[go: up one dir, main page]

GB729302A - Polymerized starch esters and ethers - Google Patents

Polymerized starch esters and ethers

Info

Publication number
GB729302A
GB729302A GB6023/51A GB602351A GB729302A GB 729302 A GB729302 A GB 729302A GB 6023/51 A GB6023/51 A GB 6023/51A GB 602351 A GB602351 A GB 602351A GB 729302 A GB729302 A GB 729302A
Authority
GB
United Kingdom
Prior art keywords
starch
water
dispersible
aqueous
ester
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired
Application number
GB6023/51A
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
NAT STARCH PRODUCTS Inc
Original Assignee
NAT STARCH PRODUCTS Inc
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by NAT STARCH PRODUCTS Inc filed Critical NAT STARCH PRODUCTS Inc
Publication of GB729302A publication Critical patent/GB729302A/en
Expired legal-status Critical Current

Links

Classifications

    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08BPOLYSACCHARIDES; DERIVATIVES THEREOF
    • C08B31/00Preparation of derivatives of starch

Landscapes

  • Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Engineering & Computer Science (AREA)
  • Biochemistry (AREA)
  • Materials Engineering (AREA)
  • Health & Medical Sciences (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Organic Chemistry (AREA)
  • Polysaccharides And Polysaccharide Derivatives (AREA)
  • Treatments For Attaching Organic Compounds To Fibrous Goods (AREA)
  • Paper (AREA)

Abstract

Textile fabrics are stiffened by treatment with an aqueous dispersion of an unsaturated starch derivative obtained by reacting a starch in an aqueous alkaline medium with an organic anhydride, a chloroformate, an organic halide etherifying agent or an epoxy compound, each containing the polymerizable group -C(R) : CH2, where R is hydrogen or an alkyl group, so as to produce a water-dispersible starch ether or ester containing not substantially more than one such polymerizable group per 15 anhydroglucose units (see Group IV (b)). The fabric is then treated with a water-soluble vinyl polymerization type catalyst, whereby the starch derivative is insolubilized by polymerization in situ (see Group IV (a)). In an example, unsized cotton sheeting is saturated with an aqueous dispersion of a starch ester derived from acid-converted corn starch and methacrylic anhydride, ironed dry and then passed through aqueous sodium bisulphite and again ironed dry; the material so treated retains its stiffness after washing.ALSO:Polymerized starch esters and ethers are prepared by reacting a water-dispersible starch in an aqueous alkaline medium with an amount of an aqueous alkaline medium with an amount of an organic anhydride, a chloroformate, an organic halide etherifying agent or an epoxy compound each containing the polymerizable olefinic group <FORM:0729302/IV (a)/1> where R is hydrogen or an alkyl group such as to produce a water-dispersible starch ester or ether containing not substantially more than one said polymerizable group per 15 anhydroglucose units (see Group IV (b)) and contacting the water-dispersible ester or ether with a water-soluble free radical producing vinyl polymerization catalyst thereby reducing the solubility in water of the starch derivative. The solubility may be so reduced that the product does not form a dispersion even after boiling in water for several hours. Suitable starches include corn, waxy maize, potato, sweet potato, sago, wheat, rice and tapioca starches; they may be in ungelatinized form or may be gelatinized or converted by heat and/or acids or oxidizing agents into thin boiling starches, dextrine or British gum. Reactants used for producing the esters or ethers include the anhydrides of acrylic and methacrylic acids, allyl chloroformate, allyl bromide and butadiene monoxide. The after-treatment of the water-dispersible starch derivatives may be effected by mixing an aqueous dispersion or suspension of the starch derivative with the catalyst, e.g. a persulphate, a bisulphite, hydrogen peroxide and ceric sulphate. Catalyst activators may also be present, e.g. ferrous and ferric sulphates, silver nitrate, hydroxylamine hydrochloride and the reductant activators. The process may be utilized in the treatment of textiles and paper, wherein the fabric and paper are sized or coated with an aqueous dispersion of the water-dispersible starch derivative and then contacted with the catalyst, e.g. an aqueous solution of sodium bisulphite whereby the material is given water-resistance and the paper has increased wet strength (see Groups IV (c) and VIII). The products may also be used in adhesives. In examples: (1) a water-dispersible starch ester obtained from corn starch and methacrylic anhydride is treated in aqueous suspension with ammonium persulphate and ferrous sulphate, sodium meta bisulphite or ceric sulphate giving a non-gelatinizable product; (2) an ether obtained from gelatinized waxy maize starch and butadiene-monoxide is treated in aqueous dispersion with sodium metabisulphite yielding a rubbery gel; (3) a starch derivative obtained from potato starch and allyl chloroformate is treated with hydrogen peroxide and various catalyst activators yielding non-gelatinizable insoluble products.ALSO:Water-dispersible starch esters or ethers are prepared by reacting a water-dispersible starch in an aqueous alkaline medium with an amount of an organic anhydride, a chloroformate, an organic halide etherifying agent or an epoxy compound each containing the polymerizable group <FORM:0729302/IV (b)/1> where R is hydrogen or an alkyl group, such as to produce a water-dispersible starch ether or ester containing not substantially more than one said polymerizable olefinic group per 15 anhydro-glucose units. Suitable starches include corn, waxy maize, potato, sago, wheat, rice, sweet potato and tapioca starches; these may be in their ungelatinized state or they may be gelatinized or converted by heat and/or acids or oxidizing agents to thin boiling starch, dextrine or British gum. If desired, the gelatinization of the starch molecule may be effected during or after the formation of the dispersible ester or ether. The dispersibility of the products may be reduced up to complete indispersibility in water by contacting them with a water-soluble free radical producing vinyl polymerization catalyst (see Group IV (a)) yielding products having application in the manufacture of high wet strength papers (see Group VIII) water-resistent sizes and coatings for textiles (see Group IV (c)) and adhesives. In examples: (1) corn starch is suspended in aqueous caustic soda solution and methacrylic anhydride added slowly, a pH of 8-9 being maintained by addition of caustic soda and the resulting ester is still dispersible after cooking in water; (2) allyl bromide is added to a suspension of tapioca in aqueous caustic soda containing sodium sulphate to prevent gelatinization; (3) allyl chloroformate is added to a suspension of potato starch in aqueous sodium carbonate; (4) butadiene monoxide is added to a mixture of acid-converted waxy maize starch in aqueous caustic soda. Acrylic acid anhydride is also mentioned.
GB6023/51A 1950-04-06 1951-03-13 Polymerized starch esters and ethers Expired GB729302A (en)

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
US729302XA 1950-04-06 1950-04-06

Publications (1)

Publication Number Publication Date
GB729302A true GB729302A (en) 1955-05-04

Family

ID=22110619

Family Applications (1)

Application Number Title Priority Date Filing Date
GB6023/51A Expired GB729302A (en) 1950-04-06 1951-03-13 Polymerized starch esters and ethers

Country Status (1)

Country Link
GB (1) GB729302A (en)

Similar Documents

Publication Publication Date Title
US2668156A (en) Unsaturated starch compounds and insoluble derivatives thereof
US4301017A (en) Stable, liquid starch graft copolymer composition
US2813093A (en) Ungelatinized tertiary amino alkyl ethers of amylaceous materials
SU1105118A3 (en) Method of obtaining cellulose mixed ethers
US4127563A (en) Low pH preparation of cationic starches and flours
US2148951A (en) Organic starch derivatives and process
US2516633A (en) Preparation of starch ethers in original granule form
US2935436A (en) Method of making paper containing a starch ether and product produced thereby
US2618633A (en) Preparation of carboxyethyl cellulose
US4940741A (en) Process for the production of hardboard
US4480091A (en) Process for preparing cellulose sulfate esters
US2539417A (en) Preparation of cellulose derivative
US2773057A (en) Method of preparing starch ether derivatives and new starch ether derivatives produced thereby
US2524400A (en) Chemically modified starches
US3354034A (en) Novel cationic starch derivatives
US3535308A (en) Process for the preparation of partially esterified polyhydroxylic polymers
US2580351A (en) Cellulose sulfamylethyl ether
US3954724A (en) Process for preparing aqueous dispersions of high polymer using pullulan as a dispersant
US2388764A (en) Cellulose ethers and process for producing the same
GB691364A (en) Polysaccharide derivatives of substituted dicarboxylic acids
US2451686A (en) Starch compositions capable of forming water-soluble derivatives
GB729302A (en) Polymerized starch esters and ethers
US2862922A (en) Method of making sodium cellulose sulfate
US3331833A (en) The graft polymerization of ethylenimine onto tertiary amino starch
US3719664A (en) Warp sizing agent