + (A2.1) + (A4.1) + (B1), (E1.4) + (A2.1) + (A4.2) + (B1);
    (E1.4) + (A2.2) + (A3.1) + (B1), (E1.4) + (A2.2) + (A3.2) + (B1), (E1.4) + (A2.2) + (A4.1) + (B1), (E1.4) + (A2.2) + (A4.2) + (B1);
    (E1.4) + (A3.1) + (A3.2) + (B1), (E1.4) + (A3.1) + (A4.1) + (B1), (E1.4) + (A3.1) + (A4.2) + (B1); (E1.4) + (A3.2) + (A4.1) + (B1), (E1.4) + (A3.2) + (A4.2) + (B1), (E1.4) + (A4.1) + (A4.2) + (B1);
    (E1.4) + (A1.1) + (A1.2) + (B2), (E1.4) + (A1.1) + (A2.1) + (B2), (E1.4) + (A1.1) + (A2.2) + (B2), (E1.4) + (A1.1) + (A3.1) + (B2), (E1.4) + (A1.1) + (A3.2) + (B2), (E1.4) + (A1.1) + (A4.1) + (B2), (E1.4) + (A1.1) + (A4.2) + (B2);
    (E1.4) + (A1.2) + (A2.1) + (B2), (E1.4) + (A1.2) + (A2.2) + (B2), (E1.4) + (A1.2) + (A3.1) + (B2), (E1.4) + (A1.2) + (A3.2) + (B2), (E1.4) + (A1.2) + (A4.1) + (B2), (E1.4) + (A1.2) + (A4.2) + (B2);
    (E1.4) + (A2.1) + (A2.2) + (B2), (E1.4) + (A2.1) + (A3.1) + (B2), (E1.4) + (A2.1) + (A3.2) + (B2), (E1.4) + (A2.1) + (A4.1) + (B2), (E1.4) + (A2.1) + (A4.2) + (B2);
    (E1.4) + (A2.2) + (A3.1) + (B2), (E1.4) + (A2.2) + (A3.2) + (B2), (E1.4) + (A2.2) + (A4.1) + (B2), (E1.4) + (A2.2) + (A4.2) + (B2);
    (E1.4) + (A3.1) + (A3.2) + (B2), (E1.4) + (A3.1) + (A4.1) + (B2), (E1.4) + (A3.1) + (A4.2) + (B2); (E1.4) + (A3.2) + (A4.1) + (B2), (E1.4) + (A3.2) + (A4.2) + (B2), (E1.4) + (A4.1) + (A4.2) + (B2);
    (E1.4) + (A1.1) + (A1.2) + (B3), (E1.4) + (A1.1) + (A2.1) + (B3), (E1.4) + (A1.1) + (A2.2) + (B3), (E1.4) + (A1.1) + (A3.1) + (B3), (E1.4) + (A1.1) + (A3.2) + (B3), (E1.4) + (A1.1) + (A4.1) + (B3), (E1.4) + (A1.1) + (A4.2) + (B3);
    (E1.4) + (A1.2) + (A2.1) + (B3), (E1.4) + (A1.2) + (A2.2) + (B3), (E1.4) + (A1.2) + (A3.1) + (B3), (E1.4) + (A1.2) + (A3.2) + (B3), (E1.4) + (A1.2) + (A4.1) + (B3), (E1.4) + (A1.2) + (A4.2) + (B3);
    (E1.4) + (A2.1) + (A2.2) + (B3), (E1.4) + (A2.1) + (A3.1) + (B3), (E1.4) + (A2.1) + (A3.2) + (B3), (E1.4) + (A2.1) + (A4.1) + (B3), (E1.4) + (A2.1) + (A4.2) + (B3);
    (E1.4) + (A2.2) + (A3.1) + (B3), (E1.4) + (A2.2) + (A3.2) + (B3), (E1.4) + (A2.2) + (A4.1) + (B3), (E1.4) + (A2.2) + (A4.2) + (B3);
    (E1.4) + (A3.1) + (A3.2) + (B3), (E1.4) + (A3.1) + (A4.1) + (B3), (E1.4) + (A3.1) + (A4.2) + (B3); (E1.4) + (A3.2) + (A4.1) + (B3), (E1.4) + (A3.2) + (A4.2) + (B3), (E1.4) + (A4.1) + (A4.2) + (B3);
    (E1.5) + (A1.1) + (B1), (E1.5) + (A1.1) + (B2), (E1.5) + (A1.1) + (B3), (E1.5) + (A2.1) + (B1), (E1.5) + (A2.1) + (B2), (E1.5) + (A2.1) + (B3), (E1.5) + (A3.1) + (B1), (E1.5) + (A3.1) + (B2), (E1.5) + (A3.1) + (B3), (E1.5) + (A4.1) + (B1), (E1.5) + (A4.1) + (B2), (E1.5) + (A4.1) + (B3), (E1.5) + (A1.2) + (B1), (E1.5) + (A1.2) + (B2), (E1.5) + (A1.2) + (B3), (E1.5) + (A2.2) + (B1), (E1.5) + (A2.2) + (B2), (E1.5) + (A2.2) + (B3), (E1.5) + (A3.2) + (B1), (E1.5) + (A3.2) + (B2), (E1.5) + (A3.2) + (B3), (E1.5) + (A4.2) + (B1), (E1.5) + (A4.2) + (B2), (E1.5) + (A4.2) + (B3),
    (E1.5) + (A1.1) + (A1.2) + (B1), (E1.5) + (A1.1) + (A2.1) + (B1), (E1.5) + (A1.1) + (A2.2) + (B1), (E1.5) + (A1.1) + (A3.1) + (B1), (E1.5) + (A1.1) + (A3.2) + (B1), (E1.5) + (A1.1) + (A4.1) + (B1), (E1.5) + (A1.1) + (A4.2) + (B1);
    (E1.5) + (A1.2) + (A2.1) + (B1), (E1.5) + (A1.2) + (A2.2) + (B1), (E1.5) + (A1.2) + (A3.1) + (B1), (E1.5) + (A1.2) + (A3.2) + (B1), (E1.5) + (A1.2) + (A4.1) + (B1), (E1.5) + (A1.2) + (A4.2) + (B1);
    (E1.5) + (A2.1) + (A2.2) + (B1), (E1.5) + (A2.1) + (A3.1) + (B1), (E1.5) + (A2.1) + (A3.2) + (B1), (E1.5) + (A2.1) + (A4.1) + (B1), (E1.5) + (A2.1) + (A4.2) + (B1);
    (E1.5) + (A2.2) + (A3.1) + (B1), (E1.5) + (A2.2) + (A3.2) + (B1), (E1.5) + (A2.2) + (A4.1) + (B1), (E1.5) + (A2.2) + (A4.2) + (B1);
    (E1.5) + (A3.1) + (A3.2) + (B1), (E1.5) + (A3.1) + (A4.1) + (B1), (E1.5) + (A3.1) + (A4.2) + (B1); (E1.5) + (A3.2) + (A4.1) + (B1), (E1.5) + (A3.2) + (A4.2) + (B1), (E1.5) + (A4.1) + (A4.2) + (B1);
    (E1.5) + (A1.1) + (A1.2) + (B2), (E1.5) + (A1.1) + (A2.1) + (B2), (E1.5) + (A1.1) + (A2.2) + (B2), (E1.5) + (A1.1) + (A3.1) + (B2), (E1.5) + (A1.1) + (A3.2) + (B2), (E1.5) + (A1.1) + (A4.1) + (B2), (E1.5) + (A1.1) + (A4.2) + (B2);
    (E1.5) + (A1.2) + (A2.1) + (B2), (E1.5) + (A1.2) + (A2.2) + (B2), (E1.5) + (A1.2) + (A3.1) + (B2), (E1.5) + (A1.2) + (A3.2) + (B2), (E1.5) + (A1.2) + (A4.1) + (B2), (E1.5) + (A1.2) + (A4.2) + (B2);
    (E1.5) + (A2.1) + (A2.2) + (B2), (E1.5) + (A2.1) + (A3.1) + (B2), (E1.5) + (A2.1) + (A3.2) + (B2), (E1.5) + (A2.1) + (A4.1) + (B2), (E1.5) + (A2.1) + (A4.2) + (B2);
    (E1.5) + (A2.2) + (A3.1) + (B2), (E1.5) + (A2.2) + (A3.2) + (B2), (E1.5) + (A2.2) + (A4.1) + (B2), (E1.5) + (A2.2) + (A4.2) + (B2);
    (E1.5) + (A3.1) + (A3.2) + (B2), (E1.5) + (A3.1) + (A4.1) + (B2), (E1.5) + (A3.1) + (A4.2) + (B2); (E1.5) + (A3.2) + (A4.1) + (B2), (E1.5) + (A3.2) + (A4.2) + (B2), (E1.5) + (A4.1) + (A4.2) + (B2);
    (E1.5) + (A1.1) + (A1.2) + (B3), (E1.5) + (A1.1) + (A2.1) + (B3), (E1.5) + (A1.1) + (A2.2) + (B3), (E1.5) + (A1.1) + (A3.1) + (B3), (E1.5) + (A1.1) + (A3.2) + (B3), (E1.5) + (A1.1) + (A4.1) + (B3), (E1.5) + (A1.1) + (A4.2) + (B3);
    (E1.5) + (A1.2) + (A2.1) + (B3), (E1.5) + (A1.2) + (A2.2) + (B3), (E1.5) + (A1.2) + (A3.1) + (B3), (E1.5) + (A1.2) + (A3.2) + (B3), (E1.5) + (A1.2) + (A4.1) + (B3), (E1.5) + (A1.2) + (A4.2) + (B3);
    (E1.5) + (A2.1) + (A2.2) + (B3), (E1.5) + (A2.1) + (A3.1) + (B3), (E1.5) + (A2.1) + (A3.2) + (B3), (E1.5) + (A2.1) + (A4.1) + (B3), (E1.5) + (A2.1) + (A4.2) + (B3);
    (E1.5) + (A2.2) + (A3.1) + (B3), (E1.5) + (A2.2) + (A3.2) + (B3), (E1.5) + (A2.2) + (A4.1) + (B3), (E1.5) + (A2.2) + (A4.2) + (B3);
    (E1.5) + (A3.1) + (A3.2) + (B3), (E1.5) + (A3.1) + (A4.1) + (B3), (E1.5) + (A3.1) + (A4.2) + (B3); (E1.5) + (A3.2) + (A4.1) + (B3), (E1.5) + (A3.2) + (A4.2) + (B3), (E1.5) + (A4.1) + (A4.2) + (B3);
    (E2) + (A1.1) + (B1), (E2) + (A1.1) + (B2), (E2) + (A1.1) + (B3), (E2) + (A2.1) + (B1), (E2) + (A2.1) + (B2), (E2) + (A2.1) + (B3), (E2) + (A3.1) + (B1), (E2) + (A3.1) + (B2), (E2) + (A3.1) + (B3), (E2) + (A4.1) + (B1), (E2) + (A4.1) + (B2), (E2) + (A4.1) + (B3), (E2) + (A1.2) + (B1), (E2) + (A1.2) + (B2), (E2) + (A1.2) + (B3), (E2) + (A2.2) + (B1), (E2) + (A2.2) + (B2), (E2) + (A2.2) + (B3), (E2) + (A3.2) + (B1), (E2) + (A3.2) + (B2), (E2) + (A3.2) + (B3), (E2) + (A4.2) + (B1), (E2) + (A4.2) + (B2), (E2) + (A4.2) + (B3), (E2) + (A1.1) + (A1.2) + (B1), (E2) + (A1.1) + (A2.1) + (B1), (E2) + (A1.1) + (A2.2) + (B1), (E2) + (A1.1) + (A3.1) + (B1), (E2) + (A1.1) + (A3.2) + (B1), (E2) + (A1.1) + (A4.1) + (B1), (E2) + (A1.1) + (A4.2) + (B1);
    (E2) + (A1.2) + (A2.1) + (B1), (E2) + (A1.2) + (A2.2) + (B1), (E2) + (A1.2) + (A3.1) + (B1), (E2) + (A1.2) + (A3.2) + (B1), (E2) + (A1.2) + (A4.1) + (B1), (E2) + (A1.2) + (A4.2) + (B1);
    (E2) + (A2.1) + (A2.2) + (B1), (E2) + (A2.1) + (A3.1) + (B1), (E2) + (A2.1) + (A3.2) + (B1), (E2) + (A2.1) + (A4.1) + (B1), (E2) + (A2.1) + (A4.2) + (B1);
    (E2) + (A2.2) + (A3.1) + (B1), (E2) + (A2.2) + (A3.2) + (B1), (E2) + (A2.2) + (A4.1) + (B1), (E2) + (A2.2) + (A4.2) + (B1);
    (E2) + (A3.1) + (A3.2) + (B1), (E2) + (A3.1) + (A4.1) + (B1), (E2) + (A3.1) + (A4.2) + (B1); (E2) + (A3.2) + (A4.1) + (B1), (E2) + (A3.2) + (A4.2) + (B1), (E2) + (A4.1) + (A4.2) + (B1);
    (E2) + (A1.1) + (A1.2) + (B2), (E2) + (A1.1) + (A2.1) + (B2), (E2) + (A1.1) + (A2.2) + (B2), (E2) + (A1.1) + (A3.1) + (B2), (E2) + (A1.1) + (A3.2) + (B2), (E2) + (A1.1) + (A4.1) + (B2), (E2) + (A1.1) + (A4.2) + (B2);
    (E2) + (A1.2) + (A2.1) + (B2), (E2) + (A1.2) + (A2.2) + (B2), (E2) + (A1.2) + (A3.1) + (B2), (E2) + (A1.2) + (A3.2) + (B2), (E2) + (A1.2) + (A4.1) + (B2), (E2) + (A1.2) + (A4.2) + (B2);
    (E2) + (A2.1) + (A2.2) + (B2), (E2) + (A2.1) + (A3.1) + (B2), (E2) + (A2.1) + (A3.2) + (B2), (E2) + (A2.1) + (A4.1) + (B2), (E2) + (A2.1) + (A4.2) + (B2);
    (E2) + (A2.2) + (A3.1) + (B2), (E2) + (A2.2) + (A3.2) + (B2), (E2) + (A2.2) + (A4.1) + (B2), (E2) + (A2.2) + (A4.2) + (B2);
    (E2) + (A3.1) + (A3.2) + (B2), (E2) + (A3.1) + (A4.1) + (B2), (E2) + (A3.1) + (A4.2) + (B2); (E2) + (A3.2) + (A4.1) + (B2), (E2) + (A3.2) + (A4.2) + (B2), (E2) + (A4.1) + (A4.2) + (B2);
    (E2) + (A1.1) + (A1.2) + (B3), (E2) + (A1.1) + (A2.1) + (B3), (E2) + (A1.1) + (A2.2) + (B3), (E2) + (A1.1) + (A3.1) + (B3), (E2) + (A1.1) + (A3.2) + (B3), (E2) + (A1.1) + (A4.1) + (B3), (E2) + (A1.1) + (A4.2) + (B3);
    (E2) + (A1.2) + (A2.1) + (B3), (E2) + (A1.2) + (A2.2) + (B3), (E2) + (A1.2) + (A3.1) + (B3), (E2) + (A1.2) + (A3.2) + (B3), (E2) + (A1.2) + (A4.1) + (B3), (E2) + (A1.2) + (A4.2) + (B3);
    (E2) + (A2.1) + (A2.2) + (B3), (E2) + (A2.1) + (A3.1) + (B3), (E2) + (A2.1) + (A3.2) + (B3), (E2) + (A2.1) + (A4.1) + (B3), (E2) + (A2.1) + (A4.2) + (B3);
    (E2) + (A2.2) + (A3.1) + (B3), (E2) + (A2.2) + (A3.2) + (B3), (E2) + (A2.2) + (A4.1) + (B3), (E2) + (A2.2) + (A4.2) + (B3);
    (E2) + (A3.1) + (A3.2) + (B3), (E2) + (A3.1) + (A4.1) + (B3), (E2) + (A3.1) + (A4.2) + (B3); (E2) + (A3.2) + (A4.1) + (B3), (E2) + (A3.2) + (A4.2) + (B3), (E2) + (A4.1) + (A4.2) + (B3);
    (E2.1) + (A1.1) + (B1), (E2.1) + (A1.1) + (B2), (E2.1) + (A1.1) + (B3), (E2.1) + (A2.1) + (B1), (E2.1) + (A2.1) + (B2), (E2.1) + (A2.1) + (B3), (E2.1) + (A3.1) + (B1), (E2.1) + (A3.1) + (B2), (E2.1) + (A3.1) + (B3), (E2.1) + (A4.1) + (B1), (E2.1) + (A4.1) + (B2), (E2.1) + (A4.1) + (B3), (E2.1) + (A1.2) + (B1), (E2.1) + (A1.2) + (B2), (E2.1) + (A1.2) + (B3), (E2.1) + (A2.2) + (B1), (E2.1) + (A2.2) + (B2), (E2.1) + (A2.2) + (B3), (E2.1) + (A3.2) + (B1), (E2.1) + (A3.2) + (B2), (E2.1) + (A3.2) + (B3), (E2.1) + (A4.2) + (B1), (E2.1) + (A4.2) + (B2), (E2.1) + (A4.2) + (B3),
    (E2.1) + (A1.1) + (A1.2) + (B1), (E2.1) + (A1.1) + (A2.1) + (B1), (E2.1) + (A1.1) + (A2.2) + (B1), (E2.1) + (A1.1) + (A3.1) + (B1), (E2.1) + (A1.1) + (A3.2) + (B1), (E2.1) + (A1.1) + (A4.1) + (B1), (E2.1) + (A1.1) + (A4.2) + (B1);
    (E2.1) + (A1.2) + (A2.1) + (B1), (E2.1) + (A1.2) + (A2.2) + (B1), (E2.1) + (A1.2) + (A3.1) + (B1), (E2.1) + (A1.2) + (A3.2) + (B1), (E2.1) + (A1.2) + (A4.1) + (B1), (E2.1) + (A1.2) + (A4.2) + (B1);
    (E2.1) + (A2.1) + (A2.2) + (B1), (E2.1) + (A2.1) + (A3.1) + (B1), (E2.1) + (A2.1) + (A3.2) + (B1), (E2.1) + (A2.1) + (A4.1) + (B1), (E2.1) + (A2.1) + (A4.2) + (B1);
    (E2.1) + (A2.2) + (A3.1) + (B1), (E2.1) + (A2.2) + (A3.2) + (B1), (E2.1) + (A2.2) + (A4.1) + (B1), (E2.1) + (A2.2) + (A4.2) + (B1);
    (E2.1) + (A3.1) + (A3.2) + (B1), (E2.1) + (A3.1) + (A4.1) + (B1), (E2.1) + (A3.1) + (A4.2) + (B1); (E2.1) + (A3.2) + (A4.1) + (B1), (E2.1) + (A3.2) + (A4.2) + (B1), (E2.1) + (A4.1) + (A4.2) + (B1);
    (E2.1) + (A1.1) + (A1.2) + (B2), (E2.1) + (A1.1) + (A2.1) + (B2), (E2.1) + (A1.1) + (A2.2) + (B2), (E2.1) + (A1.1) + (A3.1) + (B2), (E2.1) + (A1.1) + (A3.2) + (B2), (E2.1) + (A1.1) + (A4.1) + (B2), (E2.1) + (A1.1) + (A4.2) + (B2);
    (E2.1) + (A1.2) + (A2.1) + (B2), (E2.1) + (A1.2) + (A2.2) + (B2), (E2.1) + (A1.2) + (A3.1) + (B2), (E2.1) + (A1.2) + (A3.2) + (B2), (E2.1) + (A1.2) + (A4.1) + (B2), (E2.1) + (A1.2) + (A4.2) + (B2);
    (E2.1) + (A2.1) + (A2.2) + (B2), (E2.1) + (A2.1) + (A3.1) + (B2), (E2.1) + (A2.1) + (A3.2) + (B2), (E2.1) + (A2.1) + (A4.1) + (B2), (E2.1) + (A2.1) + (A4.2) + (B2);
    (E2.1) + (A2.2) + (A3.1) + (B2), (E2.1) + (A2.2) + (A3.2) + (B2), (E2.1) + (A2.2) + (A4.1) + (B2), (E2.1) + (A2.2) + (A4.2) + (B2);
    (E2.1) + (A3.1) + (A3.2) + (B2), (E2.1) + (A3.1) + (A4.1) + (B2), (E2.1) + (A3.1) + (A4.2) + (B2); (E2.1) + (A3.2) + (A4.1) + (B2), (E2.1) + (A3.2) + (A4.2) + (B2), (E2.1) + (A4.1) + (A4.2) + (B2);
    (E2.1) + (A1.1) + (A1.2) + (B3), (E2.1) + (A1.1) + (A2.1) + (B3), (E2.1) + (A1.1) + (A2.2) + (B3), (E2.1) + (A1.1) + (A3.1) + (B3), (E2.1) + (A1.1) + (A3.2) + (B3), (E2.1) + (A1.1) + (A4.1) + (B3), (E2.1) + (A1.1) + (A4.2) + (B3);
    (E2.1) + (A1.2) + (A2.1) + (B3), (E2.1) + (A1.2) + (A2.2) + (B3), (E2.1) + (A1.2) + (A3.1) + (B3), (E2.1) + (A1.2) + (A3.2) + (B3), (E2.1) + (A1.2) + (A4.1) + (B3), (E2.1) + (A1.2) + (A4.2) + (B3);
    (E2.1) + (A2.1) + (A2.2) + (B3), (E2.1) + (A2.1) + (A3.1) + (B3), (E2.1) + (A2.1) + (A3.2) + (B3), (E2.1) + (A2.1) + (A4.1) + (B3), (E2.1) + (A2.1) + (A4.2) + (B3);
    (E2.1) + (A2.2) + (A3.1) + (B3), (E2.1) + (A2.2) + (A3.2) + (B3), (E2.1) + (A2.2) + (A4.1) + (B3), (E2.1) + (A2.2) + (A4.2) + (B3);
    (E2.1) + (A3.1) + (A3.2) + (B3), (E2.1) + (A3.1) + (A4.1) + (B3), (E2.1) + (A3.1) + (A4.2) + (B3); (E2.1) + (A3.2) + (A4.1) + (B3), (E2.1) + (A3.2) + (A4.2) + (B3), (E2.1) + (A4.1) + (A4.2) + (B3);
    (E2.2) + (A1.1) + (B1), (E2.2) + (A1.1) + (B2), (E2.2) + (A1.1) + (B3), (E2.2) + (A2.1) + (B1), (E2.2) + (A2.1) + (B2), (E2.2) + (A2.1) + (B3), (E2.2) + (A3.1) + (B1), (E2.2) + (A3.1) + (B2), (E2.2) + (A3.1) + (B3), (E2.2) + (A4.1) + (B1), (E2.2) + (A4.1) + (B2), (E2.2) + (A4.1) + (B3), (E2.2) + (A1.2) + (B1), (E2.2) + (A1.2) + (B2), (E2.2) + (A1.2) + (B3), (E2.2) + (A2.2) + (B1), (E2.2) + (A2.2) + (B2), (E2.2) + (A2.2) + (B3), (E2.2) + (A3.2) + (B1), (E2.2) + (A3.2) + (B2), (E2.2) + (A3.2) + (B3), (E2.2) + (A4.2) + (B1), (E2.2) + (A4.2) + (B2), (E2.2) + (A4.2) + (B3),
    (E2.2) + (A1.1) + (A1.2) + (B1), (E2.2) + (A1.1) + (A2.1) + (B1), (E2.2) + (A1.1) + (A2.2) + (B1), (E2.2) + (A1.1) + (A3.1) + (B1), (E2.2) + (A1.1) + (A3.2) + (B1), (E2.2) + (A1.1) + (A4.1) + (B1), (E2.2) + (A1.1) + (A4.2) + (B1);
    (E2.2) + (A1.2) + (A2.1) + (B1), (E2.2) + (A1.2) + (A2.2) + (B1), (E2.2) + (A1.2) + (A3.1) + (B1), (E2.2) + (A1.2) + (A3.2) + (B1), (E2.2) + (A1.2) + (A4.1) + (B1), (E2.2) + (A1.2) + (A4.2) + (B1);
    (E2.2) + (A2.1) + (A2.2) + (B1), (E2.2) + (A2.1) + (A3.1) + (B1), (E2.2) + (A2.1) + (A3.2) + (B1), (E2.2) + (A2.1) + (A4.1) + (B1), (E2.2) + (A2.1) + (A4.2) + (B1);
    (E2.2) + (A2.2) + (A3.1) + (B1), (E2.2) + (A2.2) + (A3.2) + (B1), (E2.2) + (A2.2) + (A4.1) + (B1), (E2.2) + (A2.2) + (A4.2) + (B1);
    (E2.2) + (A3.1) + (A3.2) + (B1), (E2.2) + (A3.1) + (A4.1) + (B1), (E2.2) + (A3.1) + (A4.2) + (B1); (E2.2) + (A3.2) + (A4.1) + (B1), (E2.2) + (A3.2) + (A4.2) + (B1), (E2.2) + (A4.1) + (A4.2) + (B1);
    (E2.2) + (A1.1) + (A1.2) + (B2), (E2.2) + (A1.1) + (A2.1) + (B2), (E2.2) + (A1.1) + (A2.2) + (B2), (E2.2) + (A1.1) + (A3.1) + (B2), (E2.2) + (A1.1) + (A3.2) + (B2), (E2.2) + (A1.1) + (A4.1) + (B2), (E2.2) + (A1.1) + (A4.2) + (B2);
    (E2.2) + (A1.2) + (A2.1) + (B2), (E2.2) + (A1.2) + (A2.2) + (B2), (E2.2) + (A1.2) + (A3.1) + (B2), (E2.2) + (A1.2) + (A3.2) + (B2), (E2.2) + (A1.2) + (A4.1) + (B2), (E2.2) + (A1.2) + (A4.2) + (B2);
    (E2.2) + (A2.1) + (A2.2) + (B2), (E2.2) + (A2.1) + (A3.1) + (B2), (E2.2) + (A2.1) + (A3.2) + (B2), (E2.2) + (A2.1) + (A4.1) + (B2), (E2.2) + (A2.1) + (A4.2) + (B2);
    (E2.2) + (A2.2) + (A3.1) + (B2), (E2.2) + (A2.2) + (A3.2) + (B2), (E2.2) + (A2.2) + (A4.1) + (B2), (E2.2) + (A2.2) + (A4.2) + (B2);
    (E2.2) + (A3.1) + (A3.2) + (B2), (E2.2) + (A3.1) + (A4.1) + (B2), (E2.2) + (A3.1) + (A4.2) + (B2); (E2.2) + (A3.2) + (A4.1) + (B2), (E2.2) + (A3.2) + (A4.2) + (B2), (E2.2) + (A4.1) + (A4.2) + (B2);
    (E2.2) + (A1.1) + (A1.2) + (B3), (E2.2) + (A1.1) + (A2.1) + (B3), (E2.2) + (A1.1) + (A2.2) + (B3), (E2.2) + (A1.1) + (A3.1) + (B3), (E2.2) + (A1.1) + (A3.2) + (B3), (E2.2) + (A1.1) + (A4.1) + (B3), (E2.2) + (A1.1) + (A4.2) + (B3);
    (E2.2) + (A1.2) + (A2.1) + (B3), (E2.2) + (A1.2) + (A2.2) + (B3), (E2.2) + (A1.2) + (A3.1) + (B3), (E2.2) + (A1.2) + (A3.2) + (B3), (E2.2) + (A1.2) + (A4.1) + (B3), (E2.2) + (A1.2) + (A4.2) + (B3);
    (E2.2) + (A2.1) + (A2.2) + (B3), (E2.2) + (A2.1) + (A3.1) + (B3), (E2.2) + (A2.1) + (A3.2) + (B3), (E2.2) + (A2.1) + (A4.1) + (B3), (E2.2) + (A2.1) + (A4.2) + (B3);
    (E2.2) + (A2.2) + (A3.1) + (B3), (E2.2) + (A2.2) + (A3.2) + (B3), (E2.2) + (A2.2) + (A4.1) + (B3), (E2.2) + (A2.2) + (A4.2) + (B3);
    (E2.2) + (A3.1) + (A3.2) + (B3), (E2.2) + (A3.1) + (A4.1) + (B3), (E2.2) + (A3.1) + (A4.2) + (B3); (E2.2) + (A3.2) + (A4.1) + (B3), (E2.2) + (A3.2) + (A4.2) + (B3), (E2.2) + (A4.1) + (A4.2) + (B3);
    (E2.3) + (A1.1) + (B 1), (E2.3) + (A1.1) + (B2), (E2.3) + (A1.1) + (B3), (E2.3) + (A2.1) + (B1), (E2.3) + (A2.1) + (B2), (E2.3) + (A2.1) + (B3), (E2.3) + (A3.1) + (B1), (E2.3) + (A3.1) + (B2), (E2.3) + (A3.1) + (B3), (E2.3) + (A4.1) + (B1), (E2.3) + (A4.1) + (B2), (E2.3) + (A4.1) + (B3), (E2.3) + (A1.2) + (B1), (E2.3) + (A1.2) + (B2), (E2.3) + (A1.2) + (B3), (E2.3) + (A2.2) + (B1), (E2.3) + (A2.2) + (B2), (E2.3) + (A2.2) + (B3), (E2.3) + (A3.2) + (B1), (E2.3) + (A3.2) + (B2), (E2.3) + (A3.2) + (B3), (E2.3) + (A4.2) + (B1), (E2.3) + (A4.2) + (B2), (E2.3) + (A4.2) + (B3),
    (E2.3) + (A1.1) + (A1.2) + (B1), (E2.3) + (A1.1) + (A2.1) + (B1), (E2.3) + (A1.1) + (A2.2) + (B1), (E2.3) + (A1.1) + (A3.1) + (B1), (E2.3) + (A1.1) + (A3.2) + (B1), (E2.3) + (A1.1) + (A4.1) + (B1), (E2.3) + (A1.1) + (A4.2) + (B1);
    (E2.3) + (A1.2) + (A2.1) + (B1), (E2.3) + (A1.2) + (A2.2) + (B1), (E2.3) + (A1.2) + (A3.1) + (B1), (E2.3) + (A1.2) + (A3.2) + (B1), (E2.3) + (A1.2) + (A4.1) + (B1), (E2.3) + (A1.2) + (A4.2) + (B1);
    (E2.3) + (A2.1) + (A2.2) + (B1), (E2.3) + (A2.1) + (A3.1) + (B1), (E2.3) + (A2.1) + (A3.2) + (B1), (E2.3) + (A2.1) + (A4.1) + (B1), (E2.3) + (A2.1) + (A4.2) + (B1);
    (E2.3) + (A2.2) + (A3.1) + (B1), (E2.3) + (A2.2) + (A3.2) + (B1), (E2.3) + (A2.2) + (A4.1) + (B1), (E2.3) + (A2.2) + (A4.2) + (B1);
    (E2.3) + (A3.1) + (A3.2) + (B1), (E2.3) + (A3.1) + (A4.1) + (B1), (E2.3) + (A3.1) + (A4.2) + (B1); (E2.3) + (A3.2) + (A4.1) + (B1), (E2.3) + (A3.2) + (A4.2) + (B1), (E2.3) + (A4.1) + (A4.2) + (B1);
    (E2.3) + (A1.1) + (A1.2) + (B2), (E2.3) + (A1.1) + (A2.1) + (B2), (E2.3) + (A1.1) + (A2.2) + (B2), (E2.3) + (A1.1) + (A3.1) + (B2), (E2.3) + (A1.1) + (A3.2) + (B2), (E2.3) + (A1.1) + (A4.1) + (B2), (E2.3) + (A1.1) + (A4.2) + (B2);
    (E2.3) + (A1.2) + (A2.1) + (B2), (E2.3) + (A1.2) + (A2.2) + (B2), (E2.3) + (A1.2) + (A3.1) + (B2), (E2.3) + (A1.2) + (A3.2) + (B2), (E2.3) + (A1.2) + (A4.1) + (B2), (E2.3) + (A1.2) + (A4.2) + (B2);
    (E2.3) + (A2.1) + (A2.2) + (B2), (E2.3) + (A2.1) + (A3.1) + (B2), (E2.3) + (A2.1) + (A3.2) + (B2), (E2.3) + (A2.1) + (A4.1) + (B2), (E2.3) + (A2.1) + (A4.2) + (B2);
    (E2.3) + (A2.2) + (A3.1) + (B2), (E2.3) + (A2.2) + (A3.2) + (B2), (E2.3) + (A2.2) + (A4.1) + (B2), (E2.3) + (A2.2) + (A4.2) + (B2);
    (E2.3) + (A3.1) + (A3.2) + (B2), (E2.3) + (A3.1) + (A4.1) + (B2), (E2.3) + (A3.1) + (A4.2) + (B2); (E2.3) + (A3.2) + (A4.1) + (B2), (E2.3) + (A3.2) + (A4.2) + (B2), (E2.3) + (A4.1) + (A4.2) + (B2);
    (E2.3) + (A1.1) + (A1.2) + (B3), (E2.3) + (A1.1) + (A2.1) + (B3), (E2.3) + (A1.1) + (A2.2) + (B3), (E2.3) + (A1.1) + (A3.1) + (B3), (E2.3) + (A1.1) + (A3.2) + (B3), (E2.3) + (A1.1) + (A4.1) + (B3), (E2.3) + (A1.1) + (A4.2) + (B3);
    (E2.3) + (A1.2) + (A2.1) + (B3), (E2.3) + (A1.2) + (A2.2) + (B3), (E2.3) + (A1.2) + (A3.1) + (B3), (E2.3) + (A1.2) + (A3.2) + (B3), (E2.3) + (A1.2) + (A4.1) + (B3), (E2.3) + (A1.2) + (A4.2) + (B3);
    (E2.3) + (A2.1) + (A2.2) + (B3), (E2.3) + (A2.1) + (A3.1) + (B3), (E2.3) + (A2.1) + (A3.2) + (B3), (E2.3) + (A2.1) + (A4.1) + (B3), (E2.3) + (A2.1) + (A4.2) + (B3);
    (E2.3) + (A2.2) + (A3.1) + (B3), (E2.3) + (A2.2) + (A3.2) + (B3), (E2.3) + (A2.2) + (A4.1) + (B3), (E2.3) + (A2.2) + (A4.2) + (B3);
    (E2.3) + (A3.1) + (A3.2) + (B3), (E2.3) + (A3.1) + (A4.1) + (B3), (E2.3) + (A3.1) + (A4.2) + (B3); (E2.3) + (A3.2) + (A4.1) + (B3), (E2.3) + (A3.2) + (A4.2) + (B3), (E2.3) + (A4.1) + (A4.2) + (B3);
    (E2.4) + (A1.1) + (B1), (E2.4) + (A1.1) + (B2), (E2.4) + (A1.1) + (B3), (E2.4) + (A2.1) + (B1), (E2.4) + (A2.1) + (B2), (E2.4) + (A2.1) + (B3), (E2.4) + (A3.1) + (B1), (E2.4) + (A3.1) + (B2), (E2.4) + (A3.1) + (B3), (E2.4) + (A4.1) + (B1), (E2.4) + (A4.1) + (B2), (E2.4) + (A4.1) + (B3), (E2.4) + (A1.2) + (B1), (E2.4) + (A1.2) + (B2), (E2.4) + (A1.2) + (B3), (E2.4) + (A2.2) + (B1), (E2.4) + (A2.2) + (B2), (E2.4) + (A2.2) + (B3), (E2.4) + (A3.2) + (B1), (E2.4) + (A3.2) + (B2), (E2.4) + (A3.2) + (B3), (E2.4) + (A4.2) + (B1), (E2.4) + (A4.2) + (B2), (E2.4) + (A4.2) + (B3),
    (E2.4) + (A1.1) + (A1.2) + (B1), (E2.4) + (A1.1) + (A2.1) + (B1), (E2.4) + (A1.1) + (A2.2) + (B1), (E2.4) + (A1.1) + (A3.1) + (B1), (E2.4) + (A1.1) + (A3.2) + (B1), (E2.4) + (A1.1) + (A4.1) + (B1), (E2.4) + (A1.1) + (A4.2) + (B1);
    (E2.4) + (A1.2) + (A2.1) + (B1), (E2.4) + (A1.2) + (A2.2) + (B1), (E2.4) + (A1.2) + (A3.1) + (B1), (E2.4) + (A1.2) + (A3.2) + (B1), (E2.4) + (A1.2) + (A4.1) + (B1), (E2.4) + (A1.2) + (A4.2) + (B1);
    (E2.4) + (A2.1) + (A2.2) + (B1), (E2.4) + (A2.1) + (A3.1) + (B1), (E2.4) + (A2.1) + (A3.2) + (B1), (E2.4) + (A2.1) + (A4.1) + (B1), (E2.4) + (A2.1) + (A4.2) + (B1); (E2.4) + (A2.2) + (A3.1) + (B1), (E2.4) + (A2.2) + (A3.2) + (B1), (E2.4) + (A2.2) + (A4.1) + (B1), (E2.4) + (A2.2) + (A4.2) + (B1);
    (E2.4) + (A3.1) + (A3.2) + (B1), (E2.4) + (A3.1) + (A4.1) + (B1), (E2.4) + (A3.1) + (A4.2) + (B1); (E2.4) + (A3.2) + (A4.1) + (B1), (E2.4) + (A3.2) + (A4.2) + (B1), (E2.4) + (A4.1) + (A4.2) + (B1);
    (E2.4) + (A1.1) + (A1.2) + (B2), (E2.4) + (A1.1) + (A2.1) + (B2), (E2.4) + (A1.1) + (A2.2) + (B2), (E2.4) + (A1.1) + (A3.1) + (B2), (E2.4) + (A1.1) + (A3.2) + (B2), (E2.4) + (A1.1) + (A4.1) + (B2), (E2.4) + (A1.1) + (A4.2) + (B2);
    (E2.4) + (A1.2) + (A2.1) + (B2), (E2.4) + (A1.2) + (A2.2) + (B2), (E2.4) + (A1.2) + (A3.1) + (B2), (E2.4) + (A1.2) + (A3.2) + (B2), (E2.4) + (A1.2) + (A4.1) + (B2), (E2.4) + (A1.2) + (A4.2) + (B2);
    (E2.4) + (A2.1) + (A2.2) + (B2), (E2.4) + (A2.1) + (A3.1) + (B2), (E2.4) + (A2.1) + (A3.2) + (B2), (E2.4) + (A2.1) + (A4.1) + (B2), (E2.4) + (A2.1) + (A4.2) + (B2);
    (E2.4) + (A2.2) + (A3.1) + (B2), (E2.4) + (A2.2) + (A3.2) + (B2), (E2.4) + (A2.2) + (A4.1) + (B2), (E2.4) + (A2.2) + (A4.2) + (B2);
    (E2.4) + (A3.1) + (A3.2) + (B2), (E2.4) + (A3.1) + (A4.1) + (B2), (E2.4) + (A3.1) + (A4.2) + (B2); (E2.4) + (A3.2) + (A4.1) + (B2), (E2.4) + (A3.2) + (A4.2) + (B2), (E2.4) + (A4.1) + (A4.2) + (B2);
    (E2.4) + (A1.1) + (A1.2) + (B3), (E2.4) + (A1.1) + (A2.1) + (B3), (E2.4) + (A1.1) + (A2.2) + (B3), (E2.4) + (A1.1) + (A3.1) + (B3), (E2.4) + (A1.1) + (A3.2) + (B3), (E2.4) + (A1.1) + (A4.1) + (B3), (E2.4) + (A1.1) + (A4.2) + (B3);
    (E2.4) + (A1.2) + (A2.1) + (B3), (E2.4) + (A1.2) + (A2.2) + (B3), (E2.4) + (A1.2) + (A3.1) + (B3), (E2.4) + (A1.2) + (A3.2) + (B3), (E2.4) + (A1.2) + (A4.1) + (B3), (E2.4) + (A1.2) + (A4.2) + (B3);
    (E2.4) + (A2.1) + (A2.2) + (B3), (E2.4) + (A2.1) + (A3.1) + (B3), (E2.4) + (A2.1) + (A3.2) + (B3), (E2.4) + (A2.1) + (A4.1) + (B3), (E2.4) + (A2.1) + (A4.2) + (B3);
    (E2.4) + (A2.2) + (A3.1) + (B3), (E2.4) + (A2.2) + (A3.2) + (B3), (E2.4) + (A2.2) + (A4.1) + (B3), (E2.4) + (A2.2) + (A4.2) + (B3);
    (E2.4) + (A3.1) + (A3.2) + (B3), (E2.4) + (A3.1) + (A4.1) + (B3), (E2.4) + (A3.1) + (A4.2) + (B3); (E2.4) + (A3.2) + (A4.1) + (B3), (E2.4) + (A3.2) + (A4.2) + (B3), (E2.4) + (A4.1) + (A4.2) + (B3);
    (E2.5) + (A1.1) + (B1), (E2.5) + (A1.1) + (B2), (E2.5) + (A1.1) + (B3), (E2.5) + (A2.1) + (B1), (E2.5) + (A2.1) + (B2), (E2.5) + (A2.1) + (B3), (E2.5) + (A3.1) + (B1), (E2.5) + (A3.1) + (B2), (E2.5) + (A3.1) + (B3), (E2.5) + (A4.1) + (B1), (E2.5) + (A4.1) + (B2), (E2.5) + (A4.1) + (B3), (E2.5) + (A1.2) + (B1), (E2.5) + (A1.2) + (B2), (E2.5) + (A1.2) + (B3), (E2.5) + (A2.2) + (B1), (E2.5) + (A2.2) + (B2), (E2.5) + (A2.2) + (B3), (E2.5) + (A3.2) + (B1), (E2.5) + (A3.2) + (B2), (E2.5) + (A3.2) + (B3), (E2.5) + (A4.2) + (B1), (E2.5) + (A4.2) + (B2), (E2.5) + (A4.2) + (B3),
    (E2.5) + (A1.1) + (A1.2) + (B1), (E2.5) + (A1.1) + (A2.1) + (B1), (E2.5) + (A1.1) + (A2.2) + (B1), (E2.5) + (A1.1) + (A3.1) + (B1), (E2.5) + (A1.1) + (A3.2) + (B1), (E2.5) + (A1.1) + (A4.1) + (B1), (E2.5) + (A1.1) + (A4.2) + (B1);
    (E2.5) + (A1.2) + (A2.1) + (B1), (E2.5) + (A1.2) + (A2.2) + (B1), (E2.5) + (A1.2) + (A3.1) + (B1), (E2.5) + (A1.2) + (A3.2) + (B1), (E2.5) + (A1.2) + (A4.1) + (B1), (E2.5) + (A1.2) + (A4.2) + (B1);
    (E2.5) + (A2.1) + (A2.2) + (B1), (E2.5) + (A2.1) + (A3.1) + (B1), (E2.5) + (A2.1) + (A3.2) + (B1), (E2.5) + (A2.1) + (A4.1) + (B1), (E2.5) + (A2.1) + (A4.2) + (B1);
    (E2.5) + (A2.2) + (A3.1) + (B1), (E2.5) + (A2.2) + (A3.2) + (B1), (E2.5) + (A2.2) + (A4.1) + (B1), (E2.5) + (A2.2) + (A4.2) + (B1);
    (E2.5) + (A3.1) + (A3.2) + (B1), (E2.5) + (A3.1) + (A4.1) + (B1), (E2.5) + (A3.1) + (A4.2) + (B1); (E2.5) + (A3.2) + (A4.1) + (B1), (E2.5) + (A3.2) + (A4.2) + (B1), (E2.5) + (A4.1) + (A4.2) + (B1);
    (E2.5) + (A1.1) + (A1.2) + (B2), (E2.5) + (A1.1) + (A2.1) + (B2), (E2.5) + (A1.1) + (A2.2) + (B2), (E2.5) + (A1.1) + (A3.1) + (B2), (E2.5) + (A1.1) + (A3.2) + (B2), (E2.5) + (A1.1) + (A4.1) + (B2), (E2.5) + (A1.1) + (A4.2) + (B2);
    (E2.5) + (A1.2) + (A2.1) + (B2), (E2.5) + (A1.2) + (A2.2) + (B2), (E2.5) + (A1.2) + (A3.1) + (B2), (E2.5) + (A1.2) + (A3.2) + (B2), (E2.5) + (A1.2) + (A4.1) + (B2), (E2.5) + (A1.2) + (A4.2) + (B2);
    (E2.5) + (A2.1) + (A2.2) + (B2), (E2.5) + (A2.1) + (A3.1) + (B2), (E2.5) + (A2.1) + (A3.2) + (B2), (E2.5) + (A2.1) + (A4.1) + (B2), (E2.5) + (A2.1) + (A4.2) + (B2); (E2.5) + (A2.2) + (A3.1) + (B2), (E2.5) + (A2.2) + (A3.2) + (B2), (E2.5) + (A2.2) + (A4.1) + (B2), (E2.5) + (A2.2) + (A4.2) + (B2);
    (E2.5) + (A3.1) + (A3.2) + (B2), (E2.5) + (A3.1) + (A4.1) + (B2), (E2.5) + (A3.1) + (A4.2) + (B2); (E2.5) + (A3.2) + (A4.1) + (B2), (E2.5) + (A3.2) + (A4.2) + (B2), (E2.5) + (A4.1) + (A4.2) + (B2);
    (E2.5) + (A1.1) + (A1.2) + (B3), (E2.5) + (A1.1) + (A2.1) + (B3), (E2.5) + (A1.1) + (A2.2) + (B3), (E2.5) + (A1.1) + (A3.1) + (B3), (E2.5) + (A1.1) + (A3.2) + (B3), (E2.5) + (A1.1) + (A4.1) + (B3), (E2.5) + (A1.1) + (A4.2) + (B3);
    (E2.5) + (A1.2) + (A2.1) + (B3), (E2.5) + (A1.2) + (A2.2) + (B3), (E2.5) + (A1.2) + (A3.1) + (B3), (E2.5) + (A1.2) + (A3.2) + (B3), (E2.5) + (A1.2) + (A4.1) + (B3), (E2.5) + (A1.2) + (A4.2) + (B3);
    (E2.5) + (A2.1) + (A2.2) + (B3), (E2.5) + (A2.1) + (A3.1) + (B3), (E2.5) + (A2.1) + (A3.2) + (B3), (E2.5) + (A2.1) + (A4.1) + (B3), (E2.5) + (A2.1) + (A4.2) + (B3);
    (E2.5) + (A2.2) + (A3.1) + (B3), (E2.5) + (A2.2) + (A3.2) + (B3), (E2.5) + (A2.2) + (A4.1) + (B3), (E2.5) + (A2.2) + (A4.2) + (B3);
    (E2.5) + (A3.1) + (A3.2) + (B3), (E2.5) + (A3.1) + (A4.1) + (B3), (E2.5) + (A3.1) + (A4.2) + (B3); (E2.5) + (A3.2) + (A4.1) + (B3), (E2.5) + (A3.2) + (A4.2) + (B3), (E2.5) + (A4.1) + (A4.2) + (B3);
    (E2.6) + (A1.1) + (B1), (E2.6) + (A1.1) + (B2), (E2.6) + (A1.1) + (B3), (E2.6) + (A2.1) + (B1), (E2.6) + (A2.1) + (B2), (E2.6) + (A2.1) + (B3), (E2.6) + (A3.1) + (B1), (E2.6) + (A3.1) + (B2), (E2.6) + (A3.1) + (B3), (E2.6) + (A4.1) + (B1), (E2.6) + (A4.1) + (B2), (E2.6) + (A4.1) + (B3), (E2.6) + (A1.2) + (B1), (E2.6) + (A1.2) + (B2), (E2.6) + (A1.2) + (B3), (E2.6) + (A2.2) + (B1), (E2.6) + (A2.2) + (B2), (E2.6) + (A2.2) + (B3), (E2.6) + (A3.2) + (B1), (E2.6) + (A3.2) + (B2), (E2.6) + (A3.2) + (B3), (E2.6) + (A4.2) + (B1), (E2.6) + (A4.2) + (B2), (E2.6) + (A4.2) + (B3),
    (E2.6) + (A1.1) + (A1.2) + (B1), (E2.6) + (A1.1) + (A2.1) + (B1), (E2.6) + (A1.1) + (A2.2) + (B1), (E2.6) + (A1.1) + (A3.1) + (B1), (E2.6) + (A1.1) + (A3.2) + (B1), (E2.6) + (A1.1) + (A4.1) + (B1), (E2.6) + (A1.1) + (A4.2) + (B1);
    (E2.6) + (A1.2) + (A2.1) + (B1), (E2.6) + (A1.2) + (A2.2) + (B1), (E2.6) + (A1.2) + (A3.1) + (B1), (E2.6) + (A1.2) + (A3.2) + (B1), (E2.6) + (A1.2) + (A4.1) + (B1), (E2.6) + (A1.2) + (A4.2) + (B1);
    (E2.6) + (A2.1) + (A2.2) + (B1), (E2.6) + (A2.1) + (A3.1) + (B1), (E2.6) + (A2.1) + (A3.2) + (B1), (E2.6) + (A2.1) + (A4.1) + (B1), (E2.6) + (A2.1) + (A4.2) + (B1);
    (E2.6) + (A2.2) + (A3.1) + (B1), (E2.6) + (A2.2) + (A3.2) + (B1), (E2.6) + (A2.2) + (A4.1) + (B1), (E2.6) + (A2.2) + (A4.2) + (B1);
    (E2.6) + (A3.1) + (A3.2) + (B1), (E2.6) + (A3.1) + (A4.1) + (B1), (E2.6) + (A3.1) + (A4.2) + (B1); (E2.6) + (A3.2) + (A4.1) + (B1), (E2.6) + (A3.2) + (A4.2) + (B1), (E2.6) + (A4.1) + (A4.2) + (B1);
    (E2.6) + (A1.1) + (A1.2) + (B2), (E2.6) + (A1.1) + (A2.1) + (B2), (E2.6) + (A1.1) + (A2.2) + (B2), (E2.6) + (A1.1) + (A3.1) + (B2), (E2.6) + (A1.1) + (A3.2) + (B2), (E2.6) + (A1.1) + (A4.1) + (B2), (E2.6) + (A1.1) + (A4.2) + (B2);
    (E2.6) + (A1.2) + (A2.1) + (B2), (E2.6) + (A1.2) + (A2.2) + (B2), (E2.6) + (A1.2) + (A3.1) + (B2), (E2.6) + (A1.2) + (A3.2) + (B2), (E2.6) + (A1.2) + (A4.1) + (B2), (E2.6) + (A1.2) + (A4.2) + (B2);
    (E2.6) + (A2.1) + (A2.2) + (B2), (E2.6) + (A2.1) + (A3.1) + (B2), (E2.6) + (A2.1) + (A3.2) + (B2), (E2.6) + (A2.1) + (A4.1) + (B2), (E2.6) + (A2.1) + (A4.2) + (B2);
    (E2.6) + (A2.2) + (A3.1) + (B2), (E2.6) + (A2.2) + (A3.2) + (B2), (E2.6) + (A2.2) + (A4.1) + (B2), (E2.6) + (A2.2) + (A4.2) + (B2);
    (E2.6) + (A3.1) + (A3.2) + (B2), (E2.6) + (A3.1) + (A4.1) + (B2), (E2.6) + (A3.1) + (A4.2) + (B2); (E2.6) + (A3.2) + (A4.1) + (B2), (E2.6) + (A3.2) + (A4.2) + (B2), (E2.6) + (A4.1) + (A4.2) + (B2);
    (E2.6) + (A1.1) + (A1.2) + (B3), (E2.6) + (A1.1) + (A2.1) + (B3), (E2.6) + (A1.1) + (A2.2) + (B3), (E2.6) + (A1.1) + (A3.1) + (B3), (E2.6) + (A1.1) + (A3.2) + (B3), (E2.6) + (A1.1) + (A4.1) + (B3), (E2.6) + (A1.1) + (A4.2) + (B3);
    (E2.6) + (A1.2) + (A2.1) + (B3), (E2.6) + (A1.2) + (A2.2) + (B3), (E2.6) + (A1.2) + (A3.1) + (B3), (E2.6) + (A1.2) + (A3.2) + (B3), (E2.6) + (A1.2) + (A4.1) + (B3), (E2.6) + (A1.2) + (A4.2) + (B3);
    (E2.6) + (A2.1) + (A2.2) + (B3), (E2.6) + (A2.1) + (A3.1) + (B3), (E2.6) + (A2.1) + (A3.2) + (B3), (E2.6) + (A2.1) + (A4.1) + (B3), (E2.6) + (A2.1) + (A4.2) + (B3);
    (E2.6) + (A2.2) + (A3.1) + (B3), (E2.6) + (A2.2) + (A3.2) + (B3), (E2.6) + (A2.2) + (A4.1) + (B3), (E2.6) + (A2.2) + (A4.2) + (B3);
    (E2.6) + (A3.1) + (A3.2) + (B3), (E2.6) + (A3.1) + (A4.1) + (B3), (E2.6) + (A3.1) + (A4.2) + (B3); (E2.6) + (A3.2) + (A4.1) + (B3), (E2.6) + (A3.2) + (A4.2) + (B3), (E2.6) + (A4.1) + (A4.2) + (B3);
    (E2.7) + (A1.1) + (B1), (E2.7) + (A1.1) + (B2), (E2.7) + (A1.1) + (B3), (E2.7) + (A2.1) + (B1), (E2.7) + (A2.1) + (B2), (E2.7) + (A2.1) + (B3), (E2.7) + (A3.1) + (B1), (E2.7) + (A3.1) + (B2), (E2.7) + (A3.1) + (B3), (E2.7) + (A4.1) + (B1), (E2.7) + (A4.1) + (B2), (E2.7) + (A4.1) + (B3), (E2.7) + (A1.2) + (B1), (E2.7) + (A1.2) + (B2), (E2.7) + (A1.2) + (B3), (E2.7) + (A2.2) + (B1), (E2.7) + (A2.2) + (B2), (E2.7) + (A2.2) + (B3), (E2.7) + (A3.2) + (B1), (E2.7) + (A3.2) + (B2), (E2.7) + (A3.2) + (B3), (E2.7) + (A4.2) + (B1), (E2.7) + (A4.2) + (B2), (E2.7) + (A4.2) + (B3),
    (E2.7) + (A1.1) + (A1.2) + (B1), (E2.7) + (A1.1) + (A2.1) + (B1), (E2.7) + (A1.1) + (A2.2) + (B1), (E2.7) + (A1.1) + (A3.1) + (B1), (E2.7) + (A1.1) + (A3.2) + (B1), (E2.7) + (A1.1) + (A4.1) + (B1), (E2.7) + (A1.1) + (A4.2) + (B1);
    (E2.7) + (A1.2) + (A2.1) + (B1), (E2.7) + (A1.2) + (A2.2) + (B1), (E2.7) + (A1.2) + (A3.1) + (B1), (E2.7) + (A1.2) + (A3.2) + (B1), (E2.7) + (A1.2) + (A4.1) + (B1), (E2.7) + (A1.2) + (A4.2) + (B1);
    (E2.7) + (A2.1) + (A2.2) + (B1), (E2.7) + (A2.1) + (A3.1) + (B1), (E2.7) + (A2.1) + (A3.2) + (B1), (E2.7) + (A2.1) + (A4.1) + (B1), (E2.7) + (A2.1) + (A4.2) + (B1);
    (E2.7) + (A2.2) + (A3.1) + (B1), (E2.7) + (A2.2) + (A3.2) + (B1), (E2.7) + (A2.2) + (A4.1) + (B1), (E2.7) + (A2.2) + (A4.2) + (B1);
    (E2.7) + (A3.1) + (A3.2) + (B1), (E2.7) + (A3.1) + (A4.1) + (B1), (E2.7) + (A3.1) + (A4.2) + (B1); (E2.7) + (A3.2) + (A4.1) + (B1), (E2.7) + (A3.2) + (A4.2) + (B1), (E2.7) + (A4.1) + (A4.2) + (B1);
    (E2.7) + (A1.1) + (A1.2) + (B2), (E2.7) + (A1.1) + (A2.1) + (B2), (E2.7) + (A1.1) + (A2.2) + (B2), (E2.7) + (A1.1) + (A3.1) + (B2), (E2.7) + (A1.1) + (A3.2) + (B2), (E2.7) + (A1.1) + (A4.1) + (B2), (E2.7) + (A1.1) + (A4.2) + (B2);
    (E2.7) + (A1.2) + (A2.1) + (B2), (E2.7) + (A1.2) + (A2.2) + (B2), (E2.7) + (A1.2) + (A3.1) + (B2), (E2.7) + (A1.2) + (A3.2) + (B2), (E2.7) + (A1.2) + (A4.1) + (B2), (E2.7) + (A1.2) + (A4.2) + (B2);
    (E2.7) + (A2.1) + (A2.2) + (B2), (E2.7) + (A2.1) + (A3.1) + (B2), (E2.7) + (A2.1) + (A3.2) + (B2), (E2.7) + (A2.1) + (A4.1) + (B2), (E2.7) + (A2.1) + (A4.2) + (B2);
    (E2.7) + (A2.2) + (A3.1) + (B2), (E2.7) + (A2.2) + (A3.2) + (B2), (E2.7) + (A2.2) + (A4.1) + (B2), (E2.7) + (A2.2) + (A4.2) + (B2);
    (E2.7) + (A3.1) + (A3.2) + (B2), (E2.7) + (A3.1) + (A4.1) + (B2), (E2.7) + (A3.1) + (A4.2) + (B2); (E2.7) + (A3.2) + (A4.1) + (B2), (E2.7) + (A3.2) + (A4.2) + (B2), (E2.7) + (A4.1) + (A4.2) + (B2);
    (E2.7) + (A1.1) + (A1.2) + (B3), (E2.7) + (A1.1) + (A2.1) + (B3), (E2.7) + (A1.1) + (A2.2) + (B3), (E2.7) + (A1.1) + (A3.1) + (B3), (E2.7) + (A1.1) + (A3.2) + (B3), (E2.7) + (A1.1) + (A4.1) + (B3), (E2.7) + (A1.1) + (A4.2) + (B3);
    (E2.7) + (A1.2) + (A2.1) + (B3), (E2.7) + (A1.2) + (A2.2) + (B3), (E2.7) + (A1.2) + (A3.1) + (B3), (E2.7) + (A1.2) + (A3.2) + (B3), (E2.7) + (A1.2) + (A4.1) + (B3), (E2.7) + (A1.2) + (A4.2) + (B3);
    (E2.7) + (A2.1) + (A2.2) + (B3), (E2.7) + (A2.1) + (A3.1) + (B3), (E2.7) + (A2.1) + (A3.2) + (B3), (E2.7) + (A2.1) + (A4.1) + (B3), (E2.7) + (A2.1) + (A4.2) + (B3);
    (E2.7) + (A2.2) + (A3.1) + (B3), (E2.7) + (A2.2) + (A3.2) + (B3), (E2.7) + (A2.2) + (A4.1) + (B3), (E2.7) + (A2.2) + (A4.2) + (B3);
    (E2.7) + (A3.1) + (A3.2) + (B3), (E2.7) + (A3.1) + (A4.1) + (B3), (E2.7) + (A3.1) + (A4.2) + (B3); (E2.7) + (A3.2) + (A4.1) + (B3), (E2.7) + (A3.2) + (A4.2) + (B3), (E2.7) + (A4.1) + (A4.2) + (B3);
    (E2.8) + (A1.1) + (B1), (E2.8) + (A1.1) + (B2), (E2.8) + (A1.1) + (B3), (E2.8) + (A2.1) + (B1), (E2.8) + (A2.1) + (B2), (E2.8) + (A2.1) + (B3), (E2.8) + (A3.1) + (B1), (E2.8) + (A3.1) + (B2), (E2.8) + (A3.1) + (B3), (E2.8) + (A4.1) + (B1), (E2.8) + (A4.1) + (B2), (E2.8) + (A4.1) + (B3), (E2.8) + (A1.2) + (B1), (E2.8) + (A1.2) + (B2), (E2.8) + (A1.2) + (B3), (E2.8) + (A2.2) + (B1), (E2.8) + (A2.2) + (B2), (E2.8) + (A2.2) + (B3), (E2.8) + (A3.2) + (B1), (E2.8) + (A3.2) + (B2), (E2.8) + (A3.2) + (B3), (E2.8) + (A4.2) + (B1), (E2.8) + (A4.2) + (B2), (E2.8) + (A4.2) + (B3),
    (E2.8) + (A1.1) + (A1.2) + (B1), (E2.8) + (A1.1) + (A2.1) + (B1), (E2.8) + (A1.1) + (A2.2) + (B1), (E2.8) + (A1.1) + (A3.1) + (B1), (E2.8) + (A1.1) + (A3.2) + (B1), (E2.8) + (A1.1) + (A4.1) + (B1), (E2.8) + (A1.1) + (A4.2) + (B1);
    (E2.8) + (A1.2) + (A2.1) + (B1), (E2.8) + (A1.2) + (A2.2) + (B1), (E2.8) + (A1.2) + (A3.1) + (B1), (E2.8) + (A1.2) + (A3.2) + (B1), (E2.8) + (A1.2) + (A4.1) + (B1), (E2.8) + (A1.2) + (A4.2) + (B1);
    (E2.8) + (A2.1) + (A2.2) + (B1), (E2.8) + (A2.1) + (A3.1) + (B1), (E2.8) + (A2.1) + (A3.2) + (B1), (E2.8) + (A2.1) + (A4.1) + (B1), (E2.8) + (A2.1) + (A4.2) + (B1);
    (E2.8) + (A2.2) + (A3.1) + (B1), (E2.8) + (A2.2) + (A3.2) + (B1), (E2.8) + (A2.2) + (A4.1) + (B1), (E2.8) + (A2.2) + (A4.2) + (B1);
    (E2.8) + (A3.1) + (A3.2) + (B1), (E2.8) + (A3.1) + (A4.1) + (B1), (E2.8) + (A3.1) + (A4.2) + (B1); (E2.8) + (A3.2) + (A4.1) + (B1), (E2.8) + (A3.2) + (A4.2) + (B1), (E2.8) + (A4.1) + (A4.2) + (B1);
    (E2.8) + (A1.1) + (A1.2) + (B2), (E2.8) + (A1.1) + (A2.1) + (B2), (E2.8) + (A1.1) + (A2.2) + (B2), (E2.8) + (A1.1) + (A3.1) + (B2), (E2.8) + (A1.1) + (A3.2) + (B2), (E2.8) + (A1.1) + (A4.1) + (B2), (E2.8) + (A1.1) + (A4.2) + (B2);
    (E2.8) + (A1.2) + (A2.1) + (B2), (E2.8) + (A1.2) + (A2.2) + (B2), (E2.8) + (A1.2) + (A3.1) + (B2), (E2.8) + (A1.2) + (A3.2) + (B2), (E2.8) + (A1.2) + (A4.1) + (B2), (E2.8) + (A1.2) + (A4.2) + (B2);
    (E2.8) + (A2.1) + (A2.2) + (B2), (E2.8) + (A2.1) + (A3.1) + (B2), (E2.8) + (A2.1) + (A3.2) + (B2), (E2.8) + (A2.1) + (A4.1) + (B2), (E2.8) + (A2.1) + (A4.2) + (B2);
    (E2.8) + (A2.2) + (A3.1) + (B2), (E2.8) + (A2.2) + (A3.2) + (B2), (E2.8) + (A2.2) + (A4.1) + (B2), (E2.8) + (A2.2) + (A4.2) + (B2);
    (E2.8) + (A3.1) + (A3.2) + (B2), (E2.8) + (A3.1) + (A4.1) + (B2), (E2.8) + (A3.1) + (A4.2) + (B2); (E2.8) + (A3.2) + (A4.1) + (B2), (E2.8) + (A3.2) + (A4.2) + (B2), (E2.8) + (A4.1) + (A4.2) + (B2);
    (E2.8) + (A1.1) + (A1.2) + (B3), (E2.8) + (A1.1) + (A2.1) + (B3), (E2.8) + (A1.1) + (A2.2) + (B3), (E2.8) + (A1.1) + (A3.1) + (B3), (E2.8) + (A1.1) + (A3.2) + (B3), (E2.8) + (A1.1) + (A4.1) + (B3), (E2.8) + (A1.1) + (A4.2) + (B3);
    (E2.8) + (A1.2) + (A2.1) + (B3), (E2.8) + (A1.2) + (A2.2) + (B3), (E2.8) + (A1.2) + (A3.1) + (B3), (E2.8) + (A1.2) + (A3.2) + (B3), (E2.8) + (A1.2) + (A4.1) + (B3), (E2.8) + (A1.2) + (A4.2) + (B3);
    (E2.8) + (A2.1) + (A2.2) + (B3), (E2.8) + (A2.1) + (A3.1) + (B3), (E2.8) + (A2.1) + (A3.2) + (B3), (E2.8) + (A2.1) + (A4.1) + (B3), (E2.8) + (A2.1) + (A4.2) + (B3);
    (E2.8) + (A2.2) + (A3.1) + (B3), (E2.8) + (A2.2) + (A3.2) + (B3), (E2.8) + (A2.2) + (A4.1) + (B3), (E2.8) + (A2.2) + (A4.2) + (B3);
    (E2.8) + (A3.1) + (A3.2) + (B3), (E2.8) + (A3.1) + (A4.1) + (B3), (E2.8) + (A3.1) + (A4.2) + (B3); (E2.8) + (A3.2) + (A4.1) + (B3), (E2.8) + (A3.2) + (A4.2) + (B3), (E2.8) + (A4.1) + (A4.2) + (B3);
    (E2.9) + (A1.1) + (B1), (E2.9) + (A1.1) + (B2), (E2.9) + (A1.1) + (B3), (E2.9) + (A2.1) + (B1), (E2.9) + (A2.1) + (B2), (E2.9) + (A2.1) + (B3), (E2.9) + (A3.1) + (B1), (E2.9) + (A3.1) + (B2), (E2.9) + (A3.1) + (B3), (E2.9) + (A4.1) + (B1), (E2.9) + (A4.1) + (B2), (E2.9) + (A4.1) + (B3), (E2.9) + (A1.2) + (B1), (E2.9) + (A1.2) + (B2), (E2.9) + (A1.2) + (B3), (E2.9) + (A2.2) + (B1), (E2.9) + (A2.2) + (B2), (E2.9) + (A2.2) + (B3), (E2.9) + (A3.2) + (B1), (E2.9) + (A3.2) + (B2), (E2.9) + (A3.2) + (B3), (E2.9) + (A4.2) + (B1), (E2.9) + (A4.2) + (B2), (E2.9) + (A4.2) + (B3),
    (E2.9) + (A1.1) + (A1.2) + (B1), (E2.9) + (A1.1) + (A2.1) + (B1), (E2.9) + (A1.1) + (A2.2) + (B1), (E2.9) + (A1.1) + (A3.1) + (B1), (E2.9) + (A1.1) + (A3.2) + (B1), (E2.9) + (A1.1) + (A4.1) + (B1), (E2.9) + (A1.1) + (A4.2) + (B1);
    (E2.9) + (A1.2) + (A2.1) + (B1), (E2.9) + (A1.2) + (A2.2) + (B1), (E2.9) + (A1.2) + (A3.1) + (B1), (E2.9) + (A1.2) + (A3.2) + (B1), (E2.9) + (A1.2) + (A4.1) + (B1), (E2.9) + (A1.2) + (A4.2) + (B1);
    (E2.9) + (A2.1) + (A2.2) + (B1), (E2.9) + (A2.1) + (A3.1) + (B1), (E2.9) + (A2.1) + (A3.2) + (B1), (E2.9) + (A2.1) + (A4.1) + (B1), (E2.9) + (A2.1) + (A4.2) + (B1);
    (E2.9) + (A2.2) + (A3.1) + (B1), (E2.9) + (A2.2) + (A3.2) + (B1), (E2.9) + (A2.2) + (A4.1) + (B1), (E2.9) + (A2.2) + (A4.2) + (B1);
    (E2.9) + (A3.1) + (A3.2) + (B1), (E2.9) + (A3.1) + (A4.1) + (B1), (E2.9) + (A3.1) + (A4.2) + (B1); (E2.9) + (A3.2) + (A4.1) + (B1), (E2.9) + (A3.2) + (A4.2) + (B1), (E2.9) + (A4.1) + (A4.2 ) + (B1);
    (E2.9) + (A1.1) + (A1.2) + (B2), (E2.9) + (A1.1) + (A2.1) + (B2), (E2.9) + (A1.1) + (A2.2) + (B2), (E2.9) + (A1.1) + (A3.1) + (B2), (E2.9) + (A1.1) + (A3.2) + (B2), (E2.9) + (A1.1) + (A4.1) + (B2), (E2.9) + (A1.1) + (A4.2) + (B2);
    (E2.9) + (A1.2) + (A2.1) + (B2), (E2.9) + (A1.2) + (A2.2) + (B2), (E2.9) + (A1.2) + (A3.1) + (B2), (E2.9) + (A1.2) + (A3.2) + (B2), (E2.9) + (A1.2) + (A4.1) + (B2), (E2.9) + (A1.2) + (A4.2) + (B2);
    (E2.9) + (A2.1) + (A2.2) + (B2), (E2.9) + (A2.1) + (A3.1) + (B2), (E2.9) + (A2.1) + (A3.2) + (B2), (E2.9) + (A2.1) + (A4.1) + (B2), (E2.9) + (A2.1) + (A4.2) + (B2);
    (E2.9) + (A2.2) + (A3.1) + (B2), (E2.9) + (A2.2) + (A3.2) + (B2), (E2.9) + (A2.2) + (A4.1) + (B2), (E2.9) + (A2.2) + (A4.2) + (B2);
    (E2.9) + (A3.1) + (A3.2) + (B2), (E2.9) + (A3.1) + (A4.1) + (B2), (E2.9) + (A3.1) + (A4.2) + (B2); (E2.9) + (A3.2) + (A4.1) + (B2), (E2.9) + (A3.2) + (A4.2) + (B2), (E2.9) + (A4.1) + (A4.2) + (B2);
    (E2.9) + (A1.1) + (A1.2) + (B3), (E2.9) + (A1.1) + (A2.1) + (B3), (E2.9) + (A1.1) + (A2.2) + (B3), (E2.9) + (A1.1) + (A3.1) + (B3), (E2.9) + (A1.1) + (A3.2) + (B3), (E2.9) + (A1.1) + (A4.1) + (B3), (E2.9) + (A1.1) + (A4.2) + (B3);
    (E2.9) + (A1.2) + (A2.1) + (B3), (E2.9) + (A1.2) + (A2.2) + (B3), (E2.9) + (A1.2) + (A3.1) + (B3), (E2.9) + (A1.2) + (A3.2) + (B3), (E2.9) + (A1.2) + (A4.1) + (B3), (E2.9) + (A1.2) + (A4.2) + (B3);
    (E2.9) + (A2.1) + (A2.2) + (B3), (E2.9) + (A2.1) + (A3.1) + (B3), (E2.9) + (A2.1) + (A3.2) + (B3), (E2.9) + (A2.1) + (A4.1) + (B3), (E2.9) + (A2.1) + (A4.2) + (B3);
    (E2.9) + (A2.2) + (A3.1) + (B3), (E2.9) + (A2.2) + (A3.2) + (B3), (E2.9) + (A2.2) + (A4.1) + (B3), (E2.9) + (A2.2) + (A4.2) + (B3);
    (E2.9) + (A3.1) + (A3.2) + (B3), (E2.9) + (A3.1) + (A4.1) + (B3), (E2.9) + (A3.1) + (A4.2) + (B3); (E2.9) + (A3.2) + (A4.1) + (B3), (E2.9) + (A3.2) + (A4.2) + (B3), (E2.9) + (A4.1) + (A4.2) + (B3);
    (E3) + (A1.1) + (B1), (E3) + (A1.1) + (B2), (E3) + (A1.1) + (B3), (E3) + (A2.1) + (B1), (E3) + (A2.1) + (B2), (E3) + (A2.1) + (B3), (E3) + (A3.1) + (B1), (E3) + (A3.1) + (B2), (E3) + (A3.1) + (B3), (E3) + (A4.1) + (B1), (E3) + (A4.1) + (B2), (E3) + (A4.1) + (B3), (E3) + (A1.2) + (B1), (E3) + (A1.2) + (B2), (E3) + (A1.2) + (B3), (E3) + (A2.2) + (B1), (E3) + (A2.2) + (B2), (E3) + (A2.2) + (B3), (E3) + (A3.2) + (B1), (E3) + (A3.2) + (B2), (E3) + (A3.2) + (B3), (E3) + (A4.2) + (B1), (E3) + (A4.2) + (B2), (E3) + (A4.2) + (B3), (E3) + (A1.1) + (A1.2) + (B1), (E3) + (A1.1) + (A2.1) + (B1), (E3) + (A1.1) + (A2.2) + (B1), (E3) + (A1.1) + (A3.1) + (B1), (E3) + (A1.1) + (A3.2) + (B1), (E3) + (A1.1) + (A4.1) + (B1), (E3) + (A1.1) + (A4.2) + (B1);
    (E3) + (A1.2) + (A2.1) + (B1), (E3) + (A1.2) + (A2.2) + (B1), (E3) + (A1.2) + (A3.1) + (B1), (E3) + (A1.2) + (A3.2) + (B1), (E3) + (A1.2) + (A4.1) + (B1), (E3) + (A1.2) + (A4.2) + (B1);
    (E3) + (A2.1) + (A2.2) + (B1), (E3) + (A2.1) + (A3.1) + (B1), (E3) + (A2.1) + (A3.2) + (B1), (E3) + (A2.1) + (A4.1) + (B1), (E3) + (A2.1) + (A4.2) + (B1);
    (E3) + (A2.2) + (A3.1) + (B1), (E3) + (A2.2) + (A3.2) + (B1), (E3) + (A2.2) + (A4.1) + (B1), (E3) + (A2.2) + (A4.2) + (B1);
    (E3) + (A3.1) + (A3.2) + (B1), (E3) + (A3.1) + (A4.1) + (B1), (E3) + (A3.1) + (A4.2) + (B1); (E3) + (A3.2) + (A4.1) + (B1), (E3) + (A3.2) + (A4.2) + (B1), (E3) + (A4.1) + (A4.2) + (B1);
    (E3) + (A1.1) + (A1.2) + (B2), (E3) + (A1.1) + (A2.1) + (B2), (E3) + (A1.1) + (A2.2) + (B2), (E3) + (A1.1) + (A3.1) + (B2), (E3) + (A1.1) + (A3.2) + (B2), (E3) + (A1.1) + (A4.1) + (B2), (E3) + (A1.1) + (A4.2) + (B2);
    (E3) + (A1.2) + (A2.1) + (B2), (E3) + (A1.2) + (A2.2) + (B2), (E3) + (A1.2) + (A3.1) + (B2), (E3) + (A1.2) + (A3.2) + (B2), (E3) + (A1.2) + (A4.1) + (B2), (E3) + (A1.2) + (A4.2) + (B2);
    (E3) + (A2.1) + (A2.2) + (B2), (E3) + (A2.1) + (A3.1) + (B2), (E3) + (A2.1) + (A3.2) + (B2), (E3) + (A2.1) + (A4.1) + (B2), (E3) + (A2.1) + (A4.2) + (B2);
    (E3) + (A2.2) + (A3.1) + (B2), (E3) + (A2.2) + (A3.2) + (B2), (E3) + (A2.2) + (A4.1) + (B2), (E3) + (A2.2) + (A4.2) + (B2);
    (E3) + (A3.1) + (A3.2) + (B2), (E3) + (A3.1) + (A4.1) + (B2), (E3) + (A3.1) + (A4.2) + (B2); (E3) + (A3.2) + (A4.1) + (B2), (E3) + (A3.2) + (A4.2) + (B2), (E3) + (A4.1) + (A4.2) + (B2);
    (E3) + (A1.1) + (A1.2) + (B3), (E3) + (A1.1) + (A2.1) + (B3), (E3) + (A1.1) + (A2.2) + (B3), (E3) + (A1.1) + (A3.1) + (B3), (E3) + (A1.1) + (A3.2) + (B3), (E3) + (A1.1) + (A4.1) + (B3), (E3) + (A1.1) + (A4.2) + (B3);
    (E3) + (A1.2) + (A2.1) + (B3), (E3) + (A1.2) + (A2.2) + (B3), (E3) + (A1.2) + (A3.1) + (B3), (E3) + (A1.2) + (A3.2) + (B3), (E3) + (A1.2) + (A4.1) + (B3), (E3) + (A1.2) + (A4.2) + (B3);
    (E3) + (A2.1) + (A2.2) + (B3), (E3) + (A2.1) + (A3.1) + (B3), (E3) + (A2.1) + (A3.2) + (B3), (E3) + (A2.1) + (A4.1) + (B3), (E3) + (A2.1) + (A4.2) + (B3);
    (E3) + (A2.2) + (A3.1) + (B3), (E3) + (A2.2) + (A3.2) + (B3), (E3) + (A2.2) + (A4.1) + (B3), (E3) + (A2.2) + (A4.2) + (B3);
    (E3) + (A3.1) + (A3.2) + (B3), (E3) + (A3.1) + (A4.1) + (B3), (E3) + (A3.1) + (A4.2) + (B3); (E3) + (A3.2) + (A4.1) + (B3), (E3) + (A3.2) + (A4.2) + (B3), (E3) + (A4.1) + (A4.2) + (B3);
    (E3.1) + (A1.1) + (B1), (E3.1) + (A1.1) + (B2), (E3.1) + (A1.1) + (B3), (E3.1) + (A2.1) + (B1), (E3.1) + (A2.1) + (B2), (E3.1) + (A2.1) + (B3), (E3.1) + (A3.1) + (B1), (E3.1) + (A3.1) + (B2), (E3.1) + (A3.1) + (B3), (E3.1) + (A4.1) + (B1), (E3.1) + (A4.1) + (B2), (E3.1) + (A4.1) + (B3), (E3.1) + (A1.2) + (B1), (E3.1) + (A1.2) + (B2), (E3.1) + (A1.2) + (B3), (E3.1) + (A2.2) + (B1), (E3.1) + (A2.2) + (B2), (E3.1) + (A2.2) + (B3), (E3.1) + (A3.2) + (B1), (E3.1) + (A3.2) + (B2), (E3.1) + (A3.2) + (B3), (E3.1) + (A4.2) + (B1), (E3.1) + (A4.2) + (B2), (E3.1) + (A4.2) + (B3),
    (E3.1) + (A1.1) + (A1.2) + (B1), (E3.1) + (A1.1) + (A2.1) + (B1), (E3.1) + (A1.1) + (A2.2) + (B1), (E3.1) + (A1.1) + (A3.1) + (B1), (E3.1) + (A1.1) + (A3.2) + (B1), (E3.1) + (A1.1) + (A4.1) + (B1), (E3.1) + (A1.1) + (A4.2) + (B1);
    (E3.1) + (A1.2) + (A2.1) + (B1), (E3.1) + (A1.2) + (A2.2) + (B1), (E3.1) + (A1.2) + (A3.1) + (B1), (E3.1) + (A1.2) + (A3.2) + (B1), (E3.1) + (A1.2) + (A4.1) + (B1), (E3.1) + (A1.2) + (A4.2) + (B1);
    (E3.1) + (A2.1) + (A2.2) + (B1), (E3.1) + (A2.1) + (A3.1) + (B1), (E3.1) + (A2.1) + (A3.2) + (B1), (E3.1) + (A2.1) + (A4.1) + (B1), (E3.1) + (A2.1) + (A4.2) + (B1);
    (E3.1) + (A2.2) + (A3.1) + (B1), (E3.1) + (A2.2) + (A3.2) + (B1), (E3.1) + (A2.2) + (A4.1) + (B1), (E3.1) + (A2.2) + (A4.2) + (B1);
    (E3.1) + (A3.1) + (A3.2) + (B1), (E3.1) + (A3.1) + (A4.1) + (B1), (E3.1) + (A3.1) + (A4.2) + (B1); (E3.1) + (A3.2) + (A4.1) + (B1), (E3.1) + (A3.2) + (A4.2) + (B1), (E3.1) + (A4.1) + (A4.2) + (B1);
    (E3.1) + (A1.1) + (A1.2) + (B2), (E3.1) + (A1.1) + (A2.1) + (B2), (E3.1) + (A1.1) + (A2.2) + (B2), (E3.1) + (A1.1) + (A3.1) + (B2), (E3.1) + (A1.1) + (A3.2) + (B2), (E3.1) + (A1.1) + (A4.1) + (B2), (E3.1) + (A1.1) + (A4.2) + (B2);
    (E3.1) + (A1.2) + (A2.1) + (B2), (E3.1) + (A1.2) + (A2.2) + (B2), (E3.1) + (A1.2) + (A3.1) + (B2), (E3.1) + (A1.2) + (A3.2) + (B2), (E3.1) + (A1.2) + (A4.1) + (B2), (E3.1) + (A1.2) + (A4.2) + (B2);
    (E3.1) + (A2.1) + (A2.2) + (B2), (E3.1) + (A2.1) + (A3.1) + (B2), (E3.1) + (A2.1) + (A3.2) + (B2), (E3.1) + (A2.1) + (A4.1) + (B2), (E3.1) + (A2.1) + (A4.2) + (B2);
    (E3.1) + (A2.2) + (A3.1) + (B2), (E3.1) + (A2.2) + (A3.2) + (B2), (E3.1) + (A2.2) + (A4.1) + (B2), (E3.1) + (A2.2) + (A4.2) + (B2);
    (E3.1) + (A3.1) + (A3.2) + (B2), (E3.1) + (A3.1) + (A4.1) + (B2), (E3.1) + (A3.1) + (A4.2) + (B2); (E3.1) + (A3.2) + (A4.1) + (B2), (E3.1) + (A3.2) + (A4.2) + (B2), (E3.1) + (A4.1) + (A4.2) + (B2);
    (E3.1) + (A1.1) + (A1.2) + (B3), (E3.1) + (A1.1) + (A2.1) + (B3), (E3.1) + (A1.1) + (A2.2) + (B3), (E3.1) + (A1.1) + (A3.1) + (B3), (E3.1) + (A1.1) + (A3.2) + (B3), (E3.1) + (A1.1) + (A4.1) + (B3), (E3.1) + (A1.1) + (A4.2) + (B3);
    (E3.1) + (A1.2) + (A2.1) + (B3), (E3.1) + (A1.2) + (A2.2) + (B3), (E3.1) + (A1.2) + (A3.1) + (B3), (E3.1) + (A1.2) + (A3.2) + (B3), (E3.1) + (A1.2) + (A4.1) + (B3), (E3.1) + (A1.2) + (A4.2) + (B3);
    (E3.1) + (A2.1) + (A2.2) + (B3), (E3.1) + (A2.1) + (A3.1) + (B3), (E3.1) + (A2.1) + (A3.2) + (B3), (E3.1) + (A2.1) + (A4.1) + (B3), (E3.1) + (A2.1) + (A4.2) + (B3); (E3.1) + (A2.2) + (A3.1) + (B3), (E3.1) + (A2.2) + (A3.2) + (B3), (E3.1) + (A2.2) + (A4.1) + (B3), (E3.1) + (A2.2) + (A4.2) + (B3);
    (E3.1) + (A3.1) + (A3.2) + (B3), (E3.1) + (A3.1) + (A4.1) + (B3), (E3.1) + (A3.1) + (A4.2) + (B3); (E3.1) + (A3.2) + (A4.1) + (B3), (E3.1) + (A3.2) + (A4.2) + (B3), (E3.1) + (A4.1) + (A4.2) + (B3);
    (E3.2) + (A1.1) + (B1), (E3.2) + (A1.1) + (B2), (E3.2) + (A1.1) + (B3), (E3.2) + (A2.1) + (B1), (E3.2) + (A2.1) + (B2), (E3.2) + (A2.1) + (B3), (E3.2) + (A3.1) + (B1), (E3.2) + (A3.1) + (B2), (E3.2) + (A3.1) + (B3), (E3.2) + (A4.1) + (B1), (E3.2) + (A4.1) + (B2), (E3.2) + (A4.1) + (B3), (E3.2) + (A1.2) + (B1), (E3.2) + (A1.2) + (B2), (E3.2) + (A1.2) + (B3), (E3.2) + (A2.2) + (B1), (E3.2) + (A2.2) + (B2), (E3.2) + (A2.2) + (B3), (E3.2) + (A3.2) + (B1), (E3.2) + (A3.2) + (B2), (E3.2) + (A3.2) + (B3), (E3.2) + (A4.2) + (B1), (E3.2) + (A4.2) + (B2), (E3.2) + (A4.2) + (B3),
    (E3.2) + (A1.1) + (A1.2) + (B1), (E3.2) + (A1.1) + (A2.1) + (B1), (E3.2) + (A1.1) + (A2.2) + (B1), (E3.2) + (A1.1) + (A3.1) + (B1), (E3.2) + (A1.1) + (A3.2) + (B1), (E3.2) + (A1.1) + (A4.1) + (B1), (E3.2) + (A1.1) + (A4.2) + (B1);
    (E3.2) + (A1.2) + (A2.1) + (B1), (E3.2) + (A1.2) + (A2.2) + (B1), (E3.2) + (A1.2) + (A3.1) + (B1), (E3.2) + (A1.2) + (A3.2) + (B1), (E3.2) + (A1.2) + (A4.1) + (B1), (E3.2) + (A1.2) + (A4.2) + (B1);
    (E3.2) + (A2.1) + (A2.2) + (B1), (E3.2) + (A2.1) + (A3.1) + (B1), (E3.2) + (A2.1) + (A3.2) + (B1), (E3.2) + (A2.1) + (A4.1) + (B1), (E3.2) + (A2.1) + (A4.2) + (B1); (E3.2) + (A2.2) + (A3.1) + (B1), (E3.2) + (A2.2) + (A3.2) + (B1), (E3.2) + (A2.2) + (A4.1) + (B1), (E3.2) + (A2.2) + (A4.2) + (B1);
    (E3.2) + (A3.1) + (A3.2) + (B1), (E3.2) + (A3.1) + (A4.1) + (B1), (E3.2) + (A3.1) + (A4.2) + (B1); (E3.2) + (A3.2) + (A4.1) + (B1), (E3.2) + (A3.2) + (A4.2) + (B1), (E3.2) + (A4.1) + (A4.2) + (B1);
    (E3.2) + (A1.1) + (A1.2) + (B2), (E3.2) + (A1.1) + (A2.1) + (B2), (E3.2) + (A1.1) + (A2.2) + (B2), (E3.2) + (A1.1) + (A3.1) + (B2), (E3.2) + (A1.1) + (A3.2) + (B2), (E3.2) + (A1.1) + (A4.1) + (B2), (E3.2) + (A1.1) + (A4.2) + (B2);
    (E3.2) + (A1.2) + (A2.1) + (B2), (E3.2) + (A1.2) + (A2.2) + (B2), (E3.2) + (A1.2) + (A3.1) + (B2), (E3.2) + (A1.2) + (A3.2) + (B2), (E3.2) + (A1.2) + (A4.1) + (B2), (E3.2) + (A1.2) + (A4.2) + (B2);
    (E3.2) + (A2.1) + (A2.2) + (B2), (E3.2) + (A2.1) + (A3.1) + (B2), (E3.2) + (A2.1) + (A3.2) + (B2), (E3.2) + (A2.1) + (A4.1) + (B2), (E3.2) + (A2.1) + (A4.2) + (B2);
    (E3.2) + (A2.2) + (A3.1) + (B2), (E3.2) + (A2.2) + (A3.2) + (B2), (E3.2) + (A2.2) + (A4.1) + (B2), (E3.2) + (A2.2) + (A4.2) + (B2);
    (E3.2) + (A3.1) + (A3.2) + (B2), (E3.2) + (A3.1) + (A4.1) + (B2), (E3.2) + (A3.1) + (A4.2) + (B2); (E3.2) + (A3.2) + (A4.1) + (B2), (E3.2) + (A3.2) + (A4.2) + (B2), (E3.2) + (A4.1) + (A4.2) + (B2);
    (E3.2) + (A1.1) + (A1.2) + (B3), (E3.2) + (A1.1) + (A2.1) + (B3), (E3.2) + (A1.1) + (A2.2) + (B3), (E3.2) + (A1.1) + (A3.1) + (B3), (E3.2) + (A1.1) + (A3.2) + (B3), (E3.2) + (A1.1) + (A4.1) + (B3), (E3.2) + (A1.1) + (A4.2) + (B3);
    (E3.2) + (A1.2) + (A2.1) + (B3), (E3.2) + (A1.2) + (A2.2) + (B3), (E3.2) + (A1.2) + (A3.1) + (B3), (E3.2) + (A1.2) + (A3.2) + (B3), (E3.2) + (A1.2) + (A4.1) + (B3), (E3.2) + (A1.2) + (A4.2) + (B3);
    (E3.2) + (A2.1) + (A2.2) + (B3), (E3.2) + (A2.1) + (A3.1) + (B3), (E3.2) + (A2.1) + (A3.2) + (B3), (E3.2) + (A2.1) + (A4.1) + (B3), (E3.2) + (A2.1) + (A4.2) + (B3);
    (E3.2) + (A2.2) + (A3.1) + (B3), (E3.2) + (A2.2) + (A3.2) + (B3), (E3.2) + (A2.2) + (A4.1) + (B3), (E3.2) + (A2.2) + (A4.2) + (B3);
    (E3.2) + (A3.1) + (A3.2) + (B3), (E3.2) + (A3.1) + (A4.1) + (B3), (E3.2) + (A3.1) + (A4.2) + (B3); (E3.2) + (A3.2) + (A4.1) + (B3), (E3.2) + (A3.2) + (A4.2) + (B3), (E3.2) + (A4.1) + (A4.2) + (B3);
    (E3.3) + (A1.1) + (B1), (E3.3) + (A1.1) + (B2), (E3.3) + (A1.1) + (B3), (E3.3) + (A2.1) + (B1), (E3.3) + (A2.1) + (B2), (E3.3) + (A2.1) + (B3), (E3.3) + (A3.1) + (B1), (E3.3) + (A3.1) + (B2), (E3.3) + (A3.1) + (B3), (E3.3) + (A4.1) + (B1), (E3.3) + (A4.1) + (B2), (E3.3) + (A4.1) + (B3), (E3.3) + (A1.2) + (B1), (E3.3) + (A1.2) + (B2), (E3.3) + (A1.2) + (B3), (E3.3) + (A2.2) + (B1), (E3.3) + (A2.2) + (B2), (E3.3) + (A2.2) + (B3), (E3.3) + (A3.2) + (B1), (E3.3) + (A3.2) + (B2), (E3.3) + (A3.2) + (B3), (E3.3) + (A4.2) + (B1), (E3.3) + (A4.2) + (B2), (E3.3) + (A4.2) + (B3),
    (E3.3) + (A1.1) + (A1.2) + (B1), (E3.3) + (A1.1) + (A2.1) + (B1), (E3.3) + (A1.1) + (A2.2) + (B1), (E3.3) + (A1.1) + (A3.1) + (B1), (E3.3) + (A1.1) + (A3.2) + (B1), (E3.3) + (A1.1) + (A4.1) + (B1), (E3.3) + (A1.1) + (A4.2) + (B1);
    (E3.3) + (A1.2) + (A2.1) + (B1), (E3.3) + (A1.2) + (A2.2) + (B1), (E3.3) + (A1.2) + (A3.1) + (B1), (E3.3) + (A1.2) + (A3.2) + (B1), (E3.3) + (A1.2) + (A4.1) + (B1), (E3.3) + (A1.2) + (A4.2) + (B1);
    (E3.3) + (A2.1) + (A2.2) + (B1), (E3.3) + (A2.1) + (A3.1) + (B1), (E3.3) + (A2.1) + (A3.2) + (B1), (E3.3) + (A2.1) + (A4.1) + (B1), (E3.3) + (A2.1) + (A4.2) + (B1);
    (E3.3) + (A2.2) + (A3.1) + (B1), (E3.3) + (A2.2) + (A3.2) + (B1), (E3.3) + (A2.2) + (A4.1) + (B1), (E3.3) + (A2.2) + (A4.2) + (B1);
    (E3.3) + (A3.1) + (A3.2) + (B1), (E3.3) + (A3.1) + (A4.1) + (B1), (E3.3) + (A3.1) + (A4.2) + (B1); (E3.3) + (A3.2) + (A4.1) + (B1), (E3.3) + (A3.2) + (A4.2) + (B1), (E3.3) + (A4.1) + (A4.2) + (B1);
    (E3.3) + (A1.1) + (A1.2) + (B2), (E3.3) + (A1.1) + (A2.1) + (B2), (E3.3) + (A1.1) + (A2.2) + (B2), (E3.3) + (A1.1) + (A3.1) + (B2), (E3.3) + (A1.1) + (A3.2) + (B2), (E3.3) + (A1.1) + (A4.1) + (B2), (E3.3) + (A1.1) + (A4.2) + (B2);
    (E3.3) + (A1.2) + (A2.1) + (B2), (E3.3) + (A1.2) + (A2.2) + (B2), (E3.3) + (A1.2) + (A3.1) + (B2), (E3.3) + (A1.2) + (A3.2) + (B2), (E3.3) + (A1.2) + (A4.1) + (B2), (E3.3) + (A1.2) + (A4.2) + (B2);
    (E3.3) + (A2.1) + (A2.2) + (B2), (E3.3) + (A2.1) + (A3.1) + (B2), (E3.3) + (A2.1) + (A3.2) + (B2), (E3.3) + (A2.1) + (A4.1) + (B2), (E3.3) + (A2.1) + (A4.2) + (B2);
    (E3.3) + (A2.2) + (A3.1) + (B2), (E3.3) + (A2.2) + (A3.2) + (B2), (E3.3) + (A2.2) + (A4.1) + (B2), (E3.3) + (A2.2) + (A4.2) + (B2);
    (E3.3) + (A3.1) + (A3.2) + (B2), (E3.3) + (A3.1) + (A4.1) + (B2), (E3.3) + (A3.1) + (A4.2) + (B2); (E3.3) + (A3.2) + (A4.1) + (B2), (E3.3) + (A3.2) + (A4.2) + (B2), (E3.3) + (A4.1) + (A4.2) + (B2);
    (E3.3) + (A1.1) + (A1.2) + (B3), (E3.3) + (A1.1) + (A2.1) + (B3), (E3.3) + (A1.1) + (A2.2) + (B3), (E3.3) + (A1.1) + (A3.1) + (B3), (E3.3) + (A1.1) + (A3.2) + (B3), (E3.3) + (A1.1) + (A4.1) + (B3), (E3.3) + (A1.1) + (A4.2) + (B3);
    (E3.3) + (A1.2) + (A2.1) + (B3), (E3.3) + (A1.2) + (A2.2) + (B3), (E3.3) + (A1.2) + (A3.1) + (B3), (E3.3) + (A1.2) + (A3.2) + (B3), (E3.3) + (A1.2) + (A4.1) + (B3), (E3.3) + (A1.2) + (A4.2) + (B3);
    (E3.3) + (A2.1) + (A2.2) + (B3), (E3.3) + (A2.1) + (A3.1) + (B3), (E3.3) + (A2.1) + (A3.2) + (B3), (E3.3) + (A2.1) + (A4.1) + (B3), (E3.3) + (A2.1) + (A4.2) + (B3);
    (E3.3) + (A2.2) + (A3.1) + (B3), (E3.3) + (A2.2) + (A3.2) + (B3), (E3.3) + (A2.2) + (A4.1) + (B3), (E3.3) + (A2.2) + (A4.2) + (B3);
    (E3.3) + (A3.1) + (A3.2) + (B3), (E3.3) + (A3.1) + (A4.1) + (B3), (E3.3) + (A3.1) + (A4.2) + (B3); (E3.3) + (A3.2) + (A4.1) + (B3), (E3.3) + (A3.2) + (A4.2) + (B3), (E3.3) + (A4.1) + (A4.2) + (B3);
    (E4) + (A1.1) + (B1), (E4) + (A1.1) + (B2), (E4) + (A1.1) + (B3), (E4) + (A2.1) + (B1), (E4) + (A2.1) + (B2), (E4) + (A2.1) + (B3), (E4) + (A3.1) + (B1), (E4) + (A3.1) + (B2), (E4) + (A3.1) + (B3), (E4) + (A4.1) + (B1), (E4) + (A4.1) + (B2), (E4) + (A4.1) + (B3), (E4) + (A1.2) + (B1), (E4) + (A1.2) + (B2), (E4) + (A1.2) + (B3), (E4) + (A2.2) + (B1), (E4) + (A2.2) + (B2), (E4) + (A2.2) + (B3), (E4) + (A3.2) + (B1), (E4) + (A3.2) + (B2), (E4) + (A3.2) + (B3), (E4) + (A4.2) + (B1), (E4) + (A4.2) + (B2), (E4) + (A4.2) + (B3), (E4) + (A1.1) + (A1.2) + (B1), (E4) + (A1.1) + (A2.1) + (B1), (E4) + (A1.1) + (A2.2) + (B1), (E4) + (A1.1) + (A3.1) + (B1), (E4) + (A1.1) + (A3.2) + (B1), (E4) + (A1.1) + (A4.1) + (B1), (E4) + (A1.1) + (A4.2) + (B1);
    (E4) + (A1.2) + (A2.1) + (B1), (E4) + (A1.2) + (A2.2) + (B1), (E4) + (A1.2) + (A3.1) + (B1), (E4) + (A1.2) + (A3.2) + (B1), (E4) + (A1.2) + (A4.1) + (B1), (E4) + (A1.2) + (A4.2) + (B1);
    (E4) + (A2.1) + (A2.2) + (B1), (E4) + (A2.1) + (A3.1) + (B1), (E4) + (A2.1) + (A3.2) + (B1), (E4) + (A2.1) + (A4.1) + (B1), (E4) + (A2.1) + (A4.2) + (B1);
    (E4) + (A2.2) + (A3.1) + (B1), (E4) + (A2.2) + (A3.2) + (B1), (E4) + (A2.2) + (A4.1) + (B1), (E4) + (A2.2) + (A4.2) + (B1);
    (E4) + (A3.1) + (A3.2) + (B1), (E4) + (A3.1) + (A4.1) + (B1), (E4) + (A3.1) + (A4.2) + (B1); (E4) + (A3.2) + (A4.1) + (B1), (E4) + (A3.2) + (A4.2) + (B1), (E4) + (A4.1) + (A4.2) + (B1);
    (E4) + (A1.1) + (A1.2) + (B2), (E4) + (A1.1) + (A2.1) + (B2), (E4) + (A1.1) + (A2.2) + (B2), (E4) + (A1.1) + (A3.1) + (B2), (E4) + (A1.1) + (A3.2) + (B2), (E4) + (A1.1) + (A4.1) + (B2), (E4) + (A1.1) + (A4.2) + (B2);
    (E4) + (A1.2) + (A2.1) + (B2), (E4) + (A1.2) + (A2.2) + (B2), (E4) + (A1.2) + (A3.1) + (B2), (E4) + (A1.2) + (A3.2) + (B2), (E4) + (A1.2) + (A4.1) + (B2), (E4) + (A1.2) + (A4.2) + (B2);
    (E4) + (A2.1) + (A2.2) + (B2), (E4) + (A2.1) + (A3.1) + (B2), (E4) + (A2.1) + (A3.2) + (B2), (E4) + (A2.1) + (A4.1) + (B2), (E4) + (A2.1) + (A4.2) + (B2); (E4) + (A2.2) + (A3.1) + (B2), (E4) + (A2.2) + (A3.2) + (B2), (E4) + (A2.2) + (A4.1) + (B2), (E4) + (A2.2) + (A4.2) + (B2);
    (E4) + (A3.1) + (A3.2) + (B2), (E4) + (A3.1) + (A4.1) + (B2), (E4) + (A3.1) + (A4.2) + (B2); (E4) + (A3.2) + (A4.1) + (B2), (E4) + (A3.2) + (A4.2) + (B2), (E4) + (A4.1) + (A4.2) + (B2);
    (E4) + (A1.1) + (A1.2) + (B3), (E4) + (A1.1) + (A2.1) + (B3), (E4) + (A1.1) + (A2.2) + (B3), (E4) + (A1.1) + (A3.1) + (B3), (E4) + (A1.1) + (A3.2) + (B3), (E4) + (A1.1) + (A4.1) + (B3), (E4) + (A1.1) + (A4.2) + (B3);
    (E4) + (A1.2) + (A2.1) + (B3), (E4) + (A1.2) + (A2.2) + (B3), (E4) + (A1.2) + (A3.1) + (B3), (E4) + (A1.2) + (A3.2) + (B3), (E4) + (A1.2) + (A4.1) + (B3), (E4) + (A1.2) + (A4.2) + (B3); (E4) + (A2.1) + (A2.2) + (B3), (E4) + (A2.1) + (A3.1) + (B3), (E4) + (A2.1) + (A3.2) + (B3), (E4) + (A2.1) + (A4.1) + (B3), (E4) + (A2.1) + (A4.2) + (B3);
    (E4) + (A2.2) + (A3.1) + (B3), (E4) + (A2.2) + (A3.2) + (B3), (E4) + (A2.2) + (A4.1) + (B3), (E4) + (A2.2) + (A4.2) + (B3);
    (E4) + (A3.1) + (A3.2) + (B3), (E4) + (A3.1) + (A4.1) + (B3), (E4) + (A3.1) + (A4.2) + (B3); (E4) + (A3.2) + (A4.1) + (B3), (E4) + (A3.2) + (A4.2) + (B3), (E4) + (A4.1) + (A4.2) + (B3);
    (E4.1) + (A1.1) + (B1), (E4.1) + (A1.1) + (B2), (E4.1) + (A1.1) + (B3), (E4.1) + (A2.1) + (B1), (E4.1) + (A2.1) + (B2), (E4.1) + (A2.1) + (B3), (E4.1) + (A3.1) + (B1), (E4.1) + (A3.1) + (B2), (E4.1) + (A3.1) + (B3), (E4.1) + (A4.1) + (B1), (E4.1) + (A4.1) + (B2), (E4.1) + (A4.1) + (B3), (E4.1) + (A1.2) + (B1), (E4.1) + (A1.2) + (B2), (E4.1) + (A1.2) + (B3), (E4.1) + (A2.2) + (B1), (E4.1) + (A2.2) + (B2), (E4.1) + (A2.2) + (B3), (E4.1) + (A3.2) + (B1), (E4.1) + (A3.2) + (B2), (E4.1) + (A3.2) + (B3), (E4.1) + (A4.2) + (B1), (E4.1) + (A4.2) + (B2), (E4.1) + (A4.2) + (B3),
    (E4.1) + (A1.1) + (A1.2) + (B1), (E4.1) + (A1.1) + (A2.1) + (B1), (E4.1) + (A1.1) + (A2.2) + (B1), (E4.1) + (A1.1) + (A3.1) + (B1), (E4.1) + (A1.1) + (A3.2) + (B1), (E4.1) + (A1.1) + (A4.1) + (B1), (E4.1) + (A1.1) + (A4.2) + (B1);
    (E4.1) + (A1.2) + (A2.1) + (B1), (E4.1) + (A1.2) + (A2.2) + (B1), (E4.1) + (A1.2) + (A3.1) + (B1), (E4.1) + (A1.2) + (A3.2) + (B1), (E4.1) + (A1.2) + (A4.1) + (B1), (E4.1) + (A1.2) + (A4.2) + (B1);
    (E4.1) + (A2.1) + (A2.2) + (B1), (E4.1) + (A2.1) + (A3.1) + (B1), (E4.1) + (A2.1) + (A3.2) + (B1), (E4.1) + (A2.1) + (A4.1) + (B1), (E4.1) + (A2.1) + (A4.2) + (B1);
    (E4.1) + (A2.2) + (A3.1) + (B1), (E4.1) + (A2.2) + (A3.2) + (B1), (E4.1) + (A2.2) + (A4.1) + (B1), (E4.1) + (A2.2) + (A4.2) + (B1);
    (E4.1) + (A3.1) + (A3.2) + (B1), (E4.1) + (A3.1) + (A4.1) + (B1), (E4.1) + (A3.1) + (A4.2) + (B1); (E4.1) + (A3.2) + (A4.1) + (B1), (E4.1) + (A3.2) + (A4.2) + (B1), (E4.1) + (A4.1) + (A4.2) + (B1);
    (E4.1) + (A1.1) + (A1.2) + (B2), (E4.1) + (A1.1) + (A2.1) + (B2), (E4.1) + (A1.1) + (A2.2) + (B2), (E4.1) + (A1.1) + (A3.1) + (B2), (E4.1) + (A1.1) + (A3.2) + (B2), (E4.1) + (A1.1) + (A4.1) + (B2), (E4.1) + (A1.1) + (A4.2) + (B2);
    (E4.1) + (A1.2) + (A2.1) + (B2), (E4.1) + (A1.2) + (A2.2) + (B2), (E4.1) + (A1.2) + (A3.1) + (B2), (E4.1) + (A1.2) + (A3.2) + (B2), (E4.1) + (A1.2) + (A4.1) + (B2), (E4.1) + (A1.2) + (A4.2) + (B2);
    (E4.1) + (A2.1) + (A2.2) + (B2), (E4.1) + (A2.1) + (A3.1) + (B2), (E4.1) + (A2.1) + (A3.2) + (B2), (E4.1) + (A2.1) + (A4.1) + (B2), (E4.1) + (A2.1) + (A4.2) + (B2);
    (E4.1) + (A2.2) + (A3.1) + (B2), (E4.1) + (A2.2) + (A3.2) + (B2), (E4.1) + (A2.2) + (A4.1) + (B2), (E4.1) + (A2.2) + (A4.2) + (B2);
    (E4.1) + (A3.1) + (A3.2) + (B2), (E4.1) + (A3.1) + (A4.1) + (B2), (E4.1) + (A3.1) + (A4.2) + (B2); (E4.1) + (A3.2) + (A4.1) + (B2), (E4.1) + (A3.2) + (A4.2) + (B2), (E4.1) + (A4.1) + (A4.2) + (B2);
    (E4.1) + (A1.1) + (A1.2) + (B3), (E4.1) + (A1.1) + (A2.1) + (B3), (E4.1) + (A1.1) + (A2.2) + (B3), (E4.1) + (A1.1) + (A3.1) + (B3), (E4.1) + (A1.1) + (A3.2) + (B3), (E4.1) + (A1.1) + (A4.1) + (B3), (E4.1) + (A1.1) + (A4.2) + (B3);
    (E4.1) + (A1.2) + (A2.1) + (B3), (E4.1) + (A1.2) + (A2.2) + (B3), (E4.1) + (A1.2) + (A3.1) + (B3), (E4.1) + (A1.2) + (A3.2) + (B3), (E4.1) + (A1.2) + (A4.1) + (B3), (E4.1) + (A1.2) + (A4.2) + (B3);
    (E4.1) + (A2.1) + (A2.2) + (B3), (E4.1) + (A2.1) + (A3.1) + (B3), (E4.1) + (A2.1) + (A3.2) + (B3), (E4.1) + (A2.1) + (A4.1) + (B3), (E4.1) + (A2.1) + (A4.2) + (B3);
    (E4.1) + (A2.2) + (A3.1) + (B3), (E4.1) + (A2.2) + (A3.2) + (B3), (E4.1) + (A2.2) + (A4.1) + (B3), (E4.1) + (A2.2) + (A4.2) + (B3);
    (E4.1) + (A3.1) + (A3.2) + (B3), (E4.1) + (A3.1) + (A4.1) + (B3), (E4.1) + (A3.1) + (A4.2) + (B3); (E4.1) + (A3.2) + (A4.1) + (B3), (E4.1) + (A3.2) + (A4.2) + (B3), (E4.1) + (A4.1) + (A4.2) + (B3);
    (E4.2) + (A1.1) + (B1), (E4.2) + (A1.1) + (B2), (E4.2) + (A1.1) + (B3), (E4.2) + (A2.1) + (B1), (E4.2) + (A2.1) + (B2), (E4.2) + (A2.1) + (B3), (E4.2) + (A3.1) + (B1), (E4.2) + (A3.1) + (B2), (E4.2) + (A3.1) + (B3), (E4.2) + (A4.1) + (B1), (E4.2) + (A4.1) + (B2), (E4.2) + (A4.1) + (B3), (E4.2) + (A1.2) + (B 1), (E4.2) + (A1.2) + (B2), (E4.2) + (A1.2) + (B3), (E4.2) + (A2.2) + (B1), (E4.2) + (A2.2) + (B2), (E4.2) + (A2.2) + (B3), (E4.2) + (A3.2) + (B1), (E4.2) + (A3.2) + (B2), (E4.2) + (A3.2) + (B3), (E4.2) + (A4.2) + (B1), (E4.2) + (A4.2) + (B2), (E4.2) + (A4.2) + (B3),
    (E4.2) + (A1.1) + (A1.2) + (B1), (E4.2) + (A1.1) + (A2.1) + (B1), (E4.2) + (A1.1) + (A2.2) + (B1), (E4.2) + (A1.1) + (A3.1) + (B1), (E4.2) + (A1.1) + (A3.2) + (B1), (E4.2) + (A1.1) + (A4.1) + (B1), (E4.2) + (A1.1) + (A4.2) + (B1);
    (E4.2) + (A1.2) + (A2.1) + (B1), (E4.2) + (A1.2) + (A2.2) + (B1), (E4.2) + (A1.2) + (A3.1) + (B1), (E4.2) + (A1.2) + (A3.2) + (B1), (E4.2) + (A1.2) + (A4.1) + (B1), (E4.2) + (A1.2) + (A4.2) + (B1);
    (E4.2) + (A2.1) + (A2.2) + (B1), (E4.2) + (A2.1) + (A3.1) + (B1), (E4.2) + (A2.1) + (A3.2) + (B1), (E4.2) + (A2.1) + (A4.1) + (B1), (E4.2) + (A2.1) + (A4.2) + (B1);
    (E4.2) + (A2.2) + (A3.1) + (B1), (E4.2) + (A2.2) + (A3.2) + (B1), (E4.2) + (A2.2) + (A4.1) + (B1), (E4.2) + (A2.2) + (A4.2) + (B1);
    (E4.2) + (A3.1) + (A3.2) + (B1), (E4.2) + (A3.1) + (A4.1) + (B1), (E4.2) + (A3.1) + (A4.2) + (B1); (E4.2) + (A3.2) + (A4.1) + (B1), (E4.2) + (A3.2) + (A4.2) + (B1), (E4.2) + (A4.1) + (A4.2) + (B1);
    (E4.2) + (A1.1) + (A1.2) + (B2), (E4.2) + (A1.1) + (A2.1) + (B2), (E4.2) + (A1.1) + (A2.2) + (B2), (E4.2) + (A1.1) + (A3.1) + (B2), (E4.2) + (A1.1) + (A3.2) + (B2), (E4.2) + (A1.1) + (A4.1) + (B2), (E4.2) + (A1.1) + (A4.2) + (B2);
    (E4.2) + (A1.2) + (A2.1) + (B2), (E4.2) + (A1.2) + (A2.2) + (B2), (E4.2) + (A1.2) + (A3.1) + (B2), (E4.2) + (A1.2) + (A3.2) + (B2), (E4.2) + (A1.2) + (A4.1) + (B2), (E4.2) + (A1.2) + (A4.2) + (B2);
    (E4.2) + (A2.1) + (A2.2) + (B2), (E4.2) + (A2.1) + (A3.1) + (B2), (E4.2) + (A2.1) + (A3.2) + (B2), (E4.2) + (A2.1) + (A4.1) + (B2), (E4.2) + (A2.1) + (A4.2) + (B2);
    (E4.2) + (A2.2) + (A3.1) + (B2), (E4.2) + (A2.2) + (A3.2) + (B2), (E4.2) + (A2.2) + (A4.1) + (B2), (E4.2) + (A2.2) + (A4.2) + (B2);
    (E4.2) + (A3.1) + (A3.2) + (B2), (E4.2) + (A3.1) + (A4.1) + (B2), (E4.2) + (A3.1) + (A4.2) + (B2); (E4.2) + (A3.2) + (A4.1) + (B2), (E4.2) + (A3.2) + (A4.2) + (B2), (E4.2) + (A4.1) + (A4.2) + (B2);
    (E4.2) + (A1.1) + (A1.2) + (B3), (E4.2) + (A1.1) + (A2.1) + (B3), (E4.2) + (A1.1) + (A2.2) + (B3), (E4.2) + (A1.1) + (A3.1) + (B3), (E4.2) + (A1.1) + (A3.2) + (B3), (E4.2) + (A1.1) + (A4.1) + (B3), (E4.2) + (A1.1) + (A4.2) + (B3);
    (E4.2) + (A1.2) + (A2.1) + (B3), (E4.2) + (A1.2) + (A2.2) + (B3), (E4.2) + (A1.2) + (A3.1) + (B3), (E4.2) + (A1.2) + (A3.2) + (B3), (E4.2) + (A1.2) + (A4.1) + (B3), (E4.2) + (A1.2) + (A4.2) + (B3);
    (E4.2) + (A2.1) + (A2.2) + (B3), (E4.2) + (A2.1) + (A3.1) + (B3), (E4.2) + (A2.1) + (A3.2) + (B3), (E4.2) + (A2.1) + (A4.1) + (B3), (E4.2) + (A2.1) + (A4.2) + (B3);
    (E4.2) + (A2.2) + (A3.1) + (B3), (E4.2) + (A2.2) + (A3.2) + (B3), (E4.2) + (A2.2) + (A4.1) + (B3), (E4.2) + (A2.2) + (A4.2) + (B3);
    (E4.2) + (A3.1) + (A3.2) + (B3), (E4.2) + (A3.1) + (A4.1) + (B3), (E4.2) + (A3.1) + (A4.2) + (B3); (E4.2) + (A3.2) + (A4.1) + (B3), (E4.2) + (A3.2) + (A4.2) + (B3), (E4.2) + (A4.1) + (A4.2) + (B3);
    (E5) + (A1.1) + (B1), (E5) + (A1.1) + (B2), (E5) + (A1.1) + (B3), (E5) + (A2.1) + (B1), (E5) + (A2.1) + (B2), (E5) + (A2.1) + (B3), (E5) + (A3.1) + (B1), (E5) + (A3.1) + (B2), (E5) + (A3.1) + (B3), (E5) + (A4.1) + (B1), (E5) + (A4.1) + (B2), (E5) + (A4.1) + (B3), (E5) + (A1.2) + (B1), (E5) + (A1.2) + (B2), (E5) + (A1.2) + (B3), (E5) + (A2.2) + (B1), (E5) + (A2.2) + (B2), (E5) + (A2.2) + (B3), (E5) + (A3.2) + (B1), (E5) + (A3.2) + (B2), (E5) + (A3.2) + (B3), (E5) + (A4.2) + (B1), (E5) + (A4.2) + (B2), (E5) + (A4.2) + (B3), (E5) + (A1.1) + (A1.2) + (B1), (E5) + (A1.1) + (A2.1) + (B1), (E5) + (A1.1) + (A2.2) + (B1), (E5) + (A1.1) + (A3.1) + (B1), (E5) + (A1.1) + (A3.2) + (B1), (E5) + (A1.1) + (A4.1) + (B1), (E5) + (A1.1) + (A4.2) + (B1);
    (E5) + (A1.2) + (A2.1) + (B1), (E5) + (A1.2) + (A2.2) + (B1), (E5) + (A1.2) + (A3.1) + (B1), (E5) + (A1.2) + (A3.2) + (B1), (E5) + (A1.2) + (A4.1) + (B1), (E5) + (A1.2) + (A4.2) + (B1);
    (E5) + (A2.1) + (A2.2) + (B1), (E5) + (A2.1) + (A3.1) + (B1), (E5) + (A2.1) + (A3.2) + (B1), (E5) + (A2.1) + (A4.1) + (B1), (E5) + (A2.1) + (A4.2) + (B1);
    (E5) + (A2.2) + (A3.1) + (B1), (E5) + (A2.2) + (A3.2) + (B1), (E5) + (A2.2) + (A4.1) + (B1), (E5) + (A2.2) + (A4.2) + (B1);
    (E5) + (A3.1) + (A3.2) + (B1), (E5) + (A3.1) + (A4.1) + (B1), (E5) + (A3.1) + (A4.2) + (B1), (E5) + (A3.2) + (A4.1) + (B1), (E5) + (A3.2) + (A4.2) + (B1), (E5) + (A4.1) + (A4.2) + (B1);
    (E5) + (A1.1) + (A1.2) + (B2), (E5) + (A1.1) + (A2.1) + (B2), (E5) + (A1.1) + (A2.2) + (B2), (E5) + (A1.1) + (A3.1) + (B2), (E5) + (A1.1) + (A3.2) + (B2), (E5) + (A1.1) + (A4.1) + (B2), (E5) + (A1.1) + (A4.2) + (B2);
    (E5) + (A1.2) + (A2.1) + (B2), (E5) + (A1.2) + (A2.2) + (B2), (E5) + (A1.2) + (A3.1) + (B2), (E5) + (A1.2) + (A3.2) + (B2), (E5) + (A1.2) + (A4.1) + (B2), (E5) + (A1.2) + (A4.2) + (B2);
    (E5) + (A2.1) + (A2.2) + (B2), (E5) + (A2.1) + (A3.1) + (B2), (E5) + (A2.1) + (A3.2) + (B2), (E5) + (A2.1) + (A4.1) + (B2), (E5) + (A2.1) + (A4.2) + (B2);
    (E5) + (A2.2) + (A3.1) + (B2), (E5) + (A2.2) + (A3.2) + (B2), (E5) + (A2.2) + (A4.1) + (B2), (E5) + (A2.2) + (A4.2) + (B2);
    (E5) + (A3.1) + (A3.2) + (B2), (E5) + (A3.1) + (A4.1) + (B2), (E5) + (A3.1) + (A4.2) + (B2); (E5) + (A3.2) + (A4.1) + (B2), (E5) + (A3.2) + (A4.2) + (B2), (E5) + (A4.1) + (A4.2) + (B2);
    (E5) + (A1.1) + (A1.2) + (B3), (E5) + (A1.1) + (A2.1) + (B3), (E5) + (A1.1) + (A2.2) + (B3), (E5) + (A1.1) + (A3.1) + (B3), (E5) + (A1.1) + (A3.2) + (B3), (E5) + (A1.1) + (A4.1) + (B3), (E5) + (A1.1) + (A4.2) + (B3);
    (E5) + (A1.2) + (A2.1) + (B3), (E5) + (A1.2) + (A2.2) + (B3), (E5) + (A1.2) + (A3.1) + (B3), (E5) + (A1.2) + (A3.2) + (B3), (E5) + (A1.2) + (A4.1) + (B3), (E5) + (A1.2) + (A4.2) + (B3);
    (E5) + (A2.1) + (A2.2) + (B3), (E5) + (A2.1) + (A3.1) + (B3), (E5) + (A2.1) + (A3.2) + (B3), (E5) + (A2.1) + (A4.1) + (B3), (E5) + (A2.1) + (A4.2) + (B3); (E5) + (A2.2) + (A3.1) + (B3), (E5) + (A2.2) + (A3.2) + (B3), (E5) + (A2.2) + (A4.1) + (B3), (E5) + (A2.2) + (A4.2) + (B3);
    (E5) + (A3.1) + (A3.2) + (B3), (E5) + (A3.1) + (A4.1) + (B3), (E5) + (A3.1) + (A4.2) + (B3); (E5) + (A3.2) + (A4.1) + (B3), (E5) + (A3.2) + (A4.2) + (B3), (E5) + (A4.1) + (A4.2) + (B3);
    (E5.1) + (A1.1) + (B1), (E5.1) + (A1.1) + (B2), (E5.1) + (A1.1) + (B3), (E5.1) + (A2.1) + (B1), (E5.1) + (A2.1) + (B2), (E5.1) + (A2.1) + (B3), (E5.1) + (A3.1) + (B1), (E5.1) + (A3.1) + (B2), (E5.1) + (A3.1) + (B3), (E5.1) + (A4.1) + (B1), (E5.1) + (A4.1) + (B2), (E5.1) + (A4.1) + (B3), (E5.1) + (A1.2) + (B1), (E5.1) + (A1.2) + (B2), (E5.1) + (A1.2) + (B3), (E5.1) + (A2.2) + (B1), (E5.1) + (A2.2) + (B2), (E5.1) + (A2.2) + (B3), (E5.1) + (A3.2) + (B1), (E5.1) + (A3.2) + (B2), (E5.1) + (A3.2) + (B3), (E5.1) + (A4.2) + (B1), (E5.1) + (A4.2) + (B2), (E5.1) + (A4.2) + (B3),
    (E5.1) + (A1.1) + (A1.2) + (B1), (E5.1) + (A1.1) + (A2.1) + (B1), (E5.1) + (A1.1) + (A2.2) + (B1), (E5.1) + (A1.1) + (A3.1) + (B1), (E5.1) + (A1.1) + (A3.2) + (B1), (E5.1) + (A1.1) + (A4.1) + (B1), (E5.1) + (A1.1) + (A4.2) + (B1);
    (E5.1) + (A1.2) + (A2.1) + (B1), (E5.1) + (A1.2) + (A2.2) + (B1), (E5.1) + (A1.2) + (A3.1) + (B1), (E5.1) + (A1.2) + (A3.2) + (B1), (E5.1) + (A1.2) + (A4.1) + (B1), (E5.1) + (A1.2) + (A4.2) + (B1);
    (E5.1) + (A2.1) + (A2.2) + (B1), (E5.1) + (A2.1) + (A3.1) + (B1), (E5.1) + (A2.1) + (A3.2) + (B1), (E5.1) + (A2.1) + (A4.1) + (B1), (E5.1) + (A2.1) + (A4.2) + (B1);
    (E5.1) + (A2.2) + (A3.1) + (B1), (E5.1) + (A2.2) + (A3.2) + (B1), (E5.1) + (A2.2) + (A4.1) + (B1), (E5.1) + (A2.2) + (A4.2) + (B1);
    (E5.1) + (A3.1) + (A3.2) + (B1), (E5.1) + (A3.1) + (A4.1) + (B1), (E5.1) + (A3.1) + (A4.2) + (B1); (E5.1) + (A3.2) + (A4.1) + (B1), (E5.1) + (A3.2) + (A4.2) + (B1), (E5.1) + (A4.1) + (A4.2) + (B1);
    (E5.1) + (A1.1) + (A1.2) + (B2), (E5.1) + (A1.1) + (A2.1) + (B2), (E5.1) + (A1.1) + (A2.2) + (B2), (E5.1) + (A1.1) + (A3.1) + (B2), (E5.1) + (A1.1) + (A3.2) + (B2), (E5.1) + (A1.1) + (A4.1) + (B2), (E5.1) + (A1.1) + (A4.2) + (B2);
    (E5.1) + (A1.2) + (A2.1) + (B2), (E5.1) + (A1.2) + (A2.2) + (B2), (E5.1) + (A1.2) + (A3.1) + (B2), (E5.1) + (A1.2) + (A3.2) + (B2), (E5.1) + (A1.2) + (A4.1) + (B2), (E5.1) + (A1.2) + (A4.2) + (B2);
    (E5.1) + (A2.1) + (A2.2) + (B2), (E5.1) + (A2.1) + (A3.1) + (B2), (E5.1) + (A2.1) + (A3.2) + (B2), (E5.1) + (A2.1) + (A4.1) + (B2), (E5.1) + (A2.1) + (A4.2) + (B2); (E5.1) + (A2.2) + (A3.1) + (B2), (E5.1) + (A2.2) + (A3.2) + (B2), (E5.1) + (A2.2) + (A4.1) + (B2), (E5.1) + (A2.2) + (A4.2) + (B2);
    (E5.1) + (A3.1) + (A3.2) + (B2), (E5.1) + (A3.1) + (A4.1) + (B2), (E5.1) + (A3.1) + (A4.2) + (B2); (E5.1) + (A3.2) + (A4.1) + (B2), (E5.1) + (A3.2) + (A4.2) + (B2), (E5.1) + (A4.1) + (A4.2) + (B2);
    (E5.1) + (A1.1) + (A1.2) + (B3), (E5.1) + (A1.1) + (A2.1) + (B3), (E5.1) + (A1.1) + (A2.2) + (B3), (E5.1) + (A1.1) + (A3.1) + (B3), (E5.1) + (A1.1) + (A3.2) + (B3), (E5.1) + (A1.1) + (A4.1) + (B3), (E5.1) + (A1.1) + (A4.2) + (B3);
    (E5.1) + (A1.2) + (A2.1) + (B3), (E5.1) + (A1.2) + (A2.2) + (B3), (E5.1) + (A1.2) + (A3.1) + (B3), (E5.1) + (A1.2) + (A3.2) + (B3), (E5.1) + (A1.2) + (A4.1) + (B3), (E5.1) + (A1.2) + (A4.2) + (B3);
    (E5.1) + (A2.1) + (A2.2) + (B3), (E5.1) + (A2.1) + (A3.1) + (B3), (E5.1) + (A2.1) + (A3.2) + (B3), (E5.1) + (A2.1) + (A4.1) + (B3), (E5.1) + (A2.1) + (A4.2) + (B3); (E5.1) + (A2.2) + (A3.1) + (B3), (E5.1) + (A2.2) + (A3.2) + (B3), (E5.1) + (A2.2) + (A4.1) + (B3), (E5.1) + (A2.2) + (A4.2) + (B3);
    (E5.1) + (A3.1) + (A3.2) + (B3), (E5.1) + (A3.1) + (A4.1) + (B3), (E5.1) + (A3.1) + (A4.2) + (B3); (E5.1) + (A3.2) + (A4.1) + (B3), (E5.1) + (A3.2) + (A4.2) + (B3), (E5.1) + (A4.1) + (A4.2) + (B3);
    (E5.2) + (A1.1) + (B1), (E5.2) + (A1.1) + (B2), (E5.2) + (A1.1) + (B3), (E5.2) + (A2.1) + (B1), (E5.2) + (A2.1) + (B2), (E5.2) + (A2.1) + (B3), (E5.2) + (A3.1) + (B1), (E5.2) + (A3.1) + (B2), (E5.2) + (A3.1) + (B3), (E5.2) + (A4.1) + (B1), (E5.2) + (A4.1) + (B2), (E5.2) + (A4.1) + (B3), (E5.2) + (A1.2) + (B1), (E5.2) + (A1.2) + (B2), (E5.2) + (A1.2) + (B3), (E5.2) + (A2.2) + (B1), (E5.2) + (A2.2) + (B2), (E5.2) + (A2.2) + (B3), (E5.2) + (A3.2) + (B1), (E5.2) + (A3.2) + (B2), (E5.2) + (A3.2) + (B3), (E5.2) + (A4.2) + (B1), (E5.2) + (A4.2) + (B2), (E5.2) + (A4.2) + (B3),
    (E5.2) + (A1.1) + (A1.2) + (B1), (E5.2) + (A1.1) + (A2.1) + (B1), (E5.2) + (A1.1) + (A2.2) + (B1), (E5.2) + (A1.1) + (A3.1) + (B1), (E5.2) + (A1.1) + (A3.2) + (B1), (E5.2) + (A1.1) + (A4.1) + (B1), (E5.2) + (A1.1) + (A4.2) + (B1);
    (E5.2) + (A1.2) + (A2.1) + (B1), (E5.2) + (A1.2) + (A2.2) + (B1), (E5.2) + (A1.2) + (A3.1) + (B1), (E5.2) + (A1.2) + (A3.2) + (B1), (E5.2) + (A1.2) + (A4.1) + (B1), (E5.2) + (A1.2) + (A4.2) + (B1);
    (E5.2) + (A2.1) + (A2.2) + (B1), (E5.2) + (A2.1) + (A3.1) + (B1), (E5.2) + (A2.1) + (A3.2) + (B1), (E5.2) + (A2.1) + (A4.1) + (B1), (E5.2) + (A2.1) + (A4.2) + (B1); (E5.2) + (A2.2) + (A3.1) + (B1), (E5.2) + (A2.2) + (A3.2) + (B1), (E5.2) + (A2.2) + (A4.1) + (B1), (E5.2) + (A2.2) + (A4.2) + (B1);
    (E5.2) + (A3.1) + (A3.2) + (B1), (E5.2) + (A3.1) + (A4.1) + (B1), (E5.2) + (A3.1) + (A4.2) + (B1); (E5.2) + (A3.2) + (A4.1) + (B1), (E5.2) + (A3.2) + (A4.2) + (B1), (E5.2) + (A4.1) + (A4.2) + (B1);
    (E5.2) + (A1.1) + (A1.2) + (B2), (E5.2) + (A1.1) + (A2.1) + (B2), (E5.2) + (A1.1) + (A2.2) + (B2), (E5.2) + (A1.1) + (A3.1) + (B2), (E5.2) + (A1.1) + (A3.2) + (B2), (E5.2) + (A1.1) + (A4.1) + (B2), (E5.2) + (A1.1) + (A4.2) + (B2);
    (E5.2) + (A1.2) + (A2.1) + (B2), (E5.2) + (A1.2) + (A2.2) + (B2), (E5.2) + (A1.2) + (A3.1) + (B2), (E5.2) + (A1.2) + (A3.2) + (B2), (E5.2) + (A1.2) + (A4.1) + (B2), (E5.2) + (A1.2) + (A4.2) + (B2);
    (E5.2) + (A2.1) + (A2.2) + (B2), (E5.2) + (A2.1) + (A3.1) + (B2), (E5.2) + (A2.1) + (A3.2) + (B2), (E5.2) + (A2.1) + (A4.1) + (B2), (E5.2) + (A2.1) + (A4.2) + (B2);
    (E5.2) + (A2.2) + (A3.1) + (B2), (E5.2) + (A2.2) + (A3.2) + (B2), (E5.2) + (A2.2) + (A4.1) + (B2), (E5.2) + (A2.2) + (A4.2) + (B2);
    (E5.2) + (A3.1) + (A3.2) + (B2), (E5.2) + (A3.1) + (A4.1) + (B2), (E5.2) + (A3.1) + (A4.2) + (B2); (E5.2) + (A3.2) + (A4.1) + (B2), (E5.2) + (A3.2) + (A4.2) + (B2), (E5.2) + (A4.1) + (A4.2) + (B2);
    (E5.2) + (A1.1) + (A1.2) + (B3), (E5.2) + (A1.1) + (A2.1) + (B3), (E5.2) + (A1.1) + (A2.2) + (B3), (E5.2) + (A1.1) + (A3.1) + (B3), (E5.2) + (A1.1) + (A3.2) + (B3), (E5.2) + (A1.1) + (A4.1) + (B3), (E5.2) + (A1.1) + (A4.2) + (B3);
    (E5.2) + (A1.2) + (A2.1) + (B3), (E5.2) + (A1.2) + (A2.2) + (B3), (E5.2) + (A1.2) + (A3.1) + (B3), (E5.2) + (A1.2) + (A3.2) + (B3), (E5.2) + (A1.2) + (A4.1) + (B3), (E5.2) + (A1.2) + (A4.2) + (B3);
    (E5.2) + (A2.1) + (A2.2) + (B3), (E5.2) + (A2.1) + (A3.1) + (B3), (E5.2) + (A2.1) + (A3.2) + (B3), (E5.2) + (A2.1) + (A4.1) + (B3), (E5.2) + (A2.1) + (A4.2) + (B3);
    (E5.2) + (A2.2) + (A3.1) + (B3), (E5.2) + (A2.2) + (A3.2) + (B3), (E5.2) + (A2.2) + (A4.1) + (B3), (E5.2) + (A2.2) + (A4.2) + (B3);
    (E5.2) + (A3.1) + (A3.2) + (B3), (E5.2) + (A3.1) + (A4.1) + (B3), (E5.2) + (A3.1) + (A4.2) + (B3); (E5.2) + (A3.2) + (A4.1) + (B3), (E5.2) + (A3.2) + (A4.2) + (B3), (E5.2) + (A4.1) + (A4.2) + (B3);
    (E6) + (A1.1) + (B1), (E6) + (A1.1) + (B2), (E6) + (A1.1) + (B3), (E6) + (A2.1) + (B1), (E6) + (A2.1) + (B2), (E6) + (A2.1) + (B3), (E6) + (A3.1) + (B1), (E6) + (A3.1) + (B2), (E6) + (A3.1) + (B3), (E6) + (A4.1) + (B1), (E6) + (A4.1) + (B2), (E6) + (A4.1) + (B3), (E6) + (A1.2) + (B1), (E6) + (A1.2) + (B2), (E6) + (A1.2) + (B3), (E6) + (A2.2) + (B1), (E6) + (A2.2) + (B2), (E6) + (A2.2) + (B3), (E6) + (A3.2) + (B1), (E6) + (A3.2) + (B2), (E6) + (A3.2) + (B3), (E6) + (A4.2) + (B1), (E6) + (A4.2) + (B2), (E6) + (A4.2) + (B3), (E6) + (A1.1) + (A1.2) + (B1), (E6) + (A1.1) + (A2.1) + (B1), (E6) + (A1.1) + (A2.2) + (B1), (E6) + (A1.1) + (A3.1) + (B1), (E6) + (A1.1) + (A3.2) + (B1), (E6) + (A1.1) + (A4.1) + (B1), (E6) + (A1.1) + (A4.2) + (B1);
    (E6) + (A1.2) + (A2.1) + (B1), (E6) + (A1.2) + (A2.2) + (B1), (E6) + (A1.2) + (A3.1) + (B1), (E6) + (A1.2) + (A3.2) + (B1), (E6) + (A1.2) + (A4.1) + (B1), (E6) + (A1.2) + (A4.2) + (B1);
    (E6) + (A2.1) + (A2.2) + (B1), (E6) + (A2.1) + (A3.1) + (B1), (E6) + (A2.1) + (A3.2) + (B1), (E6) + (A2.1) + (A4.1) + (B1), (E6) + (A2.1) + (A4.2) + (B1);
    (E6) + (A2.2) + (A3.1) + (B1), (E6) + (A2.2) + (A3.2) + (B1), (E6) + (A2.2) + (A4.1) + (B1), (E6) + (A2.2) + (A4.2) + (B1);
    (E6) + (A3.1) + (A3.2) + (B1), (E6) + (A3.1) + (A4.1) + (B1), (E6) + (A3.1) + (A4.2) + (B1); (E6) + (A3.2) + (A4.1) + (B1), (E6) + (A3.2) + (A4.2) + (B1), (E6) + (A4.1) + (A4.2) + (B1);
    (E6) + (A1.1) + (A1.2) + (B2), (E6) + (A1.1) + (A2.1) + (B2), (E6) + (A1.1) + (A2.2) + (B2), (E6) + (A1.1) + (A3.1) + (B2), (E6) + (A1.1) + (A3.2) + (B2), (E6) + (A1.1) + (A4.1) + (B2), (E6) + (A1.1) + (A4.2) + (B2);
    (E6) + (A1.2) + (A2.1) + (B2), (E6) + (A1.2) + (A2.2) + (B2), (E6) + (A1.2) + (A3.1) + (B2), (E6) + (A1.2) + (A3.2) + (B2), (E6) + (A1.2) + (A4.1) + (B2), (E6) + (A1.2) + (A4.2) + (B2);
    (E6) + (A2.1) + (A2.2) + (B2), (E6) + (A2.1) + (A3.1) + (B2), (E6) + (A2.1) + (A3.2) + (B2), (E6) + (A2.1) + (A4.1) + (B2), (E6) + (A2.1) + (A4.2) + (B2);
    (E6) + (A2.2) + (A3.1) + (B2), (E6) + (A2.2) + (A3.2) + (B2), (E6) + (A2.2) + (A4.1) + (B2), (E6) + (A2.2) + (A4.2) + (B2);
    (E6) + (A3.1) + (A3.2) + (B2), (E6) + (A3.1) + (A4.1) + (B2), (E6) + (A3.1) + (A4.2) + (B2); (E6) + (A3.2) + (A4.1) + (B2), (E6) + (A3.2) + (A4.2) + (B2), (E6) + (A4.1) + (A4.2) + (B2);
    (E6) + (A1.1) + (A1.2) + (B3), (E6) + (A1.1) + (A2.1) + (B3), (E6) + (A1.1) + (A2.2) + (B3), (E6) + (A1.1) + (A3.1) + (B3), (E6) + (A1.1) + (A3.2) + (B3), (E6) + (A1.1) + (A4.1) + (B3), (E6) + (A1.1) + (A4.2) + (B3);
    (E6) + (A1.2) + (A2.1) + (B3), (E6) + (A1.2) + (A2.2) + (B3), (E6) + (A1.2) + (A3.1) + (B3), (E6) + (A1.2) + (A3.2) + (B3), (E6) + (A1.2) + (A4.1) + (B3), (E6) + (A1.2) + (A4.2) + (B3);
    (E6) + (A2.1) + (A2.2) + (B3), (E6) + (A2.1) + (A3.1) + (B3), (E6) + (A2.1) + (A3.2) + (B3), (E6) + (A2.1) + (A4.1) + (B3), (E6) + (A2.1) + (A4.2) + (B3);
    (E6) + (A2.2) + (A3.1) + (B3), (E6) + (A2.2) + (A3.2) + (B3), (E6) + (A2.2) + (A4.1) + (B3), (E6) + (A2.2) + (A4.2) + (B3);
    (E6) + (A3.1) + (A3.2) + (B3), (E6) + (A3.1) + (A4.1) + (B3), (E6) + (A3.1) + (A4.2) + (B3); (E6) + (A3.2) + (A4.1) + (B3), (E6) + (A3.2) + (A4.2) + (B3), (E6) + (A4.1) + (A4.2) + (B3);
    (E6.1) + (A1.1) + (B 1), (E6.1) + (A1.1) + (B2), (E6.1) + (A1.1) + (B3), (E6.1) + (A2.1) + (B1), (E6.1) + (A2.1) + (B2), (E6.1) + (A2.1) + (B3), (E6.1) + (A3.1) + (B1), (E6.1) + (A3.1) + (B2), (E6.1) + (A3.1) + (B3), (E6.1) + (A4.1) + (B1), (E6.1) + (A4.1) + (B2), (E6.1) + (A4.1) + (B3), (E6.1) + (A1.2) + (B1), (E6.1) + (A1.2) + (B2), (E6.1) + (A1.2) + (B3), (E6.1) + (A2.2) + (B1), (E6.1) + (A2.2) + (B2), (E6.1) + (A2.2) + (B3), (E6.1) + (A3.2) + (B1), (E6.1) + (A3.2) + (B2), (E6.1) + (A3.2) + (B3), (E6.1) + (A4.2) + (B1), (E6.1) + (A4.2) + (B2), (E6.1) + (A4.2) + (B3),
    (E6.1) + (A1.1) + (A1.2) + (B1), (E6.1) + (A1.1) + (A2.1) + (B1), (E6.1) + (A1.1) + (A2.2) + (B1), (E6.1) + (A1.1) + (A3.1) + (B1), (E6.1) + (A1.1) + (A3.2) + (B1), (E6.1) + (A1.1) + (A4.1) + (B1), (E6.1) + (A1.1) + (A4.2) + (B1);
    (E6.1) + (A1.2) + (A2.1) + (B1), (E6.1) + (A1.2) + (A2.2) + (B1), (E6.1) + (A1.2) + (A3.1) + (B1), (E6.1) + (A1.2) + (A3.2) + (B1), (E6.1) + (A1.2) + (A4.1) + (B1), (E6.1) + (A1.2) + (A4.2) + (B1);
    (E6.1) + (A2.1) + (A2.2) + (B1), (E6.1) + (A2.1) + (A3.1) + (B1), (E6.1) + (A2.1) + (A3.2) + (B1), (E6.1) + (A2.1) + (A4.1) + (B1), (E6.1) + (A2.1) + (A4.2) + (B1);
    (E6.1) + (A2.2) + (A3.1) + (B1), (E6.1) + (A2.2) + (A3.2) + (B1), (E6.1) + (A2.2) + (A4.1) + (B1), (E6.1) + (A2.2) + (A4.2) + (B1);
    (E6.1) + (A3.1) + (A3.2) + (B1), (E6.1) + (A3.1) + (A4.1) + (B1), (E6.1) + (A3.1) + (A4.2) + (B1); (E6.1) + (A3.2) + (A4.1) + (B1), (E6.1) + (A3.2) + (A4.2) + (B1), (E6.1) + (A4.1) + (A4.2) + (B1);
    (E6.1) + (A1.1) + (A1.2) + (B2), (E6.1) + (A1.1) + (A2.1) + (B2), (E6.1) + (A1.1) + (A2.2) + (B2), (E6.1) + (A1.1) + (A3.1) + (B2), (E6.1) + (A1.1) + (A3.2) + (B2), (E6.1) + (A1.1) + (A4.1) + (B2), (E6.1) + (A1.1) + (A4.2) + (B2);
    (E6.1) + (A1.2) + (A2.1) + (B2), (E6.1) + (A1.2) + (A2.2) + (B2), (E6.1) + (A1.2) + (A3.1) + (B2), (E6.1) + (A1.2) + (A3.2) + (B2), (E6.1) + (A1.2) + (A4.1) + (B2), (E6.1) + (A1.2) + (A4.2) + (B2);
    (E6.1) + (A2.1) + (A2.2) + (B2), (E6.1) + (A2.1) + (A3.1) + (B2), (E6.1) + (A2.1) + (A3.2) + (B2), (E6.1) + (A2.1) + (A4.1) + (B2), (E6.1) + (A2.1) + (A4.2) + (B2);
    (E6.1) + (A2.2) + (A3.1) + (B2), (E6.1) + (A2.2) + (A3.2) + (B2), (E6.1) + (A2.2) + (A4.1) + (B2), (E6.1) + (A2.2) + (A4.2) + (B2);
    (E6.1) + (A3.1) + (A3.2) + (B2), (E6.1) + (A3.1) + (A4.1) + (B2), (E6.1) + (A3.1) + (A4.2) + (B2); (E6.1) + (A3.2) + (A4.1) + (B2), (E6.1) + (A3.2) + (A4.2) + (B2), (E6.1) + (A4.1) + (A4.2) + (B2);
    (E6.1) + (A1.1) + (A1.2) + (B3), (E6.1) + (A1.1) + (A2.1) + (B3), (E6.1) + (A1.1) + (A2.2) + (B3), (E6.1) + (A1.1) + (A3.1) + (B3), (E6.1) + (A1.1) + (A3.2) + (B3), (E6.1) + (A1.1) + (A4.1) + (B3), (E6.1) + (A1.1) + (A4.2) + (B3);
    (E6.1) + (A1.2) + (A2.1) + (B3), (E6.1) + (A1.2) + (A2.2) + (B3), (E6.1) + (A1.2) + (A3.1) + (B3), (E6.1) + (A1.2) + (A3.2) + (B3), (E6.1) + (A1.2) + (A4.1) + (B3), (E6.1) + (A1.2) + (A4.2) + (B3);
    (E6.1) + (A2.1) + (A2.2) + (B3), (E6.1) + (A2.1) + (A3.1) + (B3), (E6.1) + (A2.1) + (A3.2) + (B3), (E6.1) + (A2.1) + (A4.1) + (B3), (E6.1) + (A2.1) + (A4.2) + (B3);
    (E6.1) + (A2.2) + (A3.1) + (B3), (E6.1) + (A2.2) + (A3.2) + (B3), (E6.1) + (A2.2) + (A4.1) + (B3), (E6.1) + (A2.2) + (A4.2) + (B3);
    (E6.1) + (A3.1) + (A3.2) + (B3), (E6.1) + (A3.1) + (A4.1) + (B3), (E6.1) + (A3.1) + (A4.2) + (B3); (E6.1) + (A3.2) + (A4.1) + (B3), (E6.1) + (A3.2) + (A4.2) + (B3), (E6.1) + (A4.1) + (A4.2) + (B3);
    (E6.2) + (A1.1) + (B1), (E6.2) + (A1.1) + (B2), (E6.2) + (A1.1) + (B3), (E6.2) + (A2.1) + (B1), (E6.2) + (A2.1) + (B2), (E6.2) + (A2.1) + (B3), (E6.2) + (A3.1) + (B1), (E6.2) + (A3.1) + (B2), (E6.2) + (A3.1) + (B3), (E6.2) + (A4.1) + (B1), (E6.2) + (A4.1) + (B2), (E6.2) + (A4.1) + (B3), (E6.2) + (A1.2) + (B1), (E6.2) + (A1.2) + (B2), (E6.2) + (A1.2) + (B3), (E6.2) + (A2.2) + (B1), (E6.2) + (A2.2) + (B2), (E6.2) + (A2.2) + (B3), (E6.2) + (A3.2) + (B1), (E6.2) + (A3.2) + (B2), (E6.2) + (A3.2) + (B3), (E6.2) + (A4.2) + (B1), (E6.2) + (A4.2) + (B2), (E6.2) + (A4.2) + (B3),
    (E6.2) + (A1.1) + (A1.2) + (B1), (E6.2) + (A1.1) + (A2.1) + (B1), (E6.2) + (A1.1) + (A2.2) + (B1), (E6.2) + (A1.1) + (A3.1) + (B1), (E6.2) + (A1.1) + (A3.2) + (B1), (E6.2) + (A1.1) + (A4.1) + (B1), (E6.2) + (A1.1) + (A4.2) + (B1);
    (E6.2) + (A1.2) + (A2.1) + (B1), (E6.2) + (A1.2) + (A2.2) + (B1), (E6.2) + (A1.2) + (A3.1) + (B1), (E6.2) + (A1.2) + (A3.2) + (B1), (E6.2) + (A1.2) + (A4.1) + (B1), (E6.2) + (A1.2) + (A4.2) + (B1);
    (E6.2) + (A2.1) + (A2.2) + (B1), (E6.2) + (A2.1) + (A3.1) + (B1), (E6.2) + (A2.1) + (A3.2) + (B1), (E6.2) + (A2.1) + (A4.1) + (B1), (E6.2) + (A2.1) + (A4.2) + (B1);
    (E6.2) + (A2.2) + (A3.1) + (B1), (E6.2) + (A2.2) + (A3.2) + (B1), (E6.2) + (A2.2) + (A4.1) + (B1), (E6.2) + (A2.2) + (A4.2) + (B1);
    (E6.2) + (A3.1) + (A3.2) + (B1), (E6.2) + (A3.1) + (A4.1) + (B1), (E6.2) + (A3.1) + (A4.2) + (B1); (E6.2) + (A3.2) + (A4.1) + (B1), (E6.2) + (A3.2) + (A4.2) + (B1), (E6.2) + (A4.1) + (A4.2) + (B1);
    (E6.2) + (A1.1) + (A1.2) + (B2), (E6.2) + (A1.1) + (A2.1) + (B2), (E6.2) + (A1.1) + (A2.2) + (B2), (E6.2) + (A1.1) + (A3.1) + (B2), (E6.2) + (A1.1) + (A3.2) + (B2), (E6.2) + (A1.1) + (A4.1) + (B2), (E6.2) + (A1.1) + (A4.2) + (B2);
    (E6.2) + (A1.2) + (A2.1) + (B2), (E6.2) + (A1.2) + (A2.2) + (B2), (E6.2) + (A1.2) + (A3.1) + (B2), (E6.2) + (A1.2) + (A3.2) + (B2), (E6.2) + (A1.2) + (A4.1) + (B2), (E6.2) + (A1.2) + (A4.2) + (B2);
    (E6.2) + (A2.1) + (A2.2) + (B2), (E6.2) + (A2.1) + (A3.1) + (B2), (E6.2) + (A2.1) + (A3.2) + (B2), (E6.2) + (A2.1) + (A4.1) + (B2), (E6.2) + (A2.1) + (A4.2) + (B2);
    (E6.2) + (A2.2) + (A3.1) + (B2), (E6.2) + (A2.2) + (A3.2) + (B2), (E6.2) + (A2.2) + (A4.1) + (B2), (E6.2) + (A2.2) + (A4.2) + (B2);
    (E6.2) + (A3.1) + (A3.2) + (B2), (E6.2) + (A3.1) + (A4.1) + (B2), (E6.2) + (A3.1) + (A4.2) + (B2); (E6.2) + (A3.2) + (A4.1) + (B2), (E6.2) + (A3.2) + (A4.2) + (B2), (E6.2) + (A4.1) + (A4.2) + (B2);
    (E6.2) + (A1.1) + (A1.2) + (B3), (E6.2) + (A1.1) + (A2.1) + (B3), (E6.2) + (A1.1) + (A2.2) + (B3), (E6.2) + (A1.1) + (A3.1) + (B3), (E6.2) + (A1.1) + (A3.2) + (B3), (E6.2) + (A1.1) + (A4.1) + (B3), (E6.2) + (A1.1) + (A4.2) + (B3);
    (E6.2) + (A1.2) + (A2.1) + (B3), (E6.2) + (A1.2) + (A2.2) + (B3), (E6.2) + (A1.2) + (A3.1) + (B3), (E6.2) + (A1.2) + (A3.2) + (B3), (E6.2) + (A1.2) + (A4.1) + (B3), (E6.2) + (A1.2) + (A4.2) + (B3);
    (E6.2) + (A2.1) + (A2.2) + (B3), (E6.2) + (A2.1) + (A3.1) + (B3), (E6.2) + (A2.1) + (A3.2) + (B3), (E6.2) + (A2.1) + (A4.1) + (B3), (E6.2) + (A2.1) + (A4.2) + (B3);
    (E6.2) + (A2.2) + (A3.1) + (B3), (E6.2) + (A2.2) + (A3.2) + (B3), (E6.2) + (A2.2) + (A4.1) + (B3), (E6.2) + (A2.2) + (A4.2) + (B3);
    (E6.2) + (A3.1) + (A3.2) + (B3), (E6.2) + (A3.1) + (A4.1) + (B3), (E6.2) + (A3.1) + (A4.2) + (B3); (E6.2) + (A3.2) + (A4.1) + (B3), (E6.2) + (A3.2) + (A4.2) + (B3), (E6.2) + (A4.1) + (A4.2) + (B3);
    (E6.3) + (A1.1) + (B1), (E6.3) + (A1.1) + (B2), (E6.3) + (A1.1) + (B3), (E6.3) + (A2.1) + (B1), (E6.3) + (A2.1) + (B2), (E6.3) + (A2.1) + (B3), (E6.3) + (A3.1) + (B1), (E6.3) + (A3.1) + (B2), (E6.3) + (A3.1) + (B3), (E6.3) + (A4.1) + (B1), (E6.3) + (A4.1) + (B2), (E6.3) + (A4.1) + (B3), (E6.3) + (A1.2) + (B1), (E6.3) + (A1.2) + (B2), (E6.3) + (A1.2) + (B3), (E6.3) + (A2.2) + (B1), (E6.3) + (A2.2) + (B2), (E6.3) + (A2.2) + (B3), (E6.3) + (A3.2) + (B1), (E6.3) + (A3.2) + (B2), (E6.3) + (A3.2) + (B3), (E6.3) + (A4.2) + (B1), (E6.3) + (A4.2) + (B2), (E6.3) + (A4.2) + (B3),
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    (E6.3) + (A3.1) + (A3.2) + (B1), (E6.3) + (A3.1) + (A4.1) + (B1), (E6.3) + (A3.1) + (A4.2) + (B1); (E6.3) + (A3.2) + (A4.1) + (B1), (E6.3) + (A3.2) + (A4.2) + (B1), (E6.3) + (A4.1) + (A4.2) + (B1);
    (E6.3) + (A1.1) + (A1.2) + (B2), (E6.3) + (A1.1) + (A2.1) + (B2), (E6.3) + (A1.1) + (A2.2) + (B2), (E6.3) + (A1.1) + (A3.1) + (B2), (E6.3) + (A1.1) + (A3.2) + (B2), (E6.3) + (A1.1) + (A4.1) + (B2), (E6.3) + (A1.1) + (A4.2) + (B2);
    (E6.3) + (A1.2) + (A2.1) + (B2), (E6.3) + (A1.2) + (A2.2) + (B2), (E6.3) + (A1.2) + (A3.1) + (B2), (E6.3) + (A1.2) + (A3.2) + (B2), (E6.3) + (A1.2) + (A4.1) + (B2), (E6.3) + (A1.2) + (A4.2) + (B2);
    (E6.3) + (A2.1) + (A2.2) + (B2), (E6.3) + (A2.1) + (A3.1) + (B2), (E6.3) + (A2.1) + (A3.2) + (B2), (E6.3) + (A2.1) + (A4.1) + (B2), (E6.3) + (A2.1) + (A4.2) + (B2);
    (E6.3) + (A2.2) + (A3.1) + (B2), (E6.3) + (A2.2) + (A3.2) + (B2), (E6.3) + (A2.2) + (A4.1) + (B2), (E6.3) + (A2.2) + (A4.2) + (B2);
    (E6.3) + (A3.1) + (A3.2) + (B2), (E6.3) + (A3.1) + (A4.1) + (B2), (E6.3) + (A3.1) + (A4.2) + (B2); (E6.3) + (A3.2) + (A4.1) + (B2), (E6.3) + (A3.2) + (A4.2) + (B2), (E6.3) + (A4.1) + (A4.2) + (B2);
    (E6.3) + (A1.1) + (A1.2) + (B3), (E6.3) + (A1.1) + (A2.1) + (B3), (E6.3) + (A1.1) + (A2.2) + (B3), (E6.3) + (A1.1) + (A3.1) + (B3), (E6.3) + (A1.1) + (A3.2) + (B3), (E6.3) + (A1.1) + (A4.1) + (B3), (E6.3) + (A1.1) + (A4.2) + (B3);
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    (E6.3) + (A2.2) + (A3.1) + (B3), (E6.3) + (A2.2) + (A3.2) + (B3), (E6.3) + (A2.2) + (A4.1) + (B3), (E6.3) + (A2.2) + (A4.2) + (B3);
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    (E6.5) + (A1.2) + (A2.1) + (B2), (E6.5) + (A1.2) + (A2.2) + (B2), (E6.5) + (A1.2) + (A3.1) + (B2), (E6.5) + (A1.2) + (A3.2) + (B2), (E6.5) + (A1.2) + (A4.1) + (B2), (E6.5) + (A1.2) + (A4.2) + (B2);
    (E6.5) + (A2.1) + (A2.2) + (B2), (E6.5) + (A2.1) + (A3.1) + (B2), (E6.5) + (A2.1) + (A3.2) + (B2), (E6.5) + (A2.1) + (A4.1) + (B2), (E6.5) + (A2.1) + (A4.2) + (B2);
    (E6.5) + (A2.2) + (A3.1) + (B2), (E6.5) + (A2.2) + (A3.2) + (B2), (E6.5) + (A2.2) + (A4.1) + (B2), (E6.5) + (A2.2) + (A4.2) + (B2);
    (E6.5) + (A3.1) + (A3.2) + (B2), (E6.5) + (A3.1) + (A4.1) + (B2), (E6.5) + (A3.1) + (A4.2) + (B2); (E6.5) + (A3.2) + (A4.1) + (B2), (E6.5) + (A3.2) + (A4.2) + (B2), (E6.5) + (A4.1) + (A4.2) + (B2);
    (E6.5) + (A1.1) + (A1.2) + (B3), (E6.5) + (A1.1) + (A2.1) + (B3), (E6.5) + (A1.1) + (A2.2) + (B3), (E6.5) + (A1.1) + (A3.1) + (B3), (E6.5) + (A1.1) + (A3.2) + (B3), (E6.5) + (A1.1) + (A4.1) + (B3), (E6.5) + (A1.1) + (A4.2) + (B3);
    (E6.5) + (A1.2) + (A2.1) + (B3), (E6.5) + (A1.2) + (A2.2) + (B3), (E6.5) + (A1.2) + (A3.1) + (B3), (E6.5) + (A1.2) + (A3.2) + (B3), (E6.5) + (A1.2) + (A4.1) + (B3), (E6.5) + (A1.2) + (A4.2) + (B3);
    (E6.5) + (A2.1) + (A2.2) + (B3), (E6.5) + (A2.1) + (A3.1) + (B3), (E6.5) + (A2.1) + (A3.2) + (B3), (E6.5) + (A2.1) + (A4.1) + (B3), (E6.5) + (A2.1) + (A4.2) + (B3);
    (E6.5) + (A2.2) + (A3.1) + (B3), (E6.5) + (A2.2) + (A3.2) + (B3), (E6.5) + (A2.2) + (A4.1) + (B3), (E6.5) + (A2.2) + (A4.2) + (B3);
    (E6.5) + (A3.1) + (A3.2) + (B3), (E6.5) + (A3.1) + (A4.1) + (B3), (E6.5) + (A3.1) + (A4.2) + (B3); (E6.5) + (A3.2) + (A4.1) + (B3), (E6.5) + (A3.2) + (A4.2) + (B3), (E6.5) + (A4.1) + (A4.2) + (B3);
    (E7) + (A1.1) + (B1), (E7) + (A1.1) + (B2), (E7) + (A1.1) + (B3), (E7) + (A2.1) + (B1), (E7) + (A2.1) + (B2), (E7) + (A2.1) + (B3), (E7) + (A3.1) + (B1), (E7) + (A3.1) + (B2), (E7) + (A3.1) + (B3), (E7) + (A4.1) + (B1), (E7) + (A4.1) + (B2), (E7) + (A4.1) + (B3), (E7) + (A1.2) + (B1), (E7) + (A1.2) + (B2), (E7) + (A1.2) + (B3), (E7) + (A2.2) + (B1), (E7) + (A2.2) + (B2), (E7) + (A2.2) + (B3), (E7) + (A3.2) + (B1), (E7) + (A3.2) + (B2), (E7) + (A3.2) + (B3), (E7) + (A4.2) + (B1), (E7) + (A4.2) + (B2), (E7) + (A4.2) + (B3), (E7) + (A1.1) + (A1.2) + (B1), (E7) + (A1.1) + (A2.1) + (B1), (E7) + (A1.1) + (A2.2) + (B1), (E7) + (A1.1) + (A3.1) + (B1), (E7) + (A1.1) + (A3.2) + (B1), (E7) + (A1.1) + (A4.1) + (B1), (E7) + (A1.1) + (A4.2) + (B1);
    (E7) + (A1.2) + (A2.1) + (B1), (E7) + (A1.2) + (A2.2) + (B1), (E7) + (A1.2) + (A3.1) + (B1), (E7) + (A1.2) + (A3.2) + (B1), (E7) + (A1.2) + (A4.1) + (B1), (E7) + (A1.2) + (A4.2) + (B1);
    (E7) + (A2.1) + (A2.2) + (B1), (E7) + (A2.1) + (A3.1) + (B1), (E7) + (A2.1) + (A3.2) + (B1), (E7) + (A2.1) + (A4.1) + (B1), (E7) + (A2.1) + (A4.2) + (B1);
    (E7) + (A2.2) + (A3.1) + (B1), (E7) + (A2.2) + (A3.2) + (B1), (E7) + (A2.2) + (A4.1) + (B1), (E7) + (A2.2) + (A4.2) + (B1);
    (E7) + (A3.1) + (A3.2) + (B1), (E7) + (A3.1) + (A4.1) + (B1), (E7) + (A3.1) + (A4.2) + (B1), (E7) + (A3.2) + (A4.1) + (B1), (E7) + (A3.2) + (A4.2) + (B1), (E7) + (A4.1) + (A4.2) + (B1);
    (E7) + (A1.1) + (A1.2) + (B2), (E7) + (A1.1) + (A2.1) + (B2), (E7) + (A1.1) + (A2.2) + (B2), (E7) + (A1.1) + (A3.1) + (B2), (E7) + (A1.1) + (A3.2) + (B2), (E7) + (A1.1) + (A4.1) + (B2), (E7) + (A1.1) + (A4.2) + (B2);
    (E7) + (A1.2) + (A2.1) + (B2), (E7) + (A1.2) + (A2.2) + (B2), (E7) + (A1.2) + (A3.1) + (B2), (E7) + (A1.2) + (A3.2) + (B2), (E7) + (A1.2) + (A4.1) + (B2), (E7) + (A1.2) + (A4.2) + (B2);
    (E7) + (A2.1) + (A2.2) + (B2), (E7) + (A2.1) + (A3.1) + (B2), (E7) + (A2.1) + (A3.2) + (B2), (E7) + (A2.1) + (A4.1) + (B2), (E7) + (A2.1) + (A4.2) + (B2);
    (E7) + (A2.2) + (A3.1) + (B2), (E7) + (A2.2) + (A3.2) + (B2), (E7) + (A2.2) + (A4.1) + (B2), (E7) + (A2.2) + (A4.2) + (B2);
    (E7) + (A3.1) + (A3.2) + (B2), (E7) + (A3.1) + (A4.1) + (B2), (E7) + (A3.1) + (A4.2) + (B2); (E7) + (A3.2) + (A4.1) + (B2), (E7) + (A3.2) + (A4.2) + (B2), (E7) + (A4.1) + (A4.2) + (B2);
    (E7) + (A1.1) + (A1.2) + (B3), (E7) + (A1.1) + (A2.1) + (B3), (E7) + (A1.1) + (A2.2) + (B3), (E7) + (A1.1) + (A3.1) + (B3), (E7) + (A1.1) + (A3.2) + (B3), (E7) + (A1.1) + (A4.1) + (B3), (E7) + (A1.1) + (A4.2) + (B3);
    (E7) + (A1.2) + (A2.1) + (B3), (E7) + (A1.2) + (A2.2) + (B3), (E7) + (A1.2) + (A3.1) + (B3), (E7) + (A1.2) + (A3.2) + (B3), (E7) + (A1.2) + (A4.1) + (B3), (E7) + (A1.2) + (A4.2) + (B3);
    (E7) + (A2.1) + (A2.2) + (B3), (E7) + (A2.1) + (A3.1) + (B3), (E7) + (A2.1) + (A3.2) + (B3), (E7) + (A2.1) + (A4.1) + (B3), (E7) + (A2.1) + (A4.2) + (B3); (E7) + (A2.2) + (A3.1) + (B3), (E7) + (A2.2) + (A3.2) + (B3), (E7) + (A2.2) + (A4.1) + (B3), (E7) + (A2.2) + (A4.2) + (B3);
    (E7) + (A3.1) + (A3.2) + (B3), (E7) + (A3.1) + (A4.1) + (B3), (E7) + (A3.1) + (A4.2) + (B3); (E7) + (A3.2) + (A4.1) + (B3), (E7) + (A3.2) + (A4.2) + (B3), (E7) + (A4.1) + (A4.2) + (B3);
    (E7.1) + (A1.1) + (B1), (E7.1) + (A1.1) + (B2), (E7.1) + (A1.1) + (B3), (E7.1) + (A2.1) + (B1), (E7.1) + (A2.1) + (B2), (E7.1) + (A2.1) + (B3), (E7.1) + (A3.1) + (B1), (E7.1) + (A3.1) + (B2), (E7.1) + (A3.1) + (B3), (E7.1) + (A4.1) + (B 1), (E7.1) + (A4.1) + (B2), (E7.1) + (A4.1) + (B3), (E7.1) + (A1.2) + (B 1), (E7.1) + (A1.2) + (B2), (E7.1) + (A1.2) + (B3), (E7.1) + (A2.2) + (B1), (E7.1) + (A2.2) + (B2), (E7.1) + (A2.2) + (B3), (E7.1) + (A3.2) + (B1), (E7.1) + (A3.2) + (B2), (E7.1) + (A3.2) + (B3), (E7.1) + (A4.2) + (B1), (E7.1) + (A4.2) + (B2), (E7.1) + (A4.2) + (B3),
    (E7.1) + (A1.1) + (A1.2) + (B1), (E7.1) + (A1.1) + (A2.1) + (B1), (E7.1) + (A1.1) + (A2.2) + (B1), (E7.1) + (A1.1) + (A3.1) + (B1), (E7.1) + (A1.1) + (A3.2) + (B1), (E7.1) + (A1.1) + (A4.1) + (B1), (E7.1) + (A1.1) + (A4.2) + (B1);
    (E7.1) + (A1.2) + (A2.1) + (B1), (E7.1) + (A1.2) + (A2.2) + (B1), (E7.1) + (A1.2) + (A3.1) + (B1), (E7.1) + (A1.2) + (A3.2) + (B1), (E7.1) + (A1.2) + (A4.1) + (B1), (E7.1) + (A1.2) + (A4.2) + (B1);
    (E7.1) + (A2.1) + (A2.2) + (B1), (E7.1) + (A2.1) + (A3.1) + (B1), (E7.1) + (A2.1) + (A3.2) + (B1), (E7.1) + (A2.1) + (A4.1) + (B1), (E7.1) + (A2.1) + (A4.2) + (B1); (E7.1) + (A2.2) + (A3.1) + (B1), (E7.1) + (A2.2) + (A3.2) + (B1), (E7.1) + (A2.2) + (A4.1) + (B1), (E7.1) + (A2.2) + (A4.2) + (B1);
    (E7.1) + (A3.1) + (A3.2) + (B1), (E7.1) + (A3.1) + (A4.1) + (B1), (E7.1) + (A3.1) + (A4.2) + (B1); (E7.1) + (A3.2) + (A4.1) + (B1), (E7.1) + (A3.2) + (A4.2) + (B1), (E7.1) + (A4.1) + (A4.2) + (B1);
    (E7.1) + (A1.1) + (A1.2) + (B2), (E7.1) + (A1.1) + (A2.1) + (B2), (E7.1) + (A1.1) + (A2.2) + (B2), (E7.1) + (A1.1) + (A3.1) + (B2), (E7.1) + (A1.1) + (A3.2) + (B2), (E7.1) + (A1.1) + (A4.1) + (B2), (E7.1) + (A1.1) + (A4.2) + (B2);
    (E7.1) + (A1.2) + (A2.1) + (B2), (E7.1) + (A1.2) + (A2.2) + (B2), (E7.1) + (A1.2) + (A3.1) + (B2), (E7.1) + (A1.2) + (A3.2) + (B2), (E7.1) + (A1.2) + (A4.1) + (B2), (E7.1) + (A1.2) + (A4.2) + (B2);
    (E7.1) + (A2.1) + (A2.2) + (B2), (E7.1) + (A2.1) + (A3.1) + (B2), (E7.1) + (A2.1) + (A3.2) + (B2), (E7.1) + (A2.1) + (A4.1) + (B2), (E7.1) + (A2.1) + (A4.2) + (B2);
    (E7.1) + (A2.2) + (A3.1) + (B2), (E7.1) + (A2.2) + (A3.2) + (B2), (E7.1) + (A2.2) + (A4.1) + (B2), (E7.1) + (A2.2) + (A4.2) + (B2);
    (E7.1) + (A3.1) + (A3.2) + (B2), (E7.1) + (A3.1) + (A4.1) + (B2), (E7.1) + (A3.1) + (A4.2) + (B2); (E7.1) + (A3.2) + (A4.1) + (B2), (E7.1) + (A3.2) + (A4.2) + (B2), (E7.1) + (A4.1) + (A4.2) + (B2);
    (E7.1) + (A1.1) + (A1.2) + (B3), (E7.1) + (A1.1) + (A2.1) + (B3), (E7.1) + (A1.1) + (A2.2) + (B3), (E7.1) + (A1.1) + (A3.1) + (B3), (E7.1) + (A1.1) + (A3.2) + (B3), (E7.1) + (A1.1) + (A4.1) + (B3), (E7.1) + (A1.1) + (A4.2) + (B3);
    (E7.1) + (A1.2) + (A2.1) + (B3), (E7.1) + (A1.2) + (A2.2) + (B3), (E7.1) + (A1.2) + (A3.1) + (B3), (E7.1) + (A1.2) + (A3.2) + (B3), (E7.1) + (A1.2) + (A4.1) + (B3), (E7.1) + (A1.2) + (A4.2) + (B3);
    (E7.1) + (A2.1) + (A2.2) + (B3), (E7.1) + (A2.1) + (A3.1) + (B3), (E7.1) + (A2.1) + (A3.2) + (B3), (E7.1) + (A2.1) + (A4.1) + (B3), (E7.1) + (A2.1) + (A4.2) + (B3);
    (E7.1) + (A2.2) + (A3.1) + (B3), (E7.1) + (A2.2) + (A3.2) + (B3), (E7.1) + (A2.2) + (A4.1) + (B3), (E7.1) + (A2.2) + (A4.2) + (B3);
    (E7.1) + (A3.1) + (A3.2) + (B3), (E7.1) + (A3.1) + (A4.1) + (B3), (E7.1) + (A3.1) + (A4.2) + (B3); (E7.1) + (A3.2) + (A4.1) + (B3), (E7.1) + (A3.2) + (A4.2) + (B3), (E7.1) + (A4.1) + (A4.2) + (B3);
    (E7.2) + (A1.1) + (B1), (E7.2) + (A1.1) + (B2), (E7.2) + (A1.1) + (B3), (E7.2) + (A2.1) + (B1), (E7.2) + (A2.1) + (B2), (E7.2) + (A2.1) + (B3), (E7.2) + (A3.1) + (B1), (E7.2) + (A3.1) + (B2), (E7.2) + (A3.1) + (B3), (E7.2) + (A4.1) + (B1), (E7.2) + (A4.1) + (B2), (E7.2) + (A4.1) + (B3), (E7.2) + (A1.2) + (B1), (E7.2) + (A1.2) + (B2), (E7.2) + (A1.2) + (B3), (E7.2) + (A2.2) + (B1), (E7.2) + (A2.2) + (B2), (E7.2) + (A2.2) + (B3), (E7.2) + (A3.2) + (B1), (E7.2) + (A3.2) + (B2), (E7.2) + (A3.2) + (B3), (E7.2) + (A4.2) + (B1), (E7.2) + (A4.2) + (B2), (E7.2) + (A4.2) + (B3),
    (E7.2) + (A1.1) + (A1.2) + (B1), (E7.2) + (A1.1) + (A2.1) + (B1), (E7.2) + (A1.1) + (A2.2) + (B1), (E7.2) + (A1.1) + (A3.1) + (B1), (E7.2) + (A1.1) + (A3.2) + (B1), (E7.2) + (A1.1) + (A4.1) + (B1), (E7.2) + (A1.1) + (A4.2) + (B1);
    (E7.2) + (A1.2) + (A2.1) + (B1), (E7.2) + (A1.2) + (A2.2) + (B1), (E7.2) + (A1.2) + (A3.1) + (B1), (E7.2) + (A1.2) + (A3.2) + (B1), (E7.2) + (A1.2) + (A4.1) + (B1), (E7.2) + (A1.2) + (A4.2) + (B1);
    (E7.2) + (A2.1) + (A2.2) + (B1), (E7.2) + (A2.1) + (A3.1) + (B1), (E7.2) + (A2.1) + (A3.2) + (B1), (E7.2) + (A2.1) + (A4.1) + (B1), (E7.2) + (A2.1) + (A4.2) + (B1);
    (E7.2) + (A2.2) + (A3.1) + (B1), (E7.2) + (A2.2) + (A3.2) + (B1), (E7.2) + (A2.2) + (A4.1) + (B1), (E7.2) + (A2.2) + (A4.2) + (B1);
    (E7.2) + (A3.1) + (A3.2) + (B1), (E7.2) + (A3.1) + (A4.1) + (B1), (E7.2) + (A3.1) + (A4.2) + (B1); (E7.2) + (A3.2) + (A4.1) + (B1), (E7.2) + (A3.2) + (A4.2) + (B1), (E7.2) + (A4.1) + (A4.2) + (B1);
    (E7.2) + (A1.1) + (A1.2) + (B2), (E7.2) + (A1.1) + (A2.1) + (B2), (E7.2) + (A1.1) + (A2.2) + (B2), (E7.2) + (A1.1) + (A3.1) + (B2), (E7.2) + (A1.1) + (A3.2) + (B2), (E7.2) + (A1.1) + (A4.1) + (B2), (E7.2) + (A1.1) + (A4.2) + (B2);
    (E7.2) + (A1.2) + (A2.1) + (B2), (E7.2) + (A1.2) + (A2.2) + (B2), (E7.2) + (A1.2) + (A3.1) + (B2), (E7.2) + (A1.2) + (A3.2) + (B2), (E7.2) + (A1.2) + (A4.1) + (B2), (E7.2) + (A1.2) + (A4.2) + (B2);
    (E7.2) + (A2.1) + (A2.2) + (B2), (E7.2) + (A2.1) + (A3.1) + (B2), (E7.2) + (A2.1) + (A3.2) + (B2), (E7.2) + (A2.1) + (A4.1) + (B2), (E7.2) + (A2.1) + (A4.2) + (B2); (E7.2) + (A2.2) + (A3.1) + (B2), (E7.2) + (A2.2) + (A3.2) + (B2), (E7.2) + (A2.2) + (A4.1) + (B2), (E7.2) + (A2.2) + (A4.2) + (B2);
    (E7.2) + (A3.1) + (A3.2) + (B2), (E7.2) + (A3.1) + (A4.1) + (B2), (E7.2) + (A3.1) + (A4.2) + (B2); (E7.2) + (A3.2) + (A4.1) + (B2), (E7.2) + (A3.2) + (A4.2) + (B2), (E7.2) + (A4.1) + (A4.2) + (B2);
    (E7.2) + (A1.1) + (A1.2) + (B3), (E7.2) + (A1.1) + (A2.1) + (B3), (E7.2) + (A1.1) + (A2.2) + (B3), (E7.2) + (A1.1) + (A3.1) + (B3), (E7.2) + (A1.1) + (A3.2) + (B3), (E7.2) + (A1.1) + (A4.1) + (B3), (E7.2) + (A1.1) + (A4.2) + (B3);
    (E7.2) + (A1.2) + (A2.1) + (B3), (E7.2) + (A1.2) + (A2.2) + (B3), (E7.2) + (A1.2) + (A3.1) + (B3), (E7.2) + (A1.2) + (A3.2) + (B3), (E7.2) + (A1.2) + (A4.1) + (B3), (E7.2) + (A1.2) + (A4.2) + (B3);
    (E7.2) + (A2.1) + (A2.2) + (B3), (E7.2) + (A2.1) + (A3.1) + (B3), (E7.2) + (A2.1) + (A3.2) + (B3), (E7.2) + (A2.1) + (A4.1) + (B3), (E7.2) + (A2.1) + (A4.2) + (B3);
    (E7.2) + (A2.2) + (A3.1) + (B3), (E7.2) + (A2.2) + (A3.2) + (B3), (E7.2) + (A2.2) + (A4.1) + (B3), (E7.2) + (A2.2) + (A4.2) + (B3);
    (E7.2) + (A3.1) + (A3.2) + (B3), (E7.2) + (A3.1) + (A4.1) + (B3), (E7.2) + (A3.1) + (A4.2) + (B3); (E7.2) + (A3.2) + (A4.1) + (B3), (E7.2) + (A3.2) + (A4.2) + (B3), (E7.2) + (A4.1) + (A4.2) + (B3);
    (E8) + (A1.1) + (B1), (E8) + (A1.1) + (B2), (E8) + (A1.1) + (B3), (E8) + (A2.1) + (B1), (E8) + (A2.1) + (B2), (E8) + (A2.1) + (B3), (E8) + (A3.1) + (B1), (E8) + (A3.1) + (B2), (E8) + (A3.1) + (B3), (E8) + (A4.1) + (B1), (E8) + (A4.1) + (B2), (E8) + (A4.1) + (B3), (E8) + (A1.2) + (B1), (E8) + (A1.2) + (B2), (E8) + (A1.2) + (B3), (E8) + (A2.2) + (B1), (E8) + (A2.2) + (B2), (E8) + (A2.2) + (B3), (E8) + (A3.2) + (B1), (E8) + (A3.2) + (B2), (E8) + (A3.2) + (B3), (E8) + (A4.2) + (B1), (E8) + (A4.2) + (B2), (E8) + (A4.2) + (B3), (E8) + (A1.1) + (A1.2) + (B1), (E8) + (A1.1) + (A2.1) + (B1), (E8) + (A1.1) + (A2.2) + (B1), (E8) + (A1.1) + (A3.1) + (B1), (E8) + (A1.1) + (A3.2) + (B1), (E8) + (A1.1) + (A4.1) + (B1), (E8) + (A1.1) + (A4.2) + (B1);
    (E8) + (A1.2) + (A2.1) + (B1), (E8) + (A1.2) + (A2.2) + (B1), (E8) + (A1.2) + (A3.1) + (B1), (E8) + (A1.2) + (A3.2) + (B1), (E8) + (A1.2) + (A4.1) + (B1), (E8) + (A1.2) + (A4.2) + (B1);
    (E8) + (A2.1) + (A2.2) + (B1), (E8) + (A2.1) + (A3.1) + (B1), (E8) + (A2.1) + (A3.2) + (B1), (E8) + (A2.1) + (A4.1) + (B1), (E8) + (A2.1) + (A4.2) + (B1);
    (E8) + (A2.2) + (A3.1) + (B1), (E8) + (A2.2) + (A3.2) + (B1), (E8) + (A2.2) + (A4.1) + (B1), (E8) + (A2.2) + (A4.2) + (B1);
    (E8) + (A3.1) + (A3.2) + (B1), (E8) + (A3.1) + (A4.1) + (B1), (E8) + (A3.1) + (A4.2) + (B1); (E8) + (A3.2) + (A4.1) + (B1), (E8) + (A3.2) + (A4.2) + (B1), (E8) + (A4.1) + (A4.2) + (B1);
    (E8) + (A1.1) + (A1.2) + (B2), (E8) + (A1.1) + (A2.1) + (B2), (E8) + (A1.1) + (A2.2) + (B2), (E8) + (A1.1) + (A3.1) + (B2), (E8) + (A1.1) + (A3.2) + (B2), (E8) + (A1.1) + (A4.1) + (B2), (E8) + (A1.1) + (A4.2) + (B2);
    (E8) + (A1.2) + (A2.1) + (B2), (E8) + (A1.2) + (A2.2) + (B2), (E8) + (A1.2) + (A3.1) + (B2), (E8) + (A1.2) + (A3.2) + (B2), (E8) + (A1.2) + (A4.1) + (B2), (E8) + (A1.2) + (A4.2) + (B2);
    (E8) + (A2.1) + (A2.2) + (B2), (E8) + (A2.1) + (A3.1) + (B2), (E8) + (A2.1) + (A3.2) + (B2), (E8) + (A2.1) + (A4.1) + (B2), (E8) + (A2.1) + (A4.2) + (B2);
    (E8) + (A2.2) + (A3.1) + (B2), (E8) + (A2.2) + (A3.2) + (B2), (E8) + (A2.2) + (A4.1) + (B2), (E8) + (A2.2) + (A4.2) + (B2);
    (E8) + (A3.1) + (A3.2) + (B2), (E8) + (A3.1) + (A4.1) + (B2), (E8) + (A3.1) + (A4.2) + (B2); (E8) + (A3.2) + (A4.1) + (B2), (E8) + (A3.2) + (A4.2) + (B2), (E8) + (A4.1) + (A4.2) + (B2);
    (E8) + (A1.1) + (A1.2) + (B3), (E8) + (A1.1) + (A2.1) + (B3), (E8) + (A1.1) + (A2.2) + (B3), (E8) + (A1.1) + (A3.1) + (B3), (E8) + (A1.1) + (A3.2) + (B3), (E8) + (A1.1) + (A4.1) + (B3), (E8) + (A1.1) + (A4.2) + (B3);
    (E8) + (A1.2) + (A2.1) + (B3), (E8) + (A1.2) + (A2.2) + (B3), (E8) + (A1.2) + (A3.1) + (B3), (E8) + (A1.2) + (A3.2) + (B3), (E8) + (A1.2) + (A4.1) + (B3), (E8) + (A1.2) + (A4.2) + (B3);
    (E8) + (A2.1) + (A2.2) + (B3), (E8) + (A2.1) + (A3.1) + (B3), (E8) + (A2.1) + (A3.2) + (B3), (E8) + (A2.1) + (A4.1) + (B3), (E8) + (A2.1) + (A4.2) + (B3);
    (E8) + (A2.2) + (A3.1) + (B3), (E8) + (A2.2) + (A3.2) + (B3), (E8) + (A2.2) + (A4.1) + (B3), (E8) + (A2.2) + (A4.2) + (B3);
    (E8) + (A3.1) + (A3.2) + (B3), (E8) + (A3.1) + (A4.1) + (B3), (E8) + (A3.1) + (A4.2) + (B3); (E8) + (A3.2) + (A4.1) + (B3), (E8) + (A3.2) + (A4.2) + (B3), (E8) + (A4.1) + (A4.2) + (B3);
    (E8.1) + (A1.1) + (B1), (E8.1) + (A1.1) + (B2), (E8.1) + (A1.1) + (B3), (E8.1) + (A2.1) + (B1), (E8.1) + (A2.1) + (B2), (E8.1) + (A2.1) + (B3), (E8.1) + (A3.1) + (B1), (E8.1) + (A3.1) + (B2), (E8.1) + (A3.1) + (B3), (E8.1) + (A4.1) + (B1), (E8.1) + (A4.1) + (B2), (E8.1) + (A4.1) + (B3), (E8.1) + (A1.2) + (B1), (E8.1) + (A1.2) + (B2), (E8.1) + (A1.2) + (B3), (E8.1) + (A2.2) + (B1), (E8.1) + (A2.2) + (B2), (E8.1) + (A2.2) + (B3), (E8.1) + (A3.2) + (B1), (E8.1) + (A3.2) + (B2), (E8.1) + (A3.2) + (B3), (E8.1) + (A4.2) + (B1), (E8.1) + (A4.2) + (B2), (E8.1) + (A4.2) + (B3),
    (E8.1) + (A1.1) + (A1.2) + (B1), (E8.1) + (A1.1) + (A2.1) + (B1), (E8.1) + (A1.1) + (A2.2) + (B1), (E8.1) + (A1.1) + (A3.1) + (B1), (E8.1) + (A1.1) + (A3.2) + (B1), (E8.1) + (A1.1) + (A4.1) + (B1), (E8.1) + (A1.1) + (A4.2) + (B1);
    (E8.1) + (A1.2) + (A2.1) + (B1), (E8.1) + (A1.2) + (A2.2) + (B1), (E8.1) + (A1.2) + (A3.1) + (B1), (E8.1) + (A1.2) + (A3.2) + (B1), (E8.1) + (A1.2) + (A4.1) + (B1), (E8.1) + (A1.2) + (A4.2) + (B1);
    (E8.1) + (A2.1) + (A2.2) + (B1), (E8.1) + (A2.1) + (A3.1) + (B1), (E8.1) + (A2.1) + (A3.2) + (B1), (E8.1) + (A2.1) + (A4.1) + (B1), (E8.1) + (A2.1) + (A4.2) + (B1);
    (E8.1) + (A2.2) + (A3.1) + (B1), (E8.1) + (A2.2) + (A3.2) + (B1), (E8.1) + (A2.2) + (A4.1) + (B1), (E8.1) + (A2.2) + (A4.2) + (B1);
    (E8.1) + (A3.1) + (A3.2) + (B1), (E8.1) + (A3.1) + (A4.1) + (B1), (E8.1) + (A3.1) + (A4.2) + (B1); (E8.1) + (A3.2) + (A4.1) + (B1), (E8.1) + (A3.2) + (A4.2) + (B1), (E8.1) + (A4.1) + (A4.2) + (B1);
    (E8.1) + (A1.1) + (A1.2) + (B2), (E8.1) + (A1.1) + (A2.1) + (B2), (E8.1) + (A1.1) + (A2.2) + (B2), (E8.1) + (A1.1) + (A3.1) + (B2), (E8.1) + (A1.1) + (A3.2) + (B2), (E8.1) + (A1.1) + (A4.1) + (B2), (E8.1) + (A1.1) + (A4.2) + (B2);
    (E8.1) + (A1.2) + (A2.1) + (B2), (E8.1) + (A1.2) + (A2.2) + (B2), (E8.1) + (A1.2) + (A3.1) + (B2), (E8.1) + (A1.2) + (A3.2) + (B2), (E8.1) + (A1.2) + (A4.1) + (B2), (E8.1) + (A1.2) + (A4.2) + (B2);
    (E8.1) + (A2.1) + (A2.2) + (B2), (E8.1) + (A2.1) + (A3.1) + (B2), (E8.1) + (A2.1) + (A3.2) + (B2), (E8.1) + (A2.1) + (A4.1) + (B2), (E8.1) + (A2.1) + (A4.2) + (B2); (E8.1) + (A2.2) + (A3.1) + (B2), (E8.1) + (A2.2) + (A3.2) + (B2), (E8.1) + (A2.2) + (A4.1) + (B2), (E8.1) + (A2.2) + (A4.2) + (B2);
    (E8.1) + (A3.1) + (A3.2) + (B2), (E8.1) + (A3.1) + (A4.1) + (B2), (E8.1) + (A3.1) + (A4.2) + (B2); (E8.1) + (A3.2) + (A4.1) + (B2), (E8.1) + (A3.2) + (A4.2) + (B2), (E8.1) + (A4.1) + (A4.2) + (B2);
    (E8.1) + (A1.1) + (A1.2) + (B3), (E8.1) + (A1.1) + (A2.1) + (B3), (E8.1) + (A1.1) + (A2.2) + (B3), (E8.1) + (A1.1) + (A3.1) + (B3), (E8.1) + (A1.1) + (A3.2) + (B3), (E8.1) + (A1.1) + (A4.1) + (B3), (E8.1) + (A1.1) + (A4.2) + (B3);
    (E8.1) + (A1.2) + (A2.1) + (B3), (E8.1) + (A1.2) + (A2.2) + (B3), (E8.1) + (A1.2) + (A3.1) + (B3), (E8.1) + (A1.2) + (A3.2) + (B3), (E8.1) + (A1.2) + (A4.1) + (B3), (E8.1) + (A1.2) + (A4.2) + (B3);
    (E8.1) + (A2.1) + (A2.2) + (B3), (E8.1) + (A2.1) + (A3.1) + (B3), (E8.1) + (A2.1) + (A3.2) + (B3), (E8.1) + (A2.1) + (A4.1) + (B3), (E8.1) + (A2.1) + (A4.2) + (B3); (E8.1) + (A2.2) + (A3.1) + (B3), (E8.1) + (A2.2) + (A3.2) + (B3), (E8.1) + (A2.2) + (A4.1) + (B3), (E8.1) + (A2.2) + (A4.2) + (B3);
    (E8.1) + (A3.1) + (A3.2) + (B3), (E8.1) + (A3.1) + (A4.1) + (B3), (E8.1) + (A3.1) + (A4.2) + (B3); (E8.1) + (A3.2) + (A4.1) + (B3), (E8.1) + (A3.2) + (A4.2) + (B3), (E8.1) + (A4.1) + (A4.2) + (B3);
    (E8.2) + (A1.1) + (B1), (E8.2) + (A1.1) + (B2), (E8.2) + (A1.1) + (B3), (E8.2) + (A2.1) + (B1), (E8.2) + (A2.1) + (B2), (E8.2) + (A2.1) + (B3), (E8.2) + (A3.1) + (B1), (E8.2) + (A3.1) + (B2), (E8.2) + (A3.1) + (B3), (E8.2) + (A4.1) + (B1), (E8.2) + (A4.1) + (B2), (E8.2) + (A4.1) + (B3), (E8.2) + (A1.2) + (B1), (E8.2) + (A1.2) + (B2), (E8.2) + (A1.2) + (B3), (E8.2) + (A2.2) + (B1), (E8.2) + (A2.2) + (B2), (E8.2) + (A2.2) + (B3), (E8.2) + (A3.2) + (B1), (E8.2) + (A3.2) + (B2), (E8.2) + (A3.2) + (B3), (E8.2) + (A4.2) + (B1), (E8.2) + (A4.2) + (B2), (E8.2) + (A4.2) + (B3),
    (E8.2) + (A1.1) + (A1.2) + (B1), (E8.2) + (A1.1) + (A2.1) + (B1), (E8.2) + (A1.1) + (A2.2) + (B1), (E8.2) + (A1.1) + (A3.1) + (B1), (E8.2) + (A1.1) + (A3.2) + (B1), (E8.2) + (A1.1) + (A4.1) + (B1), (E8.2) + (A1.1) + (A4.2) + (B1);
    (E8.2) + (A1.2) + (A2.1) + (B1), (E8.2) + (A1.2) + (A2.2) + (B1), (E8.2) + (A1.2) + (A3.1) + (B1), (E8.2) + (A1.2) + (A3.2) + (B1), (E8.2) + (A1.2) + (A4.1) + (B1), (E8.2) + (A1.2) + (A4.2) + (B1);
    (E8.2) + (A2.1) + (A2.2) + (B1), (E8.2) + (A2.1) + (A3.1) + (B1), (E8.2) + (A2.1) + (A3.2) + (B1), (E8.2) + (A2.1) + (A4.1) + (B1), (E8.2) + (A2.1) + (A4.2) + (B1);
    (E8.2) + (A2.2) + (A3.1) + (B1), (E8.2) + (A2.2) + (A3.2) + (B1), (E8.2) + (A2.2) + (A4.1) + (B1), (E8.2) + (A2.2) + (A4.2) + (B1);
    (E8.2) + (A3.1) + (A3.2) + (B1), (E8.2) + (A3.1) + (A4.1) + (B1), (E8.2) + (A3.1) + (A4.2) + (B1); (E8.2) + (A3.2) + (A4.1) + (B1), (E8.2) + (A3.2) + (A4.2) + (B1), (E8.2) + (A4.1) + (A4.2) + (B1);
    (E8.2) + (A1.1) + (A1.2) + (B2), (E8.2) + (A1.1) + (A2.1) + (B2), (E8.2) + (A1.1) + (A2.2) + (B2), (E8.2) + (A1.1) + (A3.1) + (B2), (E8.2) + (A1.1) + (A3.2) + (B2), (E8.2) + (A1.1) + (A4.1) + (B2), (E8.2) + (A1.1) + (A4.2) + (B2);
    (E8.2) + (A1.2) + (A2.1) + (B2), (E8.2) + (A1.2) + (A2.2) + (B2), (E8.2) + (A1.2) + (A3.1) + (B2), (E8.2) + (A1.2) + (A3.2) + (B2), (E8.2) + (A1.2) + (A4.1) + (B2), (E8.2) + (A1.2) + (A4.2) + (B2);
    (E8.2) + (A2.1) + (A2.2) + (B2), (E8.2) + (A2.1) + (A3.1) + (B2), (E8.2) + (A2.1) + (A3.2) + (B2), (E8.2) + (A2.1) + (A4.1) + (B2), (E8.2) + (A2.1) + (A4.2) + (B2);
    (E8.2) + (A2.2) + (A3.1) + (B2), (E8.2) + (A2.2) + (A3.2) + (B2), (E8.2) + (A2.2) + (A4.1) + (B2), (E8.2) + (A2.2) + (A4.2) + (B2);
    (E8.2) + (A3.1) + (A3.2) + (B2), (E8.2) + (A3.1) + (A4.1) + (B2), (E8.2) + (A3.1) + (A4.2) + (B2); (E8.2) + (A3.2) + (A4.1) + (B2), (E8.2) + (A3.2) + (A4.2) + (B2), (E8.2) + (A4.1) + (A4.2) + (B2);
    (E8.2) + (A1.1) + (A1.2) + (B3), (E8.2) + (A1.1) + (A2.1) + (B3), (E8.2) + (A1.1) + (A2.2) + (B3), (E8.2) + (A1.1) + (A3.1) + (B3), (E8.2) + (A1.1) + (A3.2) + (B3), (E8.2) + (A1.1) + (A4.1) + (B3), (E8.2) + (A1.1) + (A4.2) + (B3);
    (E8.2) + (A1.2) + (A2.1) + (B3), (E8.2) + (A1.2) + (A2.2) + (B3), (E8.2) + (A1.2) + (A3.1) + (B3), (E8.2) + (A1.2) + (A3.2) + (B3), (E8.2) + (A1.2) + (A4.1) + (B3), (E8.2) + (A1.2) + (A4.2) + (B3);
    (E8.2) + (A2.1) + (A2.2) + (B3), (E8.2) + (A2.1) + (A3.1) + (B3), (E8.2) + (A2.1) + (A3.2) + (B3), (E8.2) + (A2.1) + (A4.1) + (B3), (E8.2) + (A2.1) + (A4.2) + (B3); (E8.2) + (A2.2) + (A3.1) + (B3), (E8.2) + (A2.2) + (A3.2) + (B3), (E8.2) + (A2.2) + (A4.1) + (B3), (E8.2) + (A2.2) + (A4.2) + (B3);
    (E8.2) + (A3.1) + (A3.2) + (B3), (E8.2) + (A3.1) + (A4.1) + (B3), (E8.2) + (A3.1) + (A4.2) + (B3); (E8.2) + (A3.2) + (A4.1) + (B3), (E8.2) + (A3.2) + (A4.2) + (B3), (E8.2) + (A4.1) + (A4.2) + (B3);
    (E9) + (A1.1) + (B1), (E9) + (A1.1) + (B2), (E9) + (A1.1) + (B3), (E9) + (A2.1) + (B1), (E9) + (A2.1) + (B2), (E9) + (A2.1) + (B3), (E9) + (A3.1) + (B1), (E9) + (A3.1) + (B2), (E9) + (A3.1) + (B3), (E9) + (A4.1) + (B1), (E9) + (A4.1) + (B2), (E9) + (A4.1) + (B3), (E9) + (A1.2) + (B1), (E9) + (A1.2) + (B2), (E9) + (A1.2) + (B3), (E9) + (A2.2) + (B1), (E9) + (A2.2) + (B2), (E9) + (A2.2) + (B3), (E9) + (A3.2) + (B1), (E9) + (A3.2) + (B2), (E9) + (A3.2) + (B3), (E9) + (A4.2) + (B1), (E9) + (A4.2) + (B2), (E9) + (A4.2) + (B3), (E9) + (A1.1) + (A1.2) + (B1), (E9) + (A1.1) + (A2.1) + (B1), (E9) + (A1.1) + (A2.2) + (B1), (E9) + (A1.1) + (A3.1) + (B1), (E9) + (A1.1) + (A3.2) + (B1), (E9) + (A1.1) + (A4.1) + (B1), (E9) + (A1.1) + (A4.2) + (B1);
    (E9) + (A1.2) + (A2.1) + (B1), (E9) + (A1.2) + (A2.2) + (B1), (E9) + (A1.2) + (A3.1) + (B1), (E9) + (A1.2) + (A3.2) + (B1), (E9) + (A1.2) + (A4.1) + (B1), (E9) + (A1.2) + (A4.2) + (B1);
    (E9) + (A2.1) + (A2.2) + (B1), (E9) + (A2.1) + (A3.1) + (B1), (E9) + (A2.1) + (A3.2) + (B1), (E9) + (A2.1) + (A4.1) + (B1), (E9) + (A2.1) + (A4.2) + (B1);
    (E9) + (A2.2) + (A3.1) + (B1), (E9) + (A2.2) + (A3.2) + (B1), (E9) + (A2.2) + (A4.1) + (B1), (E9) + (A2.2) + (A4.2) + (B1);
    (E9) + (A3.1) + (A3.2) + (B1), (E9) + (A3.1) + (A4.1) + (B1), (E9) + (A3.1) + (A4.2) + (B1); (E9) + (A3.2) + (A4.1) + (B1), (E9) + (A3.2) + (A4.2) + (B1), (E9) + (A4.1) + (A4.2) + (B1);
    (E9) + (A1.1) + (A1.2) + (B2), (E9) + (A1.1) + (A2.1) + (B2), (E9) + (A1.1) + (A2.2) + (B2), (E9) + (A1.1) + (A3.1) + (B2), (E9) + (A1.1) + (A3.2) + (B2), (E9) + (A1.1) + (A4.1) + (B2), (E9) + (A1.1) + (A4.2) + (B2);
    (E9) + (A1.2) + (A2.1) + (B2), (E9) + (A1.2) + (A2.2) + (B2), (E9) + (A1.2) + (A3.1) + (B2), (E9) + (A1.2) + (A3.2) + (B2), (E9) + (A1.2) + (A4.1) + (B2), (E9) + (A1.2) + (A4.2) + (B2);
    (E9) + (A2.1) + (A2.2) + (B2), (E9) + (A2.1) + (A3.1) + (B2), (E9) + (A2.1) + (A3.2) + (B2), (E9) + (A2.1) + (A4.1) + (B2), (E9) + (A2.1) + (A4.2) + (B2);
    (E9) + (A2.2) + (A3.1) + (B2), (E9) + (A2.2) + (A3.2) + (B2), (E9) + (A2.2) + (A4.1) + (B2), (E9) + (A2.2) + (A4.2) + (B2);
    (E9) + (A3.1) + (A3.2) + (B2), (E9) + (A3.1) + (A4.1) + (B2), (E9) + (A3.1) + (A4.2) + (B2), (E9) + (A3.2) + (A4.1) + (B2), (E9) + (A3.2) + (A4.2) + (B2), (E9) + (A4.1) + (A4.2) + (B2);
    (E9) + (A1.1) + (A1.2) + (B3), (E9) + (A1.1) + (A2.1) + (B3), (E9) + (A1.1) + (A2.2) + (B3), (E9) + (A1.1) + (A3.1) + (B3), (E9) + (A1.1) + (A3.2) + (B3), (E9) + (A1.1) + (A4.1) + (B3), (E9) + (A1.1) + (A4.2) + (B3);
    (E9) + (A1.2) + (A2.1) + (B3), (E9) + (A1.2) + (A2.2) + (B3), (E9) + (A1.2) + (A3.1) + (B3), (E9) + (A1.2) + (A3.2) + (B3), (E9) + (A1.2) + (A4.1) + (B3), (E9) + (A1.2) + (A4.2) + (B3);
    (E9) + (A2.1) + (A2.2) + (B3), (E9) + (A2.1) + (A3.1) + (B3), (E9) + (A2.1) + (A3.2) + (B3), (E9) + (A2.1) + (A4.1) + (B3), (E9) + (A2.1) + (A4.2) + (B3);
    (E9) + (A2.2) + (A3.1) + (B3), (E9) + (A2.2) + (A3.2) + (B3), (E9) + (A2.2) + (A4.1) + (B3), (E9) + (A2.2) + (A4.2) + (B3);
    (E9) + (A3.1) + (A3.2) + (B3), (E9) + (A3.1) + (A4.1) + (B3), (E9) + (A3.1) + (A4.2) + (B3); (E9) + (A3.2) + (A4.1) + (B3), (E9) + (A3.2) + (A4.2) + (B3), (E9) + (A4.1) + (A4.2) + (B3);
    (E9.1) + (A1.1) + (B1), (E9.1) + (A1.1) + (B2), (E9.1) + (A1.1) + (B3), (E9.1) + (A2.1) + (B1), (E9.1) + (A2.1) + (B2), (E9.1) + (A2.1) + (B3), (E9.1) + (A3.1) + (B1), (E9.1) + (A3.1) + (B2), (E9.1) + (A3.1) + (B3), (E9.1) + (A4.1) + (B1), (E9.1) + (A4.1) + (B2), (E9.1) + (A4.1) + (B3), (E9.1) + (A1.2) + (B1), (E9.1) + (A1.2) + (B2), (E9.1) + (A1.2) + (B3), (E9.1) + (A2.2) + (B1), (E9.1) + (A2.2) + (B2), (E9.1) + (A2.2) + (B3), (E9.1) + (A3.2) + (B1), (E9.1) + (A3.2) + (B2), (E9.1) + (A3.2) + (B3), (E9.1) + (A4.2) + (B1), (E9.1) + (A4.2) + (B2), (E9.1) + (A4.2) + (B3),
    (E9.1) + (A1.1) + (A1.2) + (B1), (E9.1) + (A1.1) + (A2.1) + (B1), (E9.1) + (A1.1) + (A2.2) + (B1), (E9.1) + (A1.1) + (A3.1) + (B1), (E9.1) + (A1.1) + (A3.2) + (B1), (E9.1) + (A1.1) + (A4.1) + (B1), (E9.1) + (A1.1) + (A4.2) + (B1);
    (E9.1) + (A1.2) + (A2.1) + (B1), (E9.1) + (A1.2) + (A2.2) + (B1), (E9.1) + (A1.2) + (A3.1) + (B1), (E9.1) + (A1.2) + (A3.2) + (B1), (E9.1) + (A1.2) + (A4.1) + (B1), (E9.1) + (A1.2) + (A4.2) + (B1);
    (E9.1) + (A2.1) + (A2.2) + (B1), (E9.1) + (A2.1) + (A3.1) + (B1), (E9.1) + (A2.1) + (A3.2) + (B1), (E9.1) + (A2.1) + (A4.1) + (B1), (E9.1) + (A2.1) + (A4.2) + (B1);
    (E9.1) + (A2.2) + (A3.1) + (B1), (E9.1) + (A2.2) + (A3.2) + (B1), (E9.1) + (A2.2) + (A4.1) + (B1), (E9.1) + (A2.2) + (A4.2) + (B1);
    (E9.1) + (A3.1) + (A3.2) + (B1), (E9.1) + (A3.1) + (A4.1) + (B1), (E9.1) + (A3.1) + (A4.2) + (B1); (E9.1) + (A3.2) + (A4.1) + (B1), (E9.1) + (A3.2) + (A4.2) + (B1), (E9.1) + (A4.1) + (A4.2) + (B1);
    (E9.1) + (A1.1) + (A1.2) + (B2), (E9.1) + (A1.1) + (A2.1) + (B2), (E9.1) + (A1.1) + (A2.2) + (B2), (E9.1) + (A1.1) + (A3.1) + (B2), (E9.1) + (A1.1) + (A3.2) + (B2), (E9.1) + (A1.1) + (A4.1) + (B2), (E9.1) + (A1.1) + (A4.2) + (B2);
    (E9.1) + (A1.2) + (A2.1) + (B2), (E9.1) + (A1.2) + (A2.2) + (B2), (E9.1) + (A1.2) + (A3.1) + (B2), (E9.1) + (A1.2) + (A3.2) + (B2), (E9.1) + (A1.2) + (A4.1) + (B2), (E9.1) + (A1.2) + (A4.2) + (B2);
    (E9.1) + (A2.1) + (A2.2) + (B2), (E9.1) + (A2.1) + (A3.1) + (B2), (E9.1) + (A2.1) + (A3.2) + (B2), (E9.1) + (A2.1) + (A4.1) + (B2), (E9.1) + (A2.1) + (A4.2) + (B2);
    (E9.1) + (A2.2) + (A3.1) + (B2), (E9.1) + (A2.2) + (A3.2) + (B2), (E9.1) + (A2.2) + (A4.1) + (B2), (E9.1) + (A22) + (A42) + (B2);
    (E9.1) + (A3.1) + (A3.2) + (B2), (E9.1) + (A3.1) + (A4.1) + (B2), (E9.1) + (A3.1) + (A4.2) + (B2); (E9.1) + (A3.2) + (A4.1) + (B2), (E9.1) + (A3.2) + (A4.2) + (B2), (E9.1) + (A4.1) + (A4.2) + (B2);
    (E9.1) + (A1.1) + (A1.2) + (B3), (E9.1) + (A1.1) + (A2.1) + (B3), (E9.1) + (A1.1) + (A22) + (B3), (E9.1) + (A1.1) + (A3.1) + (B3), (E9.1) + (A1.1) + (A3.2) + (B3), (E9.1) + (A1.1) + (A4.1) + (B3), (E9.1) + (A1.1) + (A4.2) + (B3);
    (E9.1) + (A1.2) + (A2.1) + (B3), (E9.1) + (A1.2) + (A2.2) + (B3), (E9.1) + (A1.2) + (A3.1) + (B3), (E9.1) + (A1.2) + (A3.2) + (B3), (E9.1) + (A1.2) + (A4.1) + (B3), (E9.1) + (A1.2) + (A4.2) + (B3);
    (E9.1) + (A2.1) + (A2.2) + (B3), (E9.1) + (A2.1) + (A3.1) + (B3), (E9.1) + (A2.1) + (A3.2) + (B3), (E9.1) + (A2.1) + (A4.1) + (B3), (E9.1) + (A2.1) + (A4.2) + (B3); (E9.1) + (A2.2) + (A3.1) + (B3), (E9.1) + (A2.2) + (A3.2) + (B3), (E9.1) + (A2.2) + (A4.1) + (B3), (E9.1) + (A2.2) + (A4.2) + (B3);
    (E9.1) + (A3.1) + (A3.2) + (B3), (E9.1) + (A3.1) + (A4.1) + (B3), (E9.1) + (A3.1) + (A4.2) + (B3); (E9.1) + (A3.2) + (A4.1) + (B3), (E9.1) + (A3.2) + (A4.2) + (B3), (E9.1) + (A4.1) + (A4.2) + (B3).
  • Sämtliche vorgenannten Kombinationen können auch mehrere agrochemische Wirkstoffe (E) enthalten, insbesondere zwei oder drei Wirkstoffe ausgewählt aus der Gruppe (E1), (E1.1), (E1.2), (E1.3), (E1.4), (E1.5), (E2), (E2.1), (E2.2), (E2.3), (E2.4), (E2.5), (E2.6), (E2.7), (E2.8), (E2.9), (E3), (E3.1), (E3.2), (E3.3), (E4), (E4.1), (E4.2), (E5), (E5.1), (E5.2), (E6), (E6.1), (E6.2), (E6.3), (E6.4), (E6.5), (E7), (E7.1), (E7.2), (E8), (E8.1), (E8.2), (E9), (E9.1).
  • Als übliche Hilfs- und Zusatzstoffe (Komponente F) können in den erfindungsgemäßen herbiziden Mittel z.B. noch enthalten sein: Tenside wie Emulgatoren und Dispergatoren, Verdickungs- und Thixotropiermittel, Netz-, Antidrift-, Haft-, Penetrations-, Konservierungs- und Frostschutzmittel, Antioxidantien, Lösungsvermittler, Füll-, Träger- und Farbstoffe, Entschäumer, Düngemittel, Verdunstungshemmer, sowie den pH-Wert und die Viskosität beeinflussende Mittel.
  • Als Emulgatoren und Dispergatoren kommen z.B. nichtionische Emulgatoren und Dispergatoren in Frage, z.B.:
    • 1) polyalkoxylierte, vorzugsweise polyethoxylierte, gesättigte und ungesättigte aliphatische Alkohole, • mit 8 bis 24 C-Atomen im Alkylrest, der sich von den entsprechenden Fettsäuren oder aus petrochemischen Produkten ableitet, und • mit 1 bis 100, vorzugsweise 2 bis 50, Ethylenoxideinheiten (EO), wobei die freie Hydroxy-Gruppe gegebenenfalls alkoxyliert ist, • die z. B. kommerziell als Genapol®X- und Genapol®O-Reihe (Clariant), Crovol®M-Reihe (Croda) oder Lutensol®Reihe (BASF) erhältlich sind,
    • 2) polyalkoxylierte, vorzugsweise polyethoxylierte Arylalkylphenole, wie z. B. 2, 4, 6-Tris-(1-phenylethyl)-phenol (Tristyrylphenol) mit einem mittleren Ethoxylierungsgrad zwischen 10 und 80, bevorzugt 16 bis 40, wie z. B. Soprophor®BSU (Rhodia) oder HOE S 3474 (Clariant),
    • 3) polyalkoxylierte, vorzugsweise polyethoxylierte Alkylphenole mit einem oder mehreren Alkylresten, wie z. B. Nonylphenol oder Tri-sec-butylphenol, und einem Ethoxylierungsgrad zwischen 2 und 40, bevorzugt 4 bis 15, wie z. B. Arkopal®N-Reihe oder Sapogenat®T-Reihe (Clariant),
    • 4) polyalkoxylierte, vorzugsweise polyethoxylierte Hydroxyfettsäuren oder Hydroxyfettsäuren enthaltene Glyceride, wie z. B. Ricinin bzw. Rizinusöl, mit einem Ethoxylierungsgrad zwischen 10 und 80, bevorzugt 25 bis 40, wie z. B. Emulsogen®EL-Reihe (Clariant) oder Agnique®CSO-Reihe (Cognis),
    • 5) polyalkoxylierte, vorzugsweise polyethoxylierte Sorbitanester, wie z. B. Atplus®309 F (Unigema) oder Alkamuls®-Reihe (Rhodia)
    • 6) Di- und Tri-block-copolymere, z.B. aus Alkylenoxiden, z.B. aus Ethylen- und Propylenoxid mit mittleren Molmassen zwischen 200 und 10000, vorzugsweise 1000 bis 4000 g/mol, wobei der Massenanteil des polyethoxylierte Blocks zwischen 10 und 80% variiert, wie z. B. Genapol®PF-Reihe (Clariant), Pluronic®-Reihe (BASF), oder Synperonic®PE-Reihe (Unigema),
  • Bevorzugte nichtionische Emulgatoren und Dispergatoren sind z.B. polyethoxylierte Alkohole, polyethoxylierte Triglyceride, die Hydroxyfettsäuren enthalten und Polyethylenoxid-Polypropylenoxid-Block-Copolymere.
  • Der Gesamtanteil an nichtionischen Emulgatoren und Dispergatoren in den erfindungsgemäßen herbiziden Mitteln liegt im allgemeinen zwischen 0 und 20 Gew.%. Werden nichtionische Emulgatoren und Dispergatoren, neben ihren emulgierenden/dispergierenden Eigenschaften, auch zur Erhöhung der biologischen Effektivität, z. B. als Penetrations- oder Haftmittel, eingesetzt, kann sich ihr Anteil in den erfindungsgemäßen herbiziden Mitteln auf bis zu 60 Gew.% erhöhen.
  • Es kommen auch ionische Emulgatoren und Dispergatoren in Frage, z.B.:
    • 1) polyalkoxy0lierte, vorzugsweise polyethoxylierte Emulgatoren/Dispergatoren (vgl. Komponente e), die ionisch modifiziert sind, z. B. durch Umsetzung der endständigen freien Hydroxylfunktion des Polyethylenoxidblocks zu einem Sulfat- oder Phosphatester (z. B. als Alkali- und Erdalkalimetallsalze), wie z. B. Genapol®LRO oder Dispergiermittel 3618 (Clariant), Emulphor® (BASF) oder Crafol®AP (Cognis),
    • 2) Alkali- und Erdalkalimetallsalze von Alkylarylsulfonsäuren mit linearer oder verzweigter Alkylkette, wie Phenylsulfonat CA oder Phenylsulfonat CAL (Clariant), Atlox® 3377BM (ICI), Empiphos®TM-Reihe (Huntsman)
    • 3) Polyelektrolyte, wie Ligninsulfonate, Kondensationsprodukte aus Naphthalinsulfonat und Formaldehyd, Polystyrolsulfonat oder sulfonierte ungesättigte oder aromatische Polymere (Polystyrole, Polybutadiene oder Polyterpene), wie Tamol®-Reihe (BASF), Morwet®D425 (Witco), Kraftsperse®-Reihe (Westvaco), Borresperse®-Reihe (Borregard).
  • Bevorzugte ionische Emulgatoren/Dispergatoren sind z.B. Salze von Alkylarylsulfonsäuren und Polyelektrolyte aus der Polykondensation von Naphthalinsulfonat und Formaldehyd.
  • Der Gesamtanteil an ionischen Emulgatoren und Dispergatoren in den erfindungsgemäßen herbiziden Mitteln liegt im allgemeinen zwischen 0 und 20 Gew.%, insbesondere zwischen 0 und 8 Gew.%.
  • Als Verdickungs- und Thixotropiermittel kommen z.B. in Frage:
    • 1) modifizierte natürliche Silikate, wie chemisch modifizierte Bentonite, Hectorite, Attapulgite, Montmorillonite, Smektite oder andere Silikatmineralien, wie Bentone® (Elementis), Attagel® (Engelhard), Agsorb® (Oil-Dri Corporation) oder Hectorite® (Akzo Nobel)
    • 2) synthetische Silikate, wie Silikate der Sipernat®-, Aerosil®- oder Durosil®-Reihe (Degussa), der CAB-O-SIL®-Reihe (Cabot) oder der Van Gel-Reihe (R.T. Vanderbilt),
    • 3) Verdicker auf Basis synthetischer Polymere, wie Verdicker der Thixin®- oder Thixatrol®-Reihe (Elementis).
    • 4) Verdicker auf Basis natürlicher Polymere und natürlicher Öle, z.B. aus der Thixin®- oder Thixatrol®-Reihe (Elementis).
  • Bevorzugte Verdickungs- und Thixotropiermittel sind z.B. modifizierte Schichtsilikate und Verdicker auf Basis synthetischer Polymere.
  • Der Anteil an Verdickungs- und Thixotropiermitteln in den erfindungsgemäßen herbiziden Mitteln liegt im allgemeinen zwischen 0 und 5 Gew.%, insbesondere zwischen 0, 2 und 3 Gew.%.
  • Die erfindungsgemäßen herbizid wirksamen Mittel lassen sich durch übliche, bereits bekannte Verfahren herstellen, z.B. durch Vermischen der verschiedenen Komponenten mit Hilfe von Rührern, Schüttlern, Mühlen oder (statischen) Mischern.
  • Dabei ist gegebenenfalls kurzzeitig ein Erwärmen der Gemische vorteilhaft, um ein vollständiges Auflösen aller involvierter Komponenten zu erzielen.
  • Bevorzugt sind erfindungsgemäße herbizid wirksame Mittel, enthaltend:
    • A) 0, 1 bis 30 Gew.-% eines oder mehrerer Sulfonylharnstoffe aus der Gruppe (A1.1), (A1.2), (A1.3), (A1.4), (A2.1), (A2.2), (A2.3), A2.4), (A3.1), (A3.2), (A3.3), (A3.4), (A4.1), (A4.2), vorzugsweise aus der Gruppe (A1.1), (A2.1), (A3.1), (A4.1),
    • B) 2 bis 40 Gew.-% eines oder mehrerer Safener aus der Gruppe (B1), (B2), (B3), (B4), (B5), (B6), (B7), vorzugsweise aus der Gruppe (B1), (B2), (B3), besonders bevorzugt (B1),
    • C) 20 bis 80 Gew.-% eines oder mehrerer Lösungsmittel, vorzugsweise aus der Gruppe der aliphatischen Kohlenwasserstoffe, der Gemische von aromatischen und aliphatischen Kohlenwasserstoffe und der Pflanzenöle wie Rapsölmethylester,
    • D) 0,5 bis 30 Gew.-% eines oder mehrerer Sulfosuccinate, vorzugsweise aus der Gruppe der Alkali Di(C4-C18)alkylsulfosuccinate wie Natrium Di(C4-C18)alkylsulfosuccinat,
    • E) 1 bis 20 Gew.-% eines oder mehrerer von A) und B) verschiedener agrochemischer Wirkstoffe,
    • F) 0 bis 40 Gew.-% an üblichen Hilfs- und Zusatzstoffen, vorzugsweise 0 bis 20 Gew.-% eines oder mehrerer nichtionischer Emulgatoren und Dispergatoren, 0 bis 8 Gew.-% eines oder mehrerer ionischer Emulgatoren und Dispergatoren, und 0 bis 3 Gew.-% eines oder mehrerer Verdickungs- und Thixotriopiermittel.
  • Gegenstand der vorliegenden Erfindung ist weiterhin ein Verfahren, das dadurch gekennzeichnet ist, daß die Komponenten (A) und (B) des erfindungsgemäßen herbizid wirksamen Mittels gemeinsam oder getrennt auf die Schadpflanzen, Kulturpflanzen, Pflanzensamen oder die Fläche auf der die Pflanzen wachsen, aufgebracht werden, gegebenenfalls in Kombination mit weiteren Komponenten, z.B. gemeinsam oder getrennt mit den Komponenten (C), (D), (E) und (F). Dabei kann die antidotisch wirksame Menge an einen oder mehreren Safenern, aus der Gruppe (B) vor, nach oder gleichzeitig mit dem(n) Sulfonylharnstoffen (A) auf die Pflanzen, Pflanzensamen oder die Fläche, auf der die Pflanzen wachsen, appliziert werden.
  • Die erfindungsgemäßen herbizid wirksamen Mittel können auch zur Bekämpfung von Schadpflanzen in Kulturen von bekannten oder noch zu entwickelnden gentechnisch veränderten Pflanzen eingesetzt werden. Die transgenen Pflanzen zeichnen sich in der Regel durch besondere vorteilhafte Eigenschaften aus, beispielsweise durch Resistenzen gegenüber bestimmten Pflanzenschutzmitteln, Resistenzen gegenüber Pflanzenkrankheiten oder Erregern von Pflanzenkrankheiten wie bestimmten Insekten oder Mikroorganismen wie Pilzen, Bakterien oder Viren. Andere besondere Eigenschaften betreffen z. B. das Erntegut hinsichtlich Menge, Qualität, Lagerfähigkeit, Zusammensetzung und spezieller Inhaltsstoffe. So sind transgene Pflanzen mit erhöhtem Stärkegehalt oder veränderter Qualität der Stärke oder solche mit anderer Fettsäurezusammensetzung des Ernteguts bekannt.
  • Bevorzugt ist die Anwendung der erfindungsgemäßen Kombinationen in wirtschaftlich bedeutenden transgenen Kulturen von Nutz- und Zierpflanzen, z. B. von Getreide (z.B. Weizen, Gerste, Roggen, Hafer), Hirse, Reis, Maniok und Mais oder auch Kulturen von Zuckerrübe, Baumwolle, Soja, Raps, Kartoffel, Tomate, Erbse und anderen Gemüsesorten.
  • Bei der Anwendung der erfindungsgemäßen Kombinationen in transgenen Kulturen treten neben den in anderen Kulturen zu beobachtenden Wirkungen gegenüber Schadpflanzen oftmals Wirkungen auf, die für die Applikation in der jeweiligen transgenen Kultur spezifisch sind, beispielsweise ein verändertes oder speziell erweitertes Unkrautspektrum, das bekämpft werden kann, veränderte Aufwandmengen, die für die Applikation eingesetzt werden können, vorzugsweise gute Kombinierbarkeit mit den Herbiziden, gegenüber denen die transgene Kultur resistent ist, sowie Beeinflussung von Wuchs und Ertrag der transgenen Kulturpflanzen.
  • Gegenstand der Erfindung ist deshalb auch die Verwendung des erfindungsgemäßen herbizid wirksamen Mittels zur Bekämpfung von Schadpflanzen in transgenen Kulturpflanzen oder Kulturpflanzen, die Toleranz durch Selektionszüchtung aufweisen.
  • Die Safener aus der Gruppe (B) und die Sulfonylharnstoffe (A) können gegebenenfalls in Kombination mit weiteren Komponenten, z.B. den Komponenten (C), (D), (E) und (F), auf verschiedene Art, gemeinsam oder getrennt formuliert werden, je nachdem welche biologischen und/oder chemisch-physikalischen Parameter vorgegeben sind. Als Formulierungsmöglichkeiten kommen beispielsweise in Frage:
    Spritzpulver (WP), emulgierbare Konzentrate (EC), wasserlösliche Pulver (SP), wasserlösliche Konzentrate (SL), konzentrierte Emulsionen (BW) wie Öl-in-Wasser und Wasser-in-Öl-Emulsionen, versprühbare Lösungen oder Emulsionen, Kapselsuspensionen (CS), Dispersionen auf Öl- oder Wasserbasis (SC), Suspoemulsionen, Suspensionskonzentrate, Stäubemittel (DP), ölmischbare Lösungen (OL), Beizmittel, Granulate (GR) in Form von Mikro-, Sprüh-, Aufzugs- und Adsorptionsgranulaten, Granulate für die Boden- bzw. Streuapplikation, wasserlösliche Granulate (SG), wasserdispergierbare Granulate (WG), ULV-Formulierungen, Mikrokapseln und Wachse.
  • Diese einzelnen Formulierungstypen sind im Prinzip bekannt und beispielsweise beschrieben in: Winnacker-Küchler, "Chemische Technologie" Band 7, C. Hauser Verlag München, 4. Aufl. 1986; Wade van Valkenburg, "Pesticide Formulations", Marcel Dekker N.Y., 1973; K. Martens, "Spray Drying Handbook", 3rd Ed. 1979, G. Goodwin Ltd. London.
  • Die gegebenenfalls notwendigen Formulierungshilfsmittel, wie Inertmaterialien, Tenside, Lösungsmittel und weitere Zusatzstoffe, sind ebenfalls bekannt und beispielsweise beschrieben in: Watkins, "Handbook of Insecticide Dust Diluents and Carriers", 2nd Ed., Darland Books, Caldwell N.J., H.v. Olphen, "Introduction to Clay Colloid Chemistry"; 2nd Ed., J. Wiley & Sons, N.Y.; C. Marsden, "Solvents Guide"; 2nd Ed., Interscience, N.Y. 1963; McCutcheon's "Detergents and Emulsifiers Annual", MC Publ. Corp., Ridgewood N.J.; Sisley and Wood, "Encyclopedia of Surface Active Agents", Chem. Publ. Co. Inc., N.Y. 1964; Schönfeldt, "Grenzflächenaktive Äthylenoxidaddukte", Wiss. Verlagsgesell., Stuttgart 1976; Winnacker-Küchler, "Chemische Technologie", Band 7, C. Hauser Verlag München, 4. Aufl. 1986.
  • Auf der Basis dieser Formulierungen lassen sich auch Kombinationen mit anderen agrochemischen Wirkstoffen herstellen, z.B. mit als Pflanzenschutzmittel wirksamen Stoffen, wie Insektiziden, Akariziden, Herbiziden, Fungiziden oder Safenern, Düngemitteln und/oder Wachstumsregulatoren, z.B. in Form einer Fertigformulierung oder als Tankmix.
  • Spritzpulver sind in Wasser gleichmäßig dispergierbare Präparate, die neben dem Wirkstoff außer einem Verdünnungs- oder Inertstoff noch Tenside ionischer und/oder nichtionischer Art (Netzmittel, Dispergiermittel), z.B. polyoxyethylierte Alkylphenole, polyoxethylierte Fettalkohole, polyoxethylierte Fettamine, Fettalkoholpolyglykolethersulfate, Alkansulfonate, Alkylbenzolsulfonate, ligninsulfonsaures Natrium, 2,2'-dinaphthylmethan-6,6'-disulfonsaures Natrium, dibutylnaphthalin-sulfonsaures Natrium oder auch oleoylmethyltaurinsaures Natrium enthalten. Zur Herstellung der Spritzpulver werden die Wirkstoffe z.B. die herbiziden Wirkstoffe und/oder die Safener beispielsweise in üblichen Apparaturen, wie Hammermühlen, Gebläsemühlen und Luftstrahlmühlen, feingemahlen und gleichzeitig oder anschließend mit den Formulierungshilfsmitteln vermischt.
  • Emulgierbare Konzentrate werden z.B. durch Auflösen des Wirkstoffes z.B. des herbiziden Wirkstoffs und/oder des Safeners in einem organischen Lösungsmittel, wie Butanol, Cyclohexanon, Dimethylformamid, Xylol oder auch höhersiedende Kohlenwasserstoffe wie Aromaten, gesättige oder ungesättigte Aliphaten oder Alicyclen, oder Mischungen der organischen Lösungsmittel unter Zusatz von einem oder mehreren Tensiden ionischer und/oder nichtionischer Art (Emulgatoren) hergestellt. Als Emulgatoren können beispielsweise verwendet werden: (C6-C18)-Alkylarylsulfonsaure Calzium-Salze, wie Ca-dodecylbenzolsulfonat, oder nichtionische Emulgatoren, wie Fettsäurepolyglykolester, (C2-C18)-Alkylarylpolyglykolether, Fettalkoholpolyglykolether, Propylenoxid-Ethylenoxid-Kondensationsprodukte, Alkylpolyether, Sorbitanester, wie Sorbitanfettsäureester, oder Polyoxethylensorbitanester, wie Polyoxyethylensorbitanfettsäureester.
  • Stäubemittel erhält man im allgemeinen durch Vermahlen des Wirkstoffes z.B. des herbiziden Wirkstoffs und/oder des Safeners mit fein verteilten festen Stoffen, z.B. Talkum, natürlichen Tonen, wie Kaolin, Bentonit und Pyrophyllit, oder Diatomeenerde.
  • Suspensionskonzentrate können auf Wasser- oder Ölbasis sein. Sie können beispielsweise durch Naß-Vermahlung mittels handelsüblicher Perlmühlen und gegebenenfalls Zusatz von Tensiden, wie sie z.B. bei den anderen Formulierungstypen bereits aufgeführt sind, hergestellt werden.
  • Emulsionen, z.B. Öl-in-Wasser-Emulsionen (EW), lassen sich beispielsweise mittels Rührern, Kolloidmühlen und/oder statischen Mischern unter Verwendung von wäßrigen organischen Lösungsmitteln und gegebenenfalls Tensiden, wie sie z.B. bei den anderen Formulierungstypen bereits aufgeführt sind, herstellen.
  • Granulate können entweder durch Verdüsen des Wirkstoffes z.B. des herbiziden Wirkstoffs und/oder des Safeners auf adsorptionsfähiges, granuliertes Inertmaterial hergestellt werden oder durch Aufbringen von Wirkstoffkonzentraten mittels Klebemitteln, z.B. Polyvinylalkohol, polyacrylsaurem Natrium oder auch Mineralölen, auf die Oberfläche von Trägerstoffen, wie Sand, Kaolinite oder von granuliertem Inertmaterial. Auch können geeignete Wirkstoffe in der für die Herstellung von Düngemittelgranulaten üblichen Weise – gewünschtenfalls in Mischung mit Düngemitteln – granuliert werden. Wasserdispergierbare Granulate werden in der Regel nach den üblichen Verfahren, wie Sprühtrocknung, Wirbelbett-Granulierung, Teller-Granulierung, Mischung mit Hochgeschwindigkeitsmischern und Extrusion ohne festes Inertmaterial, hergestellt.
  • Zur Herstellung von Teller-, Fließbett-, Extruder- und Sprühgranulaten siehe z.B. in "Spray-Drying Handbook" 3rd ed. 1979, G. Goodwin Ltd., London; J.E. Browning, "Agglomeration", Chemical and Engineering 1967, Seiten 147 ff; "Perry's Chemical Engineer's Handbook", 5th Ed., McGraw-Hill, New York 1973, S. 8-57.
  • Für weitere Einzelheiten zur Formulierung von Pflanzenschutzmitteln siehe z.B. G.C. Klingman, "Weed Control as a Science", John Wiley and Sons, Inc., New York, 1961, Seiten 81-96 und J.D. Freyer, S.A. Evans, "Weed Control Handbook", 5th Ed., Blackwell Scientific Publications, Oxford, 1968, Seiten 101-103.
  • Bevorzugte Formulierungen sind Flüssigformulierungen wie Ölsuspensionen, Ölsuspensionskonzentrate, Suspoemulsionen, Suspoemulsionskonzentrate, Emulsionen z.B. auf W/O- oder O/W-Basis, Emulsionskonzentrate, Mikroemulsionen, Mikroemulsionskonzentrate, emulgierbare Konzentrate, und daraus erhältliche (wässrige) Spritzbrühen.
  • Ein besonders bevorzugter flüssiger Formulierungstyp sind Ölsuspensionskonzentrate, d.h. Suspensionkonzentrate auf Basis organischer Lösungsmittel, und daraus durch Verdünnung erhältliche Formulierungen wie Lösungen, Emulsionen, Suspoemulsionen und Suspensionen. In den Ölsuspensionskonzentraten sind ein oder mehrere Wirkstoffe in dem organischen Lösungsmittel suspendiert, weitere Wirkstoffe können in dem organischen Lösungsmittel gelöst sein. In einem bevorzugten Ölsuspensionskonzentrat liegt das Herbizid (A) in suspendierter Form in dem organischen Lösungsmittel vor. Dies bedeutet, daß der Hauptanteil (in Gew.-%) an Sulfonamid ungelöst in fein verteilter Form vorliegt, ein geringerer Teil des Sulfonamids kann gelöst vorliegen. Vorzugsweise ist das Sulfonamid im organischen Lösungsmittel zu mehr als 80 Gew.-%, besonders bevorzugt zu mehr als 90 Gew.-% suspendiert, jeweils bezogen auf die Gesamtmenge an Sulfonamid in dem erfindungsgemäßen Ölsuspensionskonzentrat.
  • Die agrochemischen Formulierungen enthalten in der Regel 0,1 bis 99 Gew.-%, insbesondere 0,1 bis 95 Gew.-% Wirkstoffe, z.B. Safener- Wirkstoffe (B), oder Sulfonylharnstoffe (A), oder des erfindungsgemäßen Herbizid/Safener-Wirkstoffgemischs, enthaltend Sulfonylharnstoffe (A) und Safener-Wirkstoffe (B), und 1 bis 99,9 Gew.-%, insbesondere 5 bis 99,8 Gew.-%, eines festen oder flüssigen Zusatzstoffes und 0 bis 25 Gew.-%, insbesondere 0,1 bis 25 Gew.-% eines Tensides.
  • In Spritzpulvern beträgt die Wirkstoffkonzentration z.B. etwa 10 bis 90 Gew.-%, der Rest zu 100 Gew.-% besteht aus üblichen Formulierungsbestandteilen. Bei emulgierbaren Konzentraten beträgt die Wirkstoffkonzentration etwa 1 bis 80 Gew.-%. Staubförmige Formulierungen enthalten etwa 1 bis 20 Gew.-% an Wirkstoffen, versprühbare Lösungen etwa 0, 2 bis 20 Gew.-% Wirkstoffe. Bei Granulaten, wie wasserdispergierbaren Granulaten, hängt der Wirkstoffgehalt zum Teil davon ab, ob die wirksame Verbindung flüssig oder fest vorliegt. In der Regel liegt der Gehalt bei den in Wasser dispergierbaren Granulaten zwischen 10 und 90 Gew.-%.
  • Daneben enthalten die genannten Wirkstoffformulierungen gegebenenfalls die jeweils üblichen Haft-, Netz-, Dispergier-, Emulgier-, Penetrations-, Konservierungs-, Frostschutz- und Lösungsmittel, Füll-, Träger- und Farbstoffe, Entschäumer, Verdunstungshemmer und den pH-Wert und die Viskosität beeinflussende Mittel.
  • Zur Anwendung werden die in handelsüblicher Form vorliegenden Formulierungen gegebenenfalls in üblicher Weise verdünnt z.B. bei Spritzpulvern, emulgierbaren Konzentraten, Dispersionen und wasserdispergierbaren Granulaten mittels Wasser. Staubförmige Zubereitungen, Boden- bzw. Streugranulate sowie versprühbare Lösungen werden vor der Anwendung üblicherweise nicht mehr mit weiteren inerten Stoffen verdünnt.
  • Mit den äußeren Bedingungen wie Temperatur, Feuchtigkeit, der Art des verwendeten Herbizids, u.a. variiert die erforderliche Aufwandmenge der Herbizide (A). Sie kann innerhalb weiter Grenzen variiert werden, z.B. zwischen 0,001 und 10,0 kg/ha oder mehr an Herbizid, vorzugsweise liegt sie zwischen 0,005 und 5 kg/ha.
    •
  • Folgende Beispiele dienen zur Erläuterung der Erfindung:
  • A. Formulierungsbeispiele
    • a) Ein Stäubemittel wird erhalten, indem man 10 Gew.-Teile eines Sulfonylharnstoffs (A) oder eines Safeners (B) oder eines Wirkstoffgemischs aus einem Sulfonylharnstoff (A) und einem Safener (B) und 90 Gew.-Teile Talkum als Inertstoff mischt und in einer Schlagmühle zerkleinert.
    • b) Ein in Wasser leicht dispergierbares, benetzbares Pulver wird erhalten, indem man 25 Gewichtsteile eines Sulfonylharnstoffs (A) oder eines Safeners (B) oder eines Wirkstoffgemischs aus einem Sulfonylharnstoff (A) und einem Safener (B), 64 Gewichtsteile kaolinhaltigen Quarz als Inertstoff, 10 Gewichtsteile ligninsulfonsaures Kalium und 1 Gew.-Teil oleoylmethyltaurinsaures Natrium als Netz- und Dispergiermittel mischt und in einer Stiftmühle mahlt.
    • b) Ein in Wasser leicht dispergierbares oder suspendierbares Konzentrat wird erhalten, indem man 20 Gewichtsteile eines Sulfonylharnstoffs (A) oder eines Safeners (B) oder eines Wirkstoffgemischs aus einem Sulfonylharnstoff (A) und einem Safener (B), 6 Gew.-Teilen Alkylphenolpolyglykolether (®Triton X 207), 3 Gew.-Teilen Isotridecanolpolyglykolether (8 EO) und 71 Gew.- Teilen paraffinischem Mineralöl (Siedebereich z.B. ca. 255 bis über 277° C) mischt und in einer Reibkugelmühle auf eine Feinheit von unter 5 Mikron vermahlt.
    • d) Ein emulgierbares Konzentrat wird erhalten aus 15 Gew.-Teilen eines Sulfonylharnstoffs (A) oder eines Safeners (B) oder eines Wirkstoffgemischs aus einem Sulfonylharnstoff (A) und einem Safener (B), 75 Gew.Teilen Cyclohexanon als Lösemittel und 10 Gew.-Teilen oxethyliertes Nonylphenol als Emulgator.
    • e) Ein in Wasser dispergierbares Granulat wird erhalten, indem man 75 Gew.-Teile eines Sulfonylharnstoffs (A) oder eines Safeners (B) oder eines Wirkstoffgemischs aus einem Sulfonylharnstoff (A) und einem Safener (B) 10 Gew.-Teile ligninsulfonsaures Calcium, 5 Gew.-Teile Natriumlaurylsulfat, 3 Gew.-Teile Polyvinylalkohol und 7 Gew.-Teile Kaolin mischt, auf einer Stiftmühle mahlt und das Pulver in einem Wirbelbett durch Aufsprühen von Wasser als Granulierflüssigkeit granuliert.
    • f) Ein in Wasser dispergierbares Granulat wird auch erhalten, indem man 25 Gew.-Teile) eines Sulfonylharnstoffs (A) oder eines Safeners (B) oder eines Wirkstoffgemischs aus einem Sulfonylharnstoff (A) und einem Safener (B) 5 Gew.-Teile 2, 2'-dinaphthylmethan-6, 6'-disulfonsaures Natrium, 2 Gew.-Teile oleoylmethyltaurinsaures Natrium, 1 Gew.-Teile Polyvinylalkohol, 17 Gew.-Teile Calciumcarbonat und 50 Gew.-Teile Wasser auf einer Kolloidmühle homogensiert und vorzerkleinert, anschließend auf einer Perlmühle mahlt und die so erhaltene Suspension in einem Sprühturm mittels einer Einstoffdüse zerstäubt und trocknet.
    • g) Ein Ölsuspensionskonzentrat wird durch Vermischen der Komponenten erhalten, z.B. indem man eine Vormischung herstellt, wobei in dem Lösungsmittel C) optional ein Sulfosuccinat D) gelöst wird und dieser Lösung, gegebenenfalls weitere Hilfs- und Zusatzstoffe F) zugegeben werden. Dann werden gegebenenfalls verwendete lösliche Safener B) und agrochemische Wirkstoffe E) in der Vormischung gelöst. Nach Abschluß des Lösungsprozesses wird fester Sulfonylharnstoff A) und gegebenenfalls verwendete unlösliche Safener B) und agrochemische Wirkstoffe E) in die Mischung suspendiert. Die grobe Suspension wird, gegebenenfalls nach einer Vorvermahlung, einer Feinvermahlung unterzogen. In einer anderen Ausführungsvariante wird fester Sulfonylharnstoff A), sowie gegebenenfalls verwendete unlösliche Komponenten B), E) und F), in das Lösungsmittel C) suspendiert, welches optional ein Sulfosuccinat D) enthält, und einer Vermahlung unterzogen. Gegebenenfalls verwendete lösliche Wirkstoffe B) und E) sowie Hilfs- und Zusatzstoffe aus F), die keiner Vermahlung bedürfen oder für den Mahlvorgang nicht notwendig sind, werden nach der Vermahlung zugesetzt.
  • B. Biologische Beispiele
  • 1. Bonitierung der Schadwirkung
  • Die Schadwirkung an den Pflanzen wird auf einer Skala von 0 bis 100 % optische im Vergleich zu Kontrollpflanzen bewertet:
    0 % = keine erkennbare Wirkung im Vergleich zur unbehandelten Pflanze,
    100 %= behandelte Pflanze stirbt ab
  • 2. Herbizidwirkung im Nachauflauf
  • Samen von mono- und dikotylen Unkräutern und von Kulturpflanzen werden in Plastiktöpfen in sandigem Lehmboden ausgelegt, mit Erde abgedeckt und im Gewächshaus unter guten Wachstumsbedingungen angezogen.
  • Drei Wochen nach der Aussaat werden die Versuchspflanzen im 3-4 Blattstadium behandelt. Die als Emulsionskonzentrate formulierten erfindungsgemäßen Einzelwirkstoffe werden in verschiedenen Dosierungen mit einer Wasseraufwandmengen von umgerechnet 300 l/ha einzeln oder als Mischungen auf die grünen Pflanzenteile gesprüht und nach 3 Wochen Standzeit der Versuchspflanzen im Gewächshaus unter optimalen Wachstumsbedingungen wird die Wirkung der Präparate optisch im Vergleich zu unbehandelten Kontrollen bonitiert. Wie die Beispiele zeigen, sind die erfindungsgemäßen Kombinationen aus Sulfonylharnstoffe und Safenern in der Lage, ein breites Spektrum von Unkräutern nachhaltig zu bekämpfen, wobei Schäden an Kulturpflanzen im Vergleich zur Anwendung der einzelnen Sulfonylharnstoffe ohne Safener wesentlich reduziert sind.

Claims (13)

  1. Herbizid wirksames Mittel, enthaltend eine Mischung aus (A) eine herbizid wirksame Menge an einem oder mehreren Sulfonylharnstoffen aus der Gruppe Metsulfuron, Thifensulfuron, Tribenuron, Chlorsulfuron und deren Salze und Ester, und (B) einer antidotisch wirksamen Menge an einem oder mehreren Safenern aus der Gruppe Mefenpyr, Isoxadifen, Cloquintocet und deren Salze und Ester.
  2. Herbizid wirksames Mittel gemäß Anspruch 1, worin die Sulfonylharnstoffe (A) ausgewählt sind aus der Gruppe bestehend aus Metsulfuron-methyl, Thifensulfuron-methyl, Tribenuron-methyl, Chlorsulfuron und deren Alkalimetallsalzen.
  3. Herbizid wirksames Mittel gemäß Anspruch 1 oder 2, worin der oder die Safener (B) ausgewählt sind aus der Gruppe bestehend aus Mefenpyr-diethyl, Isoxadifen-ethyl und Cloquintocet-mexyl.
  4. Herbizid wirksames Mittel gemäß einem oder mehreren der Ansprüche 1 bis 3, worin das Gewichtsverhältnis Herbizid:Safener 1:100 bis 100:1 beträgt.
  5. Herbizid wirksames Mittel gemäß einem oder mehreren der Ansprüche 1 bis 4, zusätzlich enthaltend (C) ein oder mehrere Lösungsmittel, bevorzugt organische Lösungsmittel, (D) ein oder mehrere Sulfosuccinate, (E) einen oder mehrere von (A) und (B) verschiedene agrochemische Wirkstoffe, und/oder (F) übliche Hilfs- und Zusatzstoffe.
  6. Herbizid wirksames Mittel gemäß einem oder mehreren der Ansprüche 1 bis 5 in Form einer Flüssigformulierung.
  7. Flüssigformulierung, enthaltend (A) eine herbizid wirksame Menge an einem oder mehreren Sulfonylharnstoffen aus der Gruppe Metsulfuron, Thifensulfuron, Tribenuron, Chlorsulfuron und deren Salze und Ester, (B) einer antidotisch wirksamen Menge an einem oder mehreren Safenern aus der Gruppe Mefenpyr, Isoxadifen, Cloquintocet und deren Salze und Ester, (C) ein oder mehrere Lösungsmittel, bevorzugt organische Lösungsmittel, (D) optional ein oder mehrere Sulfosuccinate, (E) optional einen oder mehrere von (A) und (B) verschiedene agrochemische Wirkstoffe, und (F) optional übliche Hilfs- und Zusatzstoffe.
  8. Flüssigformulierung gemäß Anspruch 7 in Form einer Ölsuspension, Ölsuspensionskonzentrat, Suspoemulsion, Suspoemulsionskonzentrat, Emulsion, Emulsionskonzentrat, Mikroemulsion, Mikroemulsionskonzentrat, emulgierbaren Konzentrats, und daraus erhältlicher (wässrige) Spritzbrühen.
  9. Verfahren zur Bekämpfung von Schadpflanzen in Pflanzenkulturen, dadurch gekennzeichnet, daß die Komponenten des herbizid wirksamen Mittels gemäß einem oder mehreren der Ansprüche 1 bis 6 oder der Flüssigformulierung gemäß Anspruch 7 oder 8 gemeinsam oder getrennt auf die Schadpflanzen, Kulturpflanzen, Pflanzensamen oder die Fläche, auf der die Pflanzen wachsen, aufgebracht werden.
  10. Verfahren gemäß Anspruch 9, dadurch gekennzeichnet, daß die Kulturpflanzen aus der Gruppe Mais, Weizen, Roggen, Gerste, Hafer, Reis, Sorghum, Baumwolle und Soja stammen.
  11. Verfahren gemäß Anspruch 9 oder 10, dadurch gekennzeichnet, daß die Kulturpflanzen transgen sind oder Toleranz durch Selektionszüchtung aufweisen.
  12. Verwendung eines herbizid wirksamen Mittels gemäß einem oder mehreren der Ansprüche 1 bis 6 oder einer Flüssigformulierung gemäß Anspruch 7 oder 8, zur Bekämpfung von Schadpflanzen in Pflanzenkulturen.
  13. Verfahren ur Herstellung eines herbizid wirksamen Mittels gemäß einem oder mehreren der Ansprüche 1 bis 6 oder einer Flüssigformulierung gemäß Anspruch 7 oder 8, worin die Komponenten miteinander vermischt werden.
DE10351234A 2003-11-03 2003-11-03 Herbizid wirksames Mittel Ceased DE10351234A1 (de)

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DE10351234A DE10351234A1 (de) 2003-11-03 2003-11-03 Herbizid wirksames Mittel
AU2004285269A AU2004285269B2 (en) 2003-11-03 2004-10-21 Herbicidally active agent
AT04790700T ATE389327T1 (de) 2003-11-03 2004-10-21 Herbizid wirksames mittel
CA002544415A CA2544415A1 (en) 2003-11-03 2004-10-21 Herbicidally active agent
UAA200606174A UA83698C2 (en) 2003-11-03 2004-10-21 Liquid herbicidal composition
DK04790700T DK1681932T3 (da) 2003-11-03 2004-10-21 Herbicidt aktivt middel
CNA2004800354706A CN1886051A (zh) 2003-11-03 2004-10-21 除草活性剂
BRPI0416159-9A BRPI0416159A (pt) 2003-11-03 2004-10-21 agente de eficácia herbicida
EP04790700A EP1681932B1 (de) 2003-11-03 2004-10-21 Herbizid wirksames mittel
EA200600856A EA012521B1 (ru) 2003-11-03 2004-10-21 Жидкий препарат, его применение, способ его получения и способ борьбы с сорными растениями
DE502004006612T DE502004006612D1 (de) 2003-11-03 2004-10-21 Herbizid wirksames mittel
PL04790700T PL1681932T3 (pl) 2003-11-03 2004-10-21 Środek chwastobójczo czynny
PCT/EP2004/011893 WO2005041654A2 (de) 2003-11-03 2004-10-21 Herbizid wirksames mittel
ES04790700T ES2302038T3 (es) 2003-11-03 2004-10-21 Agente activo como herbicida.
US10/976,217 US7432226B2 (en) 2003-11-03 2004-10-28 Herbicidally active composition
TW093133238A TW200517058A (en) 2003-11-03 2004-11-01 Herbicidally active composition
ARP040104023A AR046224A1 (es) 2003-11-03 2004-11-01 Composicion activa como herbicida
ZA200603267A ZA200603267B (en) 2003-11-03 2006-04-24 Herbicidally active agent
IL175359A IL175359A0 (en) 2003-11-03 2006-05-01 Herbicidally active agent
US12/201,115 US20090054236A1 (en) 2003-11-03 2008-08-29 Herbicidally active composition

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TW200843642A (en) * 2007-03-08 2008-11-16 Du Pont Liquid sulfonylurea herbicide formulations
JP2010235591A (ja) * 2009-03-13 2010-10-21 Sumitomo Chemical Co Ltd 除草用組成物
CN102027970B (zh) * 2009-09-28 2013-08-07 南京华洲药业有限公司 一种含二氯吡啶酸与噻吩磺隆的除草组合物及其应用
CN101919399B (zh) * 2010-06-21 2013-10-30 西北农林科技大学 一种复配化学杂交剂组合物及其应用

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EP0790771B1 (de) * 1994-11-11 1999-01-20 Hoechst Schering AgrEvo GmbH Kombinationen aus phenylsulfonylharnstoff-herbiziden und safenern
DE19827855A1 (de) * 1998-06-23 1999-12-30 Hoechst Schering Agrevo Gmbh Kombinationen aus Herbiziden und Safenern
DE19960918A1 (de) * 1999-11-18 2001-05-23 Bayer Ag Synergistische herbizide Wirkstoffkombinationen
WO2002017718A1 (de) * 2000-08-31 2002-03-07 Basf Aktiengesellschaft Verfahren zur herstellung einer herbiziden festformulierung

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Publication number Priority date Publication date Assignee Title
EP0790771B1 (de) * 1994-11-11 1999-01-20 Hoechst Schering AgrEvo GmbH Kombinationen aus phenylsulfonylharnstoff-herbiziden und safenern
DE19827855A1 (de) * 1998-06-23 1999-12-30 Hoechst Schering Agrevo Gmbh Kombinationen aus Herbiziden und Safenern
DE19960918A1 (de) * 1999-11-18 2001-05-23 Bayer Ag Synergistische herbizide Wirkstoffkombinationen
WO2002017718A1 (de) * 2000-08-31 2002-03-07 Basf Aktiengesellschaft Verfahren zur herstellung einer herbiziden festformulierung

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