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CN112273715A - Filter core material of cigarette filter tip and preparation method - Google Patents

Filter core material of cigarette filter tip and preparation method Download PDF

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Publication number
CN112273715A
CN112273715A CN202010658385.6A CN202010658385A CN112273715A CN 112273715 A CN112273715 A CN 112273715A CN 202010658385 A CN202010658385 A CN 202010658385A CN 112273715 A CN112273715 A CN 112273715A
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CN
China
Prior art keywords
melt
polypropylene
polylactic acid
blown
nano catalyst
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Pending
Application number
CN202010658385.6A
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Chinese (zh)
Inventor
陈苏
郝路伟
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Janus New Materials Co ltd
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Janus New Materials Co ltd
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Janus New Materials Co ltd filed Critical Janus New Materials Co ltd
Priority to CN202010658385.6A priority Critical patent/CN112273715A/en
Publication of CN112273715A publication Critical patent/CN112273715A/en
Pending legal-status Critical Current

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Classifications

    • AHUMAN NECESSITIES
    • A24TOBACCO; CIGARS; CIGARETTES; SIMULATED SMOKING DEVICES; SMOKERS' REQUISITES
    • A24DCIGARS; CIGARETTES; TOBACCO SMOKE FILTERS; MOUTHPIECES FOR CIGARS OR CIGARETTES; MANUFACTURE OF TOBACCO SMOKE FILTERS OR MOUTHPIECES
    • A24D3/00Tobacco smoke filters, e.g. filter-tips, filtering inserts; Filters specially adapted for simulated smoking devices; Mouthpieces for cigars or cigarettes
    • A24D3/06Use of materials for tobacco smoke filters
    • A24D3/08Use of materials for tobacco smoke filters of organic materials as carrier or major constituent
    • A24D3/10Use of materials for tobacco smoke filters of organic materials as carrier or major constituent of cellulose or cellulose derivatives
    • AHUMAN NECESSITIES
    • A24TOBACCO; CIGARS; CIGARETTES; SIMULATED SMOKING DEVICES; SMOKERS' REQUISITES
    • A24DCIGARS; CIGARETTES; TOBACCO SMOKE FILTERS; MOUTHPIECES FOR CIGARS OR CIGARETTES; MANUFACTURE OF TOBACCO SMOKE FILTERS OR MOUTHPIECES
    • A24D3/00Tobacco smoke filters, e.g. filter-tips, filtering inserts; Filters specially adapted for simulated smoking devices; Mouthpieces for cigars or cigarettes
    • A24D3/06Use of materials for tobacco smoke filters
    • A24D3/061Use of materials for tobacco smoke filters containing additives entrapped within capsules, sponge-like material or the like, for further release upon smoking

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  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Materials Engineering (AREA)
  • Cigarettes, Filters, And Manufacturing Of Filters (AREA)

Abstract

The invention discloses a cigarette filter tip filter core material and a preparation method thereof, and is characterized in that: the method is characterized in that: the polypropylene-polylactic acid composite melt-blown fabric consists of polypropylene-polylactic acid composite melt-blown fabric fiber modified by a compatibilizer and a nano catalyst adhered on the melt-blown fabric through an adhesive; wherein the weight ratio of the adhesive to the nano catalyst is 1: (0.1-0.15), the nano catalyst is loaded on the melt-blown cloth fiber through a spraying process and a drying process, and the nano catalyst is adhered on the melt-blown cloth fiber through an adhesive. The filter core material is molded by a cigarette filter core molding machine to obtain the cigarette filter core. The cigarette filter tip prepared by the method of the invention not only can effectively filter the harmful components such as tar, nicotine and the like in the smoke, but also can decompose most of the unfiltered harmful substances into harmless substances in a short time by introducing the nano catalyst, thereby effectively reducing the harm of the cigarette to the human health.

Description

Filter core material of cigarette filter tip and preparation method
Technical Field
The invention relates to a cigarette filter core material and a preparation method thereof, belonging to the field of non-woven fabric materials and cigarette filter materials.
Background
As is well known, smoking is harmful to human health, and in order to reduce the harm to human bodies, many means are taken by merchants, such as adding filter tips. Research shows that harmful substances decomposed by smoking, such as tar, aldehydes, nicotine and the like, can cause fatal diseases such as lung cancer and the like. The loss caused by smoking in China is up to more than one billion yuan each year.
The cigarette filter tip is an important component of a cigarette and is used for filtering and blocking a part of saline-alkali tar in smoke and reducing the harm of harmful substances in the smoke to human bodies when smokers smoke.
Currently, the material of cigarette filters consists mainly of cellulose acetate fibers or polypropylene fibers. The cellulose acetate is easily spun into fine fibers through a melt spinning process, and the filter stick and the filter made of the rolled fine fibers have excellent filterability and are the best filter material at present. However, since the cellulose acetate fiber is obtained by using wood as a raw material and through steps of cellulose extraction, acetification, saponification and the like, a large amount of waste water, waste gas and waste residues which seriously pollute the environment are generated in the preparation process. And forest resources in China are in short supply, cellulose acetate cannot be self-supplied, the cellulose acetate mainly depends on import, and the price is high, so that the cellulose acetate is not suitable for being used in large quantities. The polypropylene is easy to prepare fibers through melt spinning, has good lipophilicity, is nontoxic and tasteless, but is difficult to form a net structure after fiber opening due to the non-polarity and high crystallinity of the polypropylene, so that the filter tip prepared from the single polypropylene fiber has poor filtering effect and cannot meet the requirement of people on the filtering effect of the filter tip.
In recent years, there has been a great deal of development of biodegradable polymers, particularly lactic acid polymers such as polylactic acid. The research shows that the polylactic acid has better processing performance and can be processed by various processing technologies of common thermoplastic polymers, including a melt spinning technology. After the polylactic acid is formed into fibers by a spinning process, the polylactic acid has good adsorption and filtration functions on nicotine and tar. This provides the possibility of processing polylactic acid into filter material. Besides, the polylactic acid fiber has two advantages: firstly, the raw materials for preparing the polylactic acid fiber can be derived from natural starch such as corn, sweet potato and the like, the resources can be regenerated, the sources are rich, and the price is low; and secondly, the polylactic acid is a biodegradable material, the degradation products of the polylactic acid are water and carbon dioxide, no pollutant is generated, and the polylactic acid cannot cause pressure on environmental pollution when being used in large quantities. Unfortunately, polylactic acid fibers do not meet the core process of the filter process.
At present, cigarette filters made of fibers have nicotine and tar filtering performance, but can only filter 30% -50% of harmful substances. Or a part of harmful substances enter the oral cavity and respiratory tract of the human body through the cigarette filter tip, thereby causing harm to the health of the human body. Many researches show that the nano metal catalyst can decompose substances such as low aldehydes, aliphatic hydrocarbons and the like into harmless substances in a short time.
Disclosure of Invention
The invention aims to provide a filter element material of a cigarette filter and a preparation method thereof. On one hand, the polypropylene and polylactic acid mixed melt-blown fabric fiber has low price, is easy to produce, has filtering performance superior to that of polypropylene fiber, and can reduce the harm of the cigarette filter tip to the environment. On the other hand, the introduction of the nano catalyst further decomposes substances such as low aldehydes, aliphatic hydrocarbons and the like in the smoke, and reduces the harm of the cigarette smoke to human bodies. The filter element of the cigarette filter can solve the problem of filtering cigarette smoke in the modern society.
In order to achieve the technical purpose, the technical scheme adopted by the invention is as follows: a filter element material for cigarette filter, which is characterized in that: the polypropylene-polylactic acid composite melt-blown fabric consists of polypropylene-polylactic acid composite melt-blown fabric fiber modified by a compatibilizer and a nano catalyst adhered on the melt-blown fabric through an adhesive; wherein the weight ratio of the adhesive to the nano catalyst is 1: (0.1-0.15), the nano catalyst is loaded on the melt-blown cloth fiber through a spraying process and a drying process, and the nano catalyst is adhered on the melt-blown cloth fiber through an adhesive.
Preferably, the polypropylene-polylactic acid composite meltblown fiber modified by the compatibilizer is prepared by mixing polypropylene, polylactic acid and the compatibilizer in a weight ratio of 1: (0.25-0.35): (0.03-0.1) uniformly stirring the mixture in a double screw to form mixed master batches, and extruding the mixed master batches by a melt-blowing process to obtain the master batches.
Preferably, the polypropylene is homopolymerized polypropylene, and the melt index is 1200-1500g/10 min; the polylactic acid is L-polylactic acid, and the number average molecular weight is 100000-140000 Mn; the compatibilizer is one of polyethylene glycol, polypropylene grafted maleic anhydride or maleic anhydride.
Preferably, the adhesive is glycerol triacetate; the adhesive is the guarantee of the bonding strength between the nano catalyst and the polypropylene/polylactic acid melt-blown cloth fiber.
The nano catalyst is one or more of titanium dioxide, iron or zinc.
The invention also provides a method for preparing the cigarette filter core material, which comprises the following steps:
a) preparing melt-blown cloth: uniformly stirring raw materials of polypropylene, polylactic acid and a compatibilizer by a stirrer according to a proportion, feeding the mixture into a double screw, and extruding and granulating the mixture to obtain mixed master batches; then, polypropylene-polylactic acid mixed melt-blown cloth fiber modified by the compatibilizer is obtained through a melt-blown process;
b) the nano catalyst loading process comprises the following steps: the adhesive and the nano catalyst are mixed according to the weight ratio of 1: (0.1-0.15), and uniformly stirring to prepare a spraying liquid; spraying the spraying liquid on polypropylene-polylactic acid mixed melt-blown fabric fibers modified by a compatibilizer to obtain a sprayed non-woven fabric;
c) drying: and drying the sprayed polypropylene-polylactic acid melt-blown cloth to obtain the filter element material of the cigarette filter.
Preferably, in the step a), the raw materials including polypropylene, polylactic acid and the compatibilizer are mixed according to a weight ratio of 1: (0.25-0.35): (0.03-0.1) in the ratio.
Preferably, the amount sprayed in step b) is from 15 to 25g/m2The spraying pressure range is between 0.08 and 0.1 MPa.
Preferably, the drying process in the step c) is heating to 100-110 ℃ for 15-20 min.
Has the advantages that:
1. the powerful and effective cigarette filter element prepared by the invention combines the polypropylene fiber and the polylactic acid fiber, has low material price and is easy to produce. The application of the polylactic acid reduces the harm of the cigarette filter tip to the environment.
2. The cigarette filter tip prepared by only using the polypropylene fiber has poor mouthfeel during use, and particularly, the cigarette filter tip has heavy pungency and is difficult to be accepted by smokers. The filter tip prepared by the invention has more refreshing mouthfeel, can give different feelings to smokers, and has excellent economic benefit.
3. The powerful and effective cigarette filter element prepared by the invention contains the nano metal catalyst capable of decomposing harmful substances such as low aldehydes, aliphatic hydrocarbon and the like, and provides better guarantee for the health of smokers.
Detailed Description
In order to enhance understanding of the present invention, the present invention will be described in further detail with reference to examples, which are provided for illustrating the present invention and are not limited to the examples.
Example 1
a) Preparing melt-blown fabric: raw materials of polypropylene (the melt index is 1200g/10min), levorotatory polylactic acid (the number average molecular weight is 100000-140000Mn) and polypropylene grafted maleic anhydride compatibilizer are mixed according to the weight ratio of 1: 0.35: 0.1 is evenly stirred by a stirrer and enters a double screw at 220 ℃, and the mixture is extruded and granulated to form mixed master batch. Then, the polypropylene/polylactic acid mixed melt-blown cloth fiber is obtained through the melt-blown process;
b) the nano catalyst loading process comprises the following steps: mixing a glycerol triacetate adhesive and a nano catalyst (titanium dioxide and iron are mixed according to a ratio of 4: 6) according to a weight ratio of 1: mixing at a ratio of 0.11, and stirring to obtain spray solution. Spraying the spraying liquid on the polypropylene/polylactic acid mixed melt-blown fabric fiber, wherein the spraying amount is 25g/m2Spraying at a pressure of 0.1mpa to obtain a sprayed non-woven fabric;
c) and (3) drying process: drying the sprayed non-woven fabric in a drying oven at 110 ℃ for 15min, and cooling to obtain the filter element material of the cigarette filter. ,
d) the filter element forming process comprises the following steps: and winding the obtained filter element material into roll paper, and forming by a cigarette filter element forming machine to obtain the cigarette filter element.
And (3) testing results: after cigarette smoke passes through the filter element of the cigarette filter, the removal rate of nicotine, tar and particles reaches 83.15 percent.
Example 2
a) Preparing melt-blown fabric: raw materials of polypropylene (the melt index is 1300g/10min), levorotatory polylactic acid (the number average molecular weight is 100000-140000Mn) and polyethylene glycol compatibilizer are mixed according to the weight ratio of 1: 0.30: 0.08 is evenly stirred by a stirrer and enters a double screw at the temperature of 210 ℃, and the mixture is extruded and granulated to form mixed master batch. Then, the polypropylene/polylactic acid mixed melt-blown cloth fiber is obtained through the melt-blown process;
b) the nano catalyst loading process comprises the following steps: mixing a glycerol triacetate adhesive and a nano catalyst (titanium dioxide and zinc in a ratio of 2: 8) according to a weight ratio of 1: 0.13, and stirring uniformly to prepare the spray coating liquid. Spraying the spraying liquid on the polypropylene/polylactic acid mixed melt-blown fabric fiber, wherein the spraying amount is 20g/m2Spraying at a pressure of 0.09mpa to obtain a sprayed non-woven fabric;
c) and (3) drying process: drying the sprayed non-woven fabric in a drying oven at 105 ℃ for 18min, and cooling to obtain the filter element material of the cigarette filter.
d) The filter element forming process comprises the following steps: and winding the obtained filter element material into roll paper, and forming by a cigarette filter element forming machine to obtain the cigarette filter element.
And (3) testing results: after cigarette smoke passes through the filter element of the cigarette filter tip, the removal rate of nicotine, tar and particles reaches 85.23 percent.
Example 3
a) Preparing melt-blown cloth: raw materials of polypropylene (the melt index is 1450g/10min), levorotatory polylactic acid (the number average molecular weight is 100000-140000Mn) and maleic anhydride compatibilizer are mixed according to the weight ratio of 1: 0.25: 0.05, stirring the mixture evenly by a stirrer, feeding the mixture into a double screw at 215 ℃, and extruding and granulating the mixture to obtain mixed master batches. Then, the polypropylene/polylactic acid mixed melt-blown cloth fiber is obtained through the melt-blown process;
b) the nano catalyst loading process comprises the following steps: mixing a glycerol triacetate adhesive and a nano catalyst (titanium dioxide, iron and zinc in a ratio of 2: 5: 3) according to a weight ratio of 1: 0.15, and uniformly stirring to prepare the spraying liquid. Spraying the spraying liquid on the polypropylene/polylactic acid mixed melt-blown fabric fiber, wherein the spraying amount is 17g/m2Spraying at a pressure of 0.08mpa to obtain a sprayed non-woven fabric;
c) and (3) drying process: drying the sprayed non-woven fabric in an oven at 100 ℃ for 20min, and cooling to obtain the filter element material of the cigarette filter.
d) The filter element forming process comprises the following steps: and winding the obtained filter element material into roll paper, and forming by a cigarette filter element forming machine to obtain the cigarette filter element.
And (3) testing results: after cigarette smoke passes through the filter element of the cigarette filter, the removal rate of nicotine, tar and particles reaches 82.64 percent.

Claims (8)

1. A filter element material for cigarette filter, which is characterized in that: the polypropylene-polylactic acid composite melt-blown fabric consists of polypropylene-polylactic acid composite melt-blown fabric fiber modified by a compatibilizer and a nano catalyst adhered on the melt-blown fabric through an adhesive; wherein the weight ratio of the adhesive to the nano catalyst is 1: (0.1-0.15), the nano catalyst is loaded on the melt-blown cloth fiber through a spraying process and a drying process, and the nano catalyst is adhered on the melt-blown cloth fiber through an adhesive.
2. A filter element material of a cigarette filter according to claim 1, characterized in that the compatibilizer modified polypropylene-polylactic acid composite melt-blown fabric fiber is prepared by mixing polypropylene, polylactic acid and a compatibilizer in a weight ratio of 1: (0.25-0.35): (0.03-0.1) uniformly stirring the mixture in a double screw to form mixed master batches, and extruding the mixed master batches by a melt-blowing process to obtain the master batches.
3. The filter element material of cigarette filter according to claim 2, wherein the polypropylene is homo-polypropylene, and the melt index is 1200-1500g/10 min; the polylactic acid is L-polylactic acid, and the number average molecular weight is 100000-140000 Mn; the compatibilizer is one of polyethylene glycol, polypropylene grafted maleic anhydride or maleic anhydride.
4. A cigarette filter cartridge material as in claim 1 wherein the binder is triacetin; the nano catalyst is one or more of titanium dioxide, iron or zinc.
5. A method of making a cigarette filter element material of claim 1 comprising the steps of:
a) preparing melt-blown cloth: uniformly stirring raw materials of polypropylene, polylactic acid and a compatibilizer by a stirrer according to a proportion, feeding the mixture into a double screw, and extruding and granulating the mixture to obtain mixed master batches; then, polypropylene-polylactic acid mixed melt-blown cloth fiber modified by the compatibilizer is obtained through a melt-blown process;
b) the nano catalyst loading process comprises the following steps: the adhesive and the nano catalyst are mixed according to the weight ratio of 1: (0.1-0.15), and uniformly stirring to prepare a spraying liquid; spraying the spraying liquid on polypropylene-polylactic acid mixed melt-blown fabric fibers modified by a compatibilizer to obtain a sprayed non-woven fabric;
c) drying: and drying the sprayed polypropylene-polylactic acid melt-blown cloth to obtain the filter element material of the cigarette filter.
6. The method according to claim 5, characterized in that in step a) the raw polypropylene, polylactic acid and compatibilizer are mixed in a weight ratio of 1: (0.25-0.35): (0.03-0.1) in the ratio.
7. The method according to claim 5, characterized in that the amount sprayed in step b) is 15-25g/m2The spraying pressure range is between 0.08 and 0.1 MPa.
8. The method as claimed in claim 5, wherein the drying process in step c) is heating to 100 ℃ and 110 ℃ for 15-20 min.
CN202010658385.6A 2020-07-09 2020-07-09 Filter core material of cigarette filter tip and preparation method Pending CN112273715A (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
CN202010658385.6A CN112273715A (en) 2020-07-09 2020-07-09 Filter core material of cigarette filter tip and preparation method

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
CN202010658385.6A CN112273715A (en) 2020-07-09 2020-07-09 Filter core material of cigarette filter tip and preparation method

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Publication Number Publication Date
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Citations (6)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US20020096300A1 (en) * 1999-03-11 2002-07-25 Yoichiro Yamashita Biodegradable cellulose acetate structure and tobacco filter
US20110151737A1 (en) * 2009-12-17 2011-06-23 3M Innovative Properties Company Dimensionally stable nonwoven fibrous webs and methods of making and using the same
CN102669820A (en) * 2012-05-23 2012-09-19 苏州大学 Cigarette filter and preparation method thereof
WO2015160027A1 (en) * 2014-04-18 2015-10-22 구기승 Environment-friendly short fiber non-woven fabric and method for manufacturing same
CN206101573U (en) * 2016-09-05 2017-04-19 江苏大亚滤嘴材料有限公司 Short fiber filled formula of polypropylene nonwoven filter tip for cigarette
CN110575708A (en) * 2019-10-14 2019-12-17 湖州禾海材料科技有限公司 preparation method of polypropylene filter material

Patent Citations (6)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US20020096300A1 (en) * 1999-03-11 2002-07-25 Yoichiro Yamashita Biodegradable cellulose acetate structure and tobacco filter
US20110151737A1 (en) * 2009-12-17 2011-06-23 3M Innovative Properties Company Dimensionally stable nonwoven fibrous webs and methods of making and using the same
CN102669820A (en) * 2012-05-23 2012-09-19 苏州大学 Cigarette filter and preparation method thereof
WO2015160027A1 (en) * 2014-04-18 2015-10-22 구기승 Environment-friendly short fiber non-woven fabric and method for manufacturing same
CN206101573U (en) * 2016-09-05 2017-04-19 江苏大亚滤嘴材料有限公司 Short fiber filled formula of polypropylene nonwoven filter tip for cigarette
CN110575708A (en) * 2019-10-14 2019-12-17 湖州禾海材料科技有限公司 preparation method of polypropylene filter material

Non-Patent Citations (1)

* Cited by examiner, † Cited by third party
Title
杨钦等: "可生物降解聚乳酸/助剂/聚丙烯复合纺粘非织造布的制备与性能研究", 《化工新型材料》 *

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Application publication date: 20210129

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