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CN111875477A - Azeotropic purification method of o-chlorohydrin - Google Patents

Azeotropic purification method of o-chlorohydrin Download PDF

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Publication number
CN111875477A
CN111875477A CN202010769628.3A CN202010769628A CN111875477A CN 111875477 A CN111875477 A CN 111875477A CN 202010769628 A CN202010769628 A CN 202010769628A CN 111875477 A CN111875477 A CN 111875477A
Authority
CN
China
Prior art keywords
chlorohydrin
purification method
water
azeotrope
azeotropic
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Pending
Application number
CN202010769628.3A
Other languages
Chinese (zh)
Inventor
王卫华
段季
周勇
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Yueyang Longxing Industrial Co ltd
Original Assignee
Yueyang Longxing Industrial Co ltd
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Yueyang Longxing Industrial Co ltd filed Critical Yueyang Longxing Industrial Co ltd
Priority to CN202010769628.3A priority Critical patent/CN111875477A/en
Publication of CN111875477A publication Critical patent/CN111875477A/en
Pending legal-status Critical Current

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Classifications

    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07CACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C29/00Preparation of compounds having hydroxy or O-metal groups bound to a carbon atom not belonging to a six-membered aromatic ring
    • C07C29/74Separation; Purification; Use of additives, e.g. for stabilisation
    • C07C29/76Separation; Purification; Use of additives, e.g. for stabilisation by physical treatment
    • C07C29/80Separation; Purification; Use of additives, e.g. for stabilisation by physical treatment by distillation
    • C07C29/82Separation; Purification; Use of additives, e.g. for stabilisation by physical treatment by distillation by azeotropic distillation
    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07CACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C29/00Preparation of compounds having hydroxy or O-metal groups bound to a carbon atom not belonging to a six-membered aromatic ring
    • C07C29/74Separation; Purification; Use of additives, e.g. for stabilisation
    • C07C29/76Separation; Purification; Use of additives, e.g. for stabilisation by physical treatment
    • C07C29/80Separation; Purification; Use of additives, e.g. for stabilisation by physical treatment by distillation

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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)

Abstract

The invention discloses an azeotropic purification method of o-chlorohydrin, the invention only needs the vacuum degree of about-0.080 Mpa to realize normal production, and reduces the distillation temperature, reduces the possibility of over-temperature, effectively prevents corrosive gas, and greatly prolongs the service life of equipment and pipelines; the production period of each batch can be shortened by more than 2-4h, the steam is saved by 1-2 tons, and the energy is saved.

Description

Azeotropic purification method of o-chlorohydrin
The technical field is as follows:
the invention belongs to the field of chemical industry, and particularly relates to an azeotropic purification method of o-chlorohydrin.
Background art:
the o-chlorohydrin needs to be purified after production, and the existing purification method has high requirements on vacuum degree, namely the vacuum degree of-0.095 Mpa and rectification at the temperature of 128-130 ℃, so that the vacuum pump has high requirements. Under the condition of insufficient vacuum degree, the material is easy to decompose to generate corrosive gas due to over-temperature, so that equipment and pipelines are corroded. And the production cycle is long and the energy consumption is high.
The invention content is as follows:
the invention aims to provide an azeotropic purification method of o-chlorohydrin, the invention can realize normal production only by vacuum degree of about-0.080 Mpa, and reduce distillation temperature, reduce possibility of over-temperature, effectively prevent corrosive gas, and greatly prolong the service life of equipment and pipelines; the production period of each batch can be shortened by more than 2-4h, the steam is saved by 1-2 tons, and the energy is saved.
In order to solve the problems, the technical scheme of the invention is as follows:
an azeotropic purification method of o-chlorohydrin, comprising the following steps:
step one, in the later stage of the o-chloroalcoholic acid acidification distillation, continuously adding water into an o-chloroalcoholic acid acidification reaction kettle at a certain flow rate; water and o-chlorohydrin containing a small amount of light components are subjected to azeotropy to form an azeotrope, and then the azeotrope is heated and rectified to be extracted from the tower top into an intermediate tank; the light fraction is separated off in this way;
step two, standing the azeotrope in an intermediate tank to divide water and obtain an upper oil phase; adding into a rectifying still for circular rectification to obtain the ortho-chlorohydrin.
Further improvement, the temperature of the rectification in the first step is 100-105 ℃; the pressure is-0.075-0.085 MPa.
In a further improvement, the flow rate of the water is 150-200 kg/h.
The invention has the advantages that:
1. normal production can be realized only by vacuum degree of about-0.080 Mpa.
2. The distillation temperature is reduced, the possibility of overtemperature is reduced, corrosive gas is effectively prevented from being generated, and the service lives of equipment and pipelines are greatly prolonged.
3. The production period of each batch can be shortened by more than 2-4h, the steam is saved by 1-2 tons, and the energy is saved.
The specific implementation mode is as follows:
in order to make the aforementioned objects, features and advantages of the present invention comprehensible, embodiments accompanied with figures are described in detail below.
Example 1
The invention relates to an o-chlorohydrin azeotropic purification device, which comprises a rectifying tower kettle, a product tank intermediate tank and a circulating pump. The using method of the invention is as follows:
1. continuously adding water into a rectifying tower kettle at a certain flow rate in the later stage of the o-chloroalcoholic acid distillation; water and o-chlorohydrin containing a small amount of light components azeotropy to form an azeotrope, and the azeotrope is extracted from the tower top to an intermediate tank through rectification. In this way the light fraction is separated off.
2. The azeotrope is kept stand in an intermediate tank for water diversion, an upper oil phase (containing a small amount of light component of the ortho-chlorohydrin) is added into a rectifying still for cyclic application, and then the rectified product is input into a product tank.
The above-mentioned embodiment is only a specific embodiment of the present invention, and is not meant to be a limitation of the present invention, and any simple modification and replacement thereof are within the scope of the present invention.

Claims (3)

1. An o-chlorohydrin azeotropic purification method is characterized by comprising the following steps:
step one, in the later stage of the o-chloroalcoholic acid acidification distillation, continuously adding water into an o-chloroalcoholic acid acidification reaction kettle at a certain flow rate; water and o-chlorohydrin containing a small amount of light components are subjected to azeotropy to form an azeotrope, and then the azeotrope is heated and rectified to be extracted from the tower top into an intermediate tank; the light fraction is separated off in this way;
step two, standing the azeotrope in an intermediate tank to divide water and obtain an upper oil phase; adding into a rectifying still for circular rectification to obtain the ortho-chlorohydrin.
2. The azeotropic purification method of o-chlorohydrin as claimed in claim 1, wherein the temperature of the distillation in the first step is 100-105 ℃; the pressure is-0.07 to-0.085 MPa.
3. The azeotropic purification method of o-chlorohydrin as claimed in claim 1, wherein the flow rate of the water is 150-200 kg/h.
CN202010769628.3A 2020-08-03 2020-08-03 Azeotropic purification method of o-chlorohydrin Pending CN111875477A (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
CN202010769628.3A CN111875477A (en) 2020-08-03 2020-08-03 Azeotropic purification method of o-chlorohydrin

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
CN202010769628.3A CN111875477A (en) 2020-08-03 2020-08-03 Azeotropic purification method of o-chlorohydrin

Publications (1)

Publication Number Publication Date
CN111875477A true CN111875477A (en) 2020-11-03

Family

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Family Applications (1)

Application Number Title Priority Date Filing Date
CN202010769628.3A Pending CN111875477A (en) 2020-08-03 2020-08-03 Azeotropic purification method of o-chlorohydrin

Country Status (1)

Country Link
CN (1) CN111875477A (en)

Citations (9)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JPS58198477A (en) * 1982-05-12 1983-11-18 Sumitomo Chem Co Ltd Recovery of epihalohydrin
US5227541A (en) * 1990-07-17 1993-07-13 Showa Denko K.K. Purification of 2,3-dichloro-1-propanol
CN101007751A (en) * 2007-01-26 2007-08-01 江苏工业学院 Preparation method of dichloro propanol from glycerin
TW200940489A (en) * 2005-05-20 2009-10-01 Solvay Process for producing a chlorohydrin
CN101657405A (en) * 2007-04-12 2010-02-24 陶氏环球技术公司 Process and apparatus for azeotropic recovery of dichlorohydrins
CN102976897A (en) * 2012-12-18 2013-03-20 山东科技大学 Method for purifying tetrafluoro propanol
CN103694082A (en) * 2013-11-26 2014-04-02 浙江巨圣氟化学有限公司 Method for purifying tetrafluoro propanol
CN106831339A (en) * 2016-12-19 2017-06-13 西安近代化学研究所 A kind of method for isolating and purifying trifluoroethanol and water azeotropic mixture
CN107445799A (en) * 2016-05-31 2017-12-08 王圣洁 Apparatus for producing dichloropropanol and method for producing the same

Patent Citations (9)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JPS58198477A (en) * 1982-05-12 1983-11-18 Sumitomo Chem Co Ltd Recovery of epihalohydrin
US5227541A (en) * 1990-07-17 1993-07-13 Showa Denko K.K. Purification of 2,3-dichloro-1-propanol
TW200940489A (en) * 2005-05-20 2009-10-01 Solvay Process for producing a chlorohydrin
CN101007751A (en) * 2007-01-26 2007-08-01 江苏工业学院 Preparation method of dichloro propanol from glycerin
CN101657405A (en) * 2007-04-12 2010-02-24 陶氏环球技术公司 Process and apparatus for azeotropic recovery of dichlorohydrins
CN102976897A (en) * 2012-12-18 2013-03-20 山东科技大学 Method for purifying tetrafluoro propanol
CN103694082A (en) * 2013-11-26 2014-04-02 浙江巨圣氟化学有限公司 Method for purifying tetrafluoro propanol
CN107445799A (en) * 2016-05-31 2017-12-08 王圣洁 Apparatus for producing dichloropropanol and method for producing the same
CN106831339A (en) * 2016-12-19 2017-06-13 西安近代化学研究所 A kind of method for isolating and purifying trifluoroethanol and water azeotropic mixture

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Address after: 414014 Yuehua second industrial zone, Yunxi District, Yueyang City, Hunan Province

Applicant after: Yueyang Longxing Industrial Co.,Ltd.

Address before: 414014 Yuehua second industrial zone, Yunxi District, Yueyang City, Hunan Province

Applicant before: Yueyang Longxing Industrial Co.,Ltd.

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Application publication date: 20201103

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